The impact of seasonalities on direct radiative effects and radiative heating rates of absorbing aerosols above clouds

2017 ◽  
Vol 143 (704) ◽  
pp. 1395-1405 ◽  
Author(s):  
Ian Chang ◽  
Sundar A. Christopher
2016 ◽  
Vol 29 (8) ◽  
pp. 2741-2763 ◽  
Author(s):  
Bryce E. Harrop ◽  
Dennis L. Hartmann

Abstract The relationship between the tropical circulation and cloud radiative effect is investigated. Output from the Clouds On–Off Klimate Intercomparison Experiment (COOKIE) is used to examine the impact of cloud radiative effects on circulation and climate. In aquaplanet simulations with a fixed SST pattern, the cloud radiative effect leads to an equatorward contraction of the intertropical convergence zone (ITCZ) and a reduction of the double ITCZ problem. It is shown that the cloud radiative heating in the upper troposphere increases the temperature, weakens CAPE, and inhibits the onset of convection until it is closer to the equator, where SSTs are higher. Precipitation peaks at higher values in a narrower band when the cloud radiative effects are active, compared to when they are inactive, owing to the enhancement in moisture convergence. Additionally, cloud–radiation interactions strengthen the mean meridional circulation and consequently enhance the moisture convergence. Although the mean tropical precipitation decreases, the atmospheric cloud radiative effect has a strong meridional gradient, which supports stronger poleward energy flux and speeds up the Hadley circulation. Cloud radiative heating also enhances cloud water path (liquid plus ice), which, combined with the reduction in precipitation, suggests that the cloud radiative heating reduces precipitation efficiency in these models.


2004 ◽  
Vol 22 (5) ◽  
pp. 1421-1434 ◽  
Author(s):  
A. Chakraborty ◽  
S. K. Satheesh ◽  
R. S. Nanjundiah ◽  
J. Srinivasan

Abstract. The impact of anthropogenic absorbing aerosols (such as soot) on the climate over the Indian region has been studied using the NCMRWF general circulation model. The absorbing aerosols increase shortwave radiative heating of the lower troposphere and reduce the heating at the surface. These effects have been incorporated as heating of the lower troposphere (up to 700hPa) and cooling over the continental surface based on INDOEX measurements. The heating effect is constant in the pre-monsoon season and reduces to zero during the monsoon season. It is shown that even in the monsoon season when the aerosol forcing is zero, there is an overall increase in rainfall and a reduction in surface temperature over the Indian region. The rainfall averaged over the Tropics shows a small reduction in most of the months during the January to September period. The impact of aerosol forcing, the model's sensitivity to this forcing and its interaction with model-physics has been studied by changing the cumulus parameterization from the Simplified Arakawa-Schubert (SAS) scheme to the Kuo scheme. During the pre-monsoon season the major changes in precipitation occur in the oceanic Inter Tropical Convergence Zone (ITCZ), where both the schemes show an increase in precipitation. This result is similar to that reported in Chung2002. On the other hand, during the monsoon season the changes in precipitation in the continental region are different in the SAS and Kuo schemes. It is shown that the heating due to absorbing aerosols changes the vertical moist-static stability of the atmosphere. The difference in the precipitation changes in the two cumulus schemes is on account of the different responses in the two parameterization schemes to changes in vertical stability. Key words. Atmospheric composition and structure (aerosols and particles) – Meteorology and atmospheric dynamics (tropical meteorology; precipitation)


2021 ◽  
Author(s):  
Jing Feng ◽  
Yi Huang

Abstract. The tropical tropopause layer (TTL) is the transition layer between the troposphere and the stratosphere. Tropical cyclones may impact the TTL by perturbing the vertical distributions of cloud, temperature, and water vapor, although this impact is poorly quantified due to the lack of collocated data. To address this problem, we implement a synergistic retrieval approach to obtain the thermodynamic profiles and ice water content above thick high-level clouds using the A-Train satellite measurements that pass over the tropical cyclones. This study detects the signature of cyclone impact on the distribution patterns of cloud, water vapor, temperature, and radiation by compositing these thermodynamic fields with respect to cyclone center locations. It is found that tropical cyclone events considerably increase the occurrence of TTL clouds, in the form of cirrus clouds above a clear troposphere. The amount of TTL cloud ice, however, is found to be mostly contributed by overshooting deep convections that penetrate the bottom of TTL. Using the synergistic retrieval method, we find a vertically oscillating pattern of temperature anomalies above tropical cyclones, with warming beneath the cloud top (around 16 km) and cooling above. The atmospheric column above 16 km is generally hydrated by overshooting convections, although dehydration is detected above non-overshooting TTL clouds. Above overshooting deep convections, the column-integrated water vapor is found to be on average 40 % higher than the climatology. Moreover, the TTL above tropical cyclones is cooled due to longwave radiative cooling. The radiative heating rates above cyclones are well differentiated by the brightness temperature of a satellite infrared channel in the window band. Using radiative calculations, it is found that TTL hydration is usually associated with radiative cooling of the TTL, which inhibits the diabatic ascent of moist air. The radiative balance of the TTL under the impact of the cyclone, therefore, is not in favor of maintaining the moist anomalies in the TTL or transporting water vertically to the stratosphere.


