Particulate-Phase and Gaseous Elemental Mercury Emissions During Biomass Combustion: Controlling Factors and Correlation with Particulate Matter Emissions

2008 ◽  
Vol 42 (3) ◽  
pp. 721-727 ◽  
Author(s):  
Daniel Obrist ◽  
Hans Moosmüller ◽  
Roger Schürmann ◽  
L.-W. Antony Chen ◽  
Sonia M. Kreidenweis
Keyword(s):  
Particulate Matter ◽  
Elemental Mercury ◽  
Controlling Factors ◽  
Biomass Combustion ◽  
Particulate Phase ◽  
Mercury Emissions ◽  
Gaseous Elemental Mercury ◽  
Particulate Matter Emissions

scholarly journals Speciated Atmospheric Mercury during Haze and Non-haze Days in an Inland City in China

2016 ◽  
Author(s):  
Qianqian Hong ◽  
Zhouqing Xie ◽  
Cheng Liu ◽  
Feiyue Wang ◽  
Pinhua Xie ◽  
...  
Keyword(s):  
Elemental Mercury ◽  
Atmospheric Mercury ◽  
Central China ◽  
Mercury Emissions ◽  
Gaseous Elemental Mercury ◽  
Enhanced Production ◽  
Mercury Transport ◽  
Haze Pollution ◽  
The Mean ◽  
Haze Days

Abstract. Long-term continuous measurements of speciated atmospheric mercury were conducted at Hefei, a mid-latitude inland city in east central China, from July 2013 to June 2014. The mean concentrations (± standard deviation) of gaseous elemental mercury (GEM), reactive gaseous mercury (RGM) and particle-bound mercury (PBM) were 3.95 ± 1.93 ng m−3, 2.49 ± 2.41 pg m−3 and 23.3 ± 90.8 pg m−3, respectively, during non-haze days, and 4.74 ± 1.62 ng m−3, 4.32 ± 8.36 pg m−3 and 60.2 ± 131.4 pg m−3, respectively, during haze days. Potential source contribution function (PSCF) analysis suggested that the atmospheric mercury pollution during haze days was caused primarily by local mercury emissions, instead of via long-range mercury transport. In addition, the disadvantageous diffussion during haze days will also enhance the level of atmospheric mercury. Compared to the GEM and RGM, change in PBM was more sensitive to the haze pollution. The mean PBM concentration during haze days was 2.5 times that during non-haze days due to elevated concentrations of particulate matter. A remarkable seasonal trend in PBM was observed with concentration decreasing in the following order in response to the frequency of haze days: autumn, winter, spring, summer. A distinct diurnal relationship was found between GEM and RGM during haze days, with the peak values of RGM coinciding with the decline in GEM. Using HgOH as an intermediate product during GEM oxidation, our results suggest that NO2 aggregation with HgOH could explain the enhanced production of RGM during the daytime in haze days. Increasing level of NOx will potentially accelerate the oxidation of GEM despite the decrease of solar radiation.

Gaseous mercury in coastal urban areas

2010 ◽  
Vol 7 (6) ◽  
pp. 537 ◽  
Author(s):  
Anne L. Soerensen ◽  
Henrik Skov ◽  
Matthew S. Johnson ◽  
Marianne Glasius
Keyword(s):  
Urban Areas ◽  
Marine Boundary Layer ◽  
Elemental Mercury ◽  
Atmospheric Mercury ◽  
Mercury Deposition ◽  
Mercury Emissions ◽  
Gaseous Elemental Mercury ◽  
Gaseous Mercury ◽  
Range Transport ◽  
Aquatic Food

Environmental context Mercury is a neurotoxin that bioaccumulates in the aquatic food web. Atmospheric emissions from urban areas close to the coast could cause increased local mercury deposition to the ocean. Our study adds important new data to the current limited knowledge on atmospheric mercury emissions and dynamics in coastal urban areas. Abstract Approximately 50% of primary atmospheric mercury emissions are anthropogenic, resulting from e.g. emission hotspots in urban areas. Emissions from urban areas close to the coast are of interest because they could increase deposition loads to nearby coastal waters as well as contribute to long range transport of mercury. We present results from measurements of gaseous elemental mercury (GEM) and reactive gaseous mercury (RGM) in 15 coastal cities and their surrounding marine boundary layer (MBL). An increase of 15–90% in GEM concentration in coastal urban areas was observed compared with the remote MBL. Strong RGM enhancements were only found in two cities. In urban areas with statistically significant GEM/CO enhancement ratios, slopes between 0.0020 and 0.0087 ng m–3 ppb–1 were observed, which is consistent with other observations of anthropogenic enhancement. The emission ratios were used to estimate GEM emissions from the areas. A closer examination of data from Sydney (Australia), the coast of Chile, and Valparaiso region (Chile) in the southern hemisphere, is presented.

scholarly journals Novel Test Bench for the Active Reduction of Biomass Particulate Matter Emissions

2020 ◽  
Vol 12 (1) ◽  
pp. 422 ◽  
Author(s):  
Raquel Pérez-Orozco ◽  
David Patiño ◽  
Jacobo Porteiro ◽  
José Luís Míguez
Keyword(s):  
Particulate Matter ◽  
Fixed Bed ◽  
Biomass Combustion ◽  
Particulate Emissions ◽  
Experimental Plant ◽  
Exhaust Temperature ◽  
Specific Effects ◽  
Bed Temperature ◽  
Particulate Matter Emissions ◽  
The Stability

