scholarly journals Simultaneous Control of Emission Localization and Two-Photon Absorption Efficiency in Dissymmetrical Chromophores

2010 ◽  
Vol 114 (9) ◽  
pp. 3152-3169 ◽  
Author(s):  
Claudine Katan ◽  
Marina Charlot ◽  
Olivier Mongin ◽  
Céline Le Droumaguet ◽  
Viatcheslav Jouikov ◽  
...  
2021 ◽  
Vol 4 (4) ◽  
Author(s):  
Edoardo Carnio ◽  
Andreas Buchleitner ◽  
Frank Schlawin

We investigate how entanglement can enhance two-photon absorption in a three-level system. First, we employ the Schmidt decomposition to determine the entanglement properties of the optimal two-photon state to drive such a transition, and the maximum enhancement which can be achieved in comparison to the optimal classical pulse. We then adapt the optimization problem to realistic experimental constraints, where photon pairs from a down-conversion source are manipulated by local operations such as spatial light modulators. We derive optimal pulse shaping functions to enhance the absorption efficiency, and compare the maximal enhancement achievable by entanglement to the yield of optimally shaped, separable pulses.


2015 ◽  
Vol 6 (10) ◽  
pp. 3783 ◽  
Author(s):  
Yalun Wang ◽  
Rongrong Hu ◽  
Wang Xi ◽  
Fuhong Cai ◽  
Shaowei Wang ◽  
...  

1996 ◽  
Vol 43 (9) ◽  
pp. 1765-1771 ◽  
Author(s):  
M. W. HAMILTON and D. S. ELLIOTT

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