Atmosphere ◽  
2018 ◽  
Vol 9 (10) ◽  
pp. 377 ◽  
Author(s):  
Qiang Fu ◽  
Maxwell Smith ◽  
Qiong Yang

A single-column radiative-convective model (RCM) is a useful tool to investigate the physical processes that determine the tropical tropopause layer (TTL) temperature structures. Previous studies on the TTL using the RCMs, however, omitted the cloud radiative effects. In this study, we examine the impact of cloud radiative effects on the simulated TTL temperatures using an RCM. We derive the cloud radiative effects based on satellite observations, which show heating rates in the troposphere but cooling rates in the stratosphere. We find that the cloud radiative effect warms the TTL by as much as 2 K but cools the lower stratosphere by as much as −1.5 K, resulting in a thicker TTL. With (without) considering cloud radiative effects, we obtain a convection top of ≈167 hPa (≈150 hPa) with a temperature of ≈213 K (≈209 K), and a cold point at ≈87 hPa (≈94 hPa) with a temperature of ≈204 K (≈204 K). Therefore, the cloud radiative effects widen the TTL by both lowering the convection-top height and enhancing the cold-point height. We also examine the impact of TTL cirrus radiative effects on the RCM-simulated temperatures. We find that the TTL cirrus warms the TTL with a maximum temperature increase of ≈1.3 K near 110 hPa.


2016 ◽  
Vol 16 (1) ◽  
pp. 247-264 ◽  
Author(s):  
Y. Feng ◽  
V. R. Kotamarthi ◽  
R. Coulter ◽  
C. Zhao ◽  
M. Cadeddu

Abstract. Aerosol radiative effects and thermodynamic responses over South Asia are examined with the Weather Research and Forecasting model coupled with Chemistry (WRF-Chem) for March 2012. Model results of aerosol optical depths (AODs) and extinction profiles are analyzed and compared to satellite retrievals and two ground-based lidars located in northern India. The WRF-Chem model is found to heavily underestimate the AOD during the simulated pre-monsoon month and about 83 % of the model's low bias is due to aerosol extinctions below  ∼  2 km. Doubling the calculated aerosol extinctions below 850 hPa generates much better agreement with the observed AOD and extinction profiles averaged over South Asia. To separate the effect of absorption and scattering properties, two runs were conducted: in one run (Case I), the calculated scattering and absorption coefficients were increased proportionally, while in the second run (Case II) only the calculated aerosol scattering coefficient was increased. With the same AOD and extinction profiles, the two runs produce significantly different radiative effects over land and oceans. On the regional mean basis, Case I generates 48 % more heating in the atmosphere and 21 % more dimming at the surface than Case II. Case I also produces stronger cooling responses over the land from the longwave radiation adjustment and boundary layer mixing. These rapid adjustments offset the stronger radiative heating in Case I and lead to an overall lower-troposphere cooling up to −0.7 K day−1, which is smaller than that in Case II. Over the ocean, direct radiative effects dominate the heating rate changes in the lower atmosphere lacking such surface and lower atmosphere adjustments due to fixed sea surface temperature, and the strongest atmospheric warming is obtained in Case I. Consequently, atmospheric dynamics (boundary layer heights and meridional circulation) and thermodynamic processes (water vapor and cloudiness) are shown to respond differently between Case I and Case II, underlining the importance of determining the exact portion of scattering or absorbing aerosols that lead to the underestimation of aerosol optical depth in the model. In addition, the model results suggest that both the direct radiative effect and rapid thermodynamic responses need to be quantified for understanding aerosol radiative impacts.


2018 ◽  
Vol 18 (16) ◽  
pp. 12105-12121 ◽  
Author(s):  
Thomas Fauchez ◽  
Steven Platnick ◽  
Tamás Várnai ◽  
Kerry Meyer ◽  
Céline Cornet ◽  
...  