This paper introduces an experimental plant specifically designed to challenge the main operating issues related to modern biomass combustion systems (mainly NOx, particulate matter, and deposition phenomena). The prototype is an 11–18 kW overfed fixed-bed burner with a modular configuration, and the design considers the implementation of certain strategies for improving combustion: (1) a complete refrigeration system that also includes the fuel bed; and (2) an air injection control through flue gas recirculation. First, the stability and repeatability of the facility were successfully tested, establishing the duration of transient periods in the phase of experiment design. The results revealed similar effects in temperature and particulate emissions when comparing the use of the cooling bed and recirculation techniques. Reductions of 15% and up to 70% were achieved for the exhaust temperature and particulate matter concentration, respectively. Otherwise, the refrigeration considerably reduced the bed temperature, especially in its core, which enhanced the condensation of volatile salts and therefore the fouling phenomena. Although the viability of using both techniques as temperature control methods is demonstrated, further studies are needed to clarify the specific effects of each technology and to clarify the possible significance of a hybrid solution that combines both strategies.

Bed cooling effects in solid particulate matter emissions during biomass combustion. A morphological insight

Energy ◽  
2020 ◽  
Vol 205 ◽  
pp. 118088 ◽  
Author(s):  
Raquel Pérez-Orozco ◽  
David Patiño ◽  
Jacobo Porteiro ◽  
José Luis Míguez
Keyword(s):  
Particulate Matter ◽  
Biomass Combustion ◽  
Particulate Matter Emissions ◽  
Cooling Effects

scholarly journals Trend of atmospheric mercury concentrations at Cape Point for 1995–2004 and since 2007

2017 ◽  
Vol 17 (3) ◽  
pp. 2393-2399 ◽  
Author(s):  
Lynwill G. Martin ◽  
Casper Labuschagne ◽  
Ernst-Günther Brunke ◽  
Andreas Weigelt ◽  
Ralf Ebinghaus ◽  
...  
Keyword(s):  
Biomass Burning ◽  
Wet Deposition ◽  
Southern Oscillation ◽  
Elemental Mercury ◽  
Atmospheric Mercury ◽  
Austral Spring ◽  
Mercury Emissions ◽  
Gaseous Elemental Mercury ◽  
Regional Processes

Abstract. Long-term measurements of gaseous elemental mercury (GEM) concentrations at Cape Point, South Africa, reveal a downward trend between September 1995 and December 2005 and an upward one from March 2007 until June 2015, implying a change in trend sign between 2004 and 2007. The trend change is qualitatively consistent with the trend changes in GEM concentrations observed at Mace Head, Ireland, and in mercury wet deposition over North America, suggesting a change in worldwide mercury emissions. Seasonally resolved trends suggest a modulation of the overall trend by regional processes. The trends in absolute terms (downward in 1995–2004 and upward in 2007–2015) are highest in austral spring (SON), coinciding with the peak in emissions from biomass burning in South America and southern Africa. The influence of trends in biomass burning is further supported by a biennial variation in GEM concentration found here and an El Niño–Southern Oscillation (ENSO) signature in GEM concentrations reported recently.

P-Based Additive for Reducing Fine Particulate Matter Emissions during Agricultural Biomass Combustion

2019 ◽  
Vol 33 (11) ◽  
pp. 11274-11284 ◽  
Author(s):  
Youjian Zhu ◽  
Jiyuan Fan ◽  
Peng Yang ◽  
Wei Cheng ◽  
Kuo Zeng ◽  
...  
Keyword(s):  
Particulate Matter ◽  
Fine Particulate Matter ◽  
Biomass Combustion ◽  
Agricultural Biomass ◽  
Fine Particulate ◽  
Particulate Matter Emissions

scholarly journals Trend of atmospheric mercury concentrations at Cape Point for 1995–2004 and since 2007

2016 ◽  
Author(s):  
Lynwill G. Martin ◽  
Casper Labuschagne ◽  
Ernst-Günther Brunke ◽  
Andreas Weigelt ◽  
Ralf Ebinghaus ◽  
...  
Keyword(s):  
South Africa ◽  
Biomass Burning ◽  
Wet Deposition ◽  
Elemental Mercury ◽  
Atmospheric Mercury ◽  
Austral Spring ◽  
Mercury Emissions ◽  
Gaseous Elemental Mercury ◽  
Regional Processes

Abstract. Long-term measurements of gaseous elemental mercury (GEM) concentrations at Cape Point, South Africa, reveal a downward trend between September 1995 and December 2005 and an upward one since March 2007 until June 2015 implying a change in trend sign between 2004 and 2007. The trend change is qualitatively consistent with the trend changes in GEM concentrations observed at Mace Head, Ireland, and in mercury wet deposition over North America suggesting a change in worldwide mercury emissions. Seasonally resolved trends suggest a modulation of the overall trend by regional processes. The trends in absolute terms (downward in 1995–2004 and upward in 2007–2015) are the highest in austral spring (SON) coinciding with the peak in emissions from biomass burning in South America and southern Africa. The influence of trends in biomass burning is further supported by a biennial variation in GEM concentration found here and an ENSO signature in GEM concentrations reported recently.

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