Abstract. In a context of global climate change, the understanding of the radiative role of clouds is crucial. On average, ice clouds such as cirrus have a significant positive radiative effect, but under some conditions the effect may be negative. However, many uncertainties remain regarding the role of ice clouds on Earth's radiative budget and in a changing climate. Global satellite observations are particularly well suited to monitoring clouds, retrieving their characteristics and inferring their radiative impact. To retrieve ice cloud properties (optical thickness and ice crystal effective size), current operational algorithms assume that each pixel of the observed scene is plane-parallel and homogeneous, and that there is no radiative connection between neighboring pixels. Yet these retrieval assumptions are far from accurate, as real radiative transfer is 3-D. This leads to the plane-parallel and homogeneous bias (PPHB) plus the independent pixel approximation bias (IPAB), which impacts both the estimation of top-of-the-atmosphere (TOA) radiation and the retrievals. An important factor that determines the impact of these assumptions is the sensor spatial resolution. High-spatial-resolution pixels can better represent cloud variability (low PPHB), but the radiative path through the cloud can involve many pixels (high IPAB). In contrast, low-spatial-resolution pixels poorly represent the cloud variability (high PPHB), but the radiation is better contained within the pixel field of view (low IPAB). In addition, the solar and viewing geometry (as well as cloud optical properties) can modulate the magnitude of the PPHB and IPAB. In this, Part II of our study, we simulate TOA 0.86 and 2.13 µm solar reflectances over a cirrus uncinus scene produced by the 3DCLOUD model. Then, 3-D radiative transfer simulations are performed with the 3DMCPOL code at spatial resolutions ranging from 50 m to 10 km, for 12 viewing geometries and nine solar geometries. It is found that, for simulated nadir observations taken at resolution higher than 2.5 km, horizontal radiation transport (HRT) dominates biases between 3-D and 1-D reflectance calculations, but these biases are mitigated by the side illumination and shadowing effects for off-zenith solar geometries. At resolutions coarser than 2.5 km, PPHB dominates. For off-nadir observations at resolutions higher than 2.5 km, the effect that we call THEAB (tilted and homogeneous extinction approximation bias) due to the oblique line of sight passing through many cloud columns contributes to a large increase of the reflectances, but 3-D radiative effects such as shadowing and side illumination for oblique Sun are also important. At resolutions coarser than 2.5 km, the PPHB is again the dominant effect. The magnitude and resolution dependence of PPHB and IPAB is very different for visible, near-infrared and shortwave infrared channels compared with the thermal infrared channels discussed in Part I of this study. The contrast of 3-D radiative effects between solar and thermal infrared channels may be a significant issue for retrieval techniques that simultaneously use radiative measurements across a wide range of solar reflectance and infrared wavelengths.


2015 ◽  
Vol 15 (23) ◽  
pp. 13633-13646 ◽  
Author(s):  
B. L. Zhuang ◽  
T. J. Wang ◽  
J. Liu ◽  
Y. Ma ◽  
C. Q. Yin ◽  
...  

Abstract. Absorbing aerosols can significantly modulate short-wave solar radiation in the atmosphere, affecting regional and global climate. The aerosol absorption coefficient (AAC) is an indicator that assesses the impact of absorbing aerosols on radiative forcing. In this study, the near-surface AAC and absorption Ångström exponent (AAE) in the urban area of Nanjing, China, are characterized on the basis of measurements in 2012 and 2013 using the seven-channel Aethalometer (model AE-31, Magee Scientific, USA). The AAC is estimated with direct and indirect corrections, which result in consistent temporal variations and magnitudes of AAC at 532 nm. The mean AAC at 532 nm is about 43.23 ± 28.13 M m−1 in the urban area of Nanjing, which is much lower than that in Pearl River Delta and the same as in rural areas (Lin'an) in Yangtze River Delta. The AAC in the urban area of Nanjing shows strong seasonality (diurnal variations); it is high in cold seasons (at rush hour) and low in summer (in the afternoon). It also shows synoptic and quasi-2-week cycles in response to weather systems. Its frequency distribution follows a typical log-normal pattern. The 532 nm AAC ranging from 15 to 65 M m−1 dominates, accounting for more than 72 % of the total data samples in the entire study period. Frequent high pollution episodes, such as those observed in June 2012 and in winter 2013, greatly enhanced AAC and altered its temporal variations and frequency distributions. These episodes are mostly due to local emissions and regional pollution. Air masses flowing from northern China to Nanjing can sometimes be highly polluted and lead to high AAC at the site. AAE at 660/470 nm from the Schmid correction (Schmid et al., 2006) is about 1.56, which might be more reasonable than from the Weingartner correction (Weingartner et al., 2003). Low AAEs mainly occur in summer, likely due to high relative humidity (RH) in the season. AAC increases with increasing AAE at a fixed aerosol loading. The RH–AAC relationship is more complex. Overall, AAC peaks at RH values of around 40 % (1.3 < AAE < 1.6), 65 % (AAE < 1.3 and AAE > 1.6), and 80 % (1.3 < AAE < 1.6).


2020 ◽  
Vol 33 (15) ◽  
pp. 5527-5542
Author(s):  
Louis Rivoire ◽  
Thomas Birner ◽  
John A. Knaff ◽  
Natalie Tourville

AbstractA ubiquitous cold signal near the tropopause, here called “tropopause layer cooling” (TLC), has been documented in deep convective regions such as tropical cyclones (TCs). Temperature retrievals from the Constellation Observing System for Meteorology, Ionosphere, and Climate (COSMIC) reveal cooling of order 0.1–1 K day−1 on spatial scales of order 1000 km above TCs. Data from the Cloud Profiling Radar (onboard CloudSat) and from the Cloud–Aerosol Lidar with Orthogonal Polarization [onboard the Cloud–Aerosol Lidar and Infrared Pathfinder Satellite Observations (CALIPSO)] are used to analyze cloud distributions associated with TCs. Evidence is found that convective clouds within TCs reach the upper part of the tropical tropopause layer (TTL) more frequently than do convective clouds outside TCs, raising the possibility that convective clouds within TCs and associated cirrus clouds modulate TLC. The contribution of clouds to radiative heating rates is then quantified using the CloudSat and CALIPSO datasets: in the lower TTL (below the tropopause), clouds produce longwave cooling of order 0.1–1 K day−1 inside the TC main convective region, and longwave warming of order 0.01–0.1 K day−1 outside; in the upper TTL (near and above the tropopause), clouds produce longwave cooling of the same order as TLC inside the TC main convective region, and up to one order of magnitude smaller outside. Considering that clouds also produce shortwave warming, it is suggested that cloud radiative effects inside and outside TCs only explain modest amounts of TLC while other processes must provide the remaining cooling.


2021 ◽  
Author(s):  
Ulrike Niemeier ◽  
Felix Riede ◽  
Claudia Timmreck

&lt;p&gt;The large explosive eruption of the Laacher See volcano c. 12,900 yrs BP marked the end of explosive volcanism in the East Eifel volcanic zone (Germany). We have reviewed the current evidence for the impact of the Laacher See Eruption (LSE) on the immediate and wider environment as recorded in a range of proxies with a series of interactive stratospheric aerosol model experiments. Recent studies about the climate impact of NH extratropical eruptions and new insights about the dating of the LSE warrant a return to this cataclysmic eruption and its potential influence on Northern Hemisphere climate. Rather detailed reconstructions of its eruption dynamics have been proposed. The eruption might have lasted several weeks or even months, most likely with an initial (~10h) intense early phase resulting in deposits over north-east Germany and the Baltic Sea, and a slightly later and weaker phase leaving deposits south of the volcano towards the Alps.&lt;/p&gt;&lt;p&gt;Our interactive stratospheric aerosol model experiments are based on a reference LSE experiment with emission estimates of 20 Tg of sulfur dioxide (SO&lt;sub&gt;2&lt;/sub&gt;) and 200 Tg of fine-ash, across two eruptive phases in May and June. Additional sensitivity experiments reflect the estimated range of uncertainty of the injection rate and altitude and, assess how the solar-absorptive heating from the 150 Tg of sub-micron ash emitted in the first eruptive phase changed the LSE cloud&amp;#8217;s dispersion. Our simulations reveal that the heating of the ash likely played an important role in the transport of ash and sulfate. Depending on the altitude of the injection, our simulated volcanic cloud begins to rotate shortly after the eruption. This meso-cyclone, as well as the additional radiative heating of the fine ash then changes the dispersion of the cloud to be more southerly compared to dispersal estimated without fine-ash heating. Sulfate transport is similarly impacted by the heating of the ash, resulting in a stronger transport to low-latitudes, later arrival of the volcanic cloud in the Arctic regions and a longer lifetime compared to cases without injection of fine ash.&lt;/p&gt;


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