Observation of Energy-Dependent Carrier Scattering in Conducting Polymer Nanowire Blends for Enhanced Thermoelectric Performance

2020 ◽  
Vol 12 (30) ◽  
pp. 34451-34461 ◽  
Author(s):  
Xinyi Chen ◽  
Wen Shi ◽  
Kun Zhang
2015 ◽  
Vol 3 (42) ◽  
pp. 20896-20902 ◽  
Author(s):  
Xincheng Hu ◽  
Guangming Chen ◽  
Xin Wang ◽  
Hanfu Wang

The thermoelectric performance of PEDOT can be conveniently and effectively tuned by nanostructure evolution.


2015 ◽  
Vol 3 (27) ◽  
pp. 7045-7052 ◽  
Author(s):  
Yuanyue Li ◽  
Di Li ◽  
Xiaoying Qin ◽  
Xiuhui Yang ◽  
Yongfei Liu ◽  
...  

Owing to enhanced power factor and reduced lattice thermal conductivity through interface scattering, a largest thermoelectric figure of merit ZT = 1.61 is achieved at 467 K for BiSbTe based composite with Cu3SbSe4 nanoinclusions.


2017 ◽  
Vol 114 (40) ◽  
pp. 10548-10553 ◽  
Author(s):  
Jun Mao ◽  
Jing Shuai ◽  
Shaowei Song ◽  
Yixuan Wu ◽  
Rebecca Dally ◽  
...  

Achieving higher carrier mobility plays a pivotal role for obtaining potentially high thermoelectric performance. In principle, the carrier mobility is governed by the band structure as well as by the carrier scattering mechanism. Here, we demonstrate that by manipulating the carrier scattering mechanism in n-type Mg3Sb2-based materials, a substantial improvement in carrier mobility, and hence the power factor, can be achieved. In this work, Fe, Co, Hf, and Ta are doped on the Mg site of Mg3.2Sb1.5Bi0.49Te0.01, where the ionized impurity scattering crosses over to mixed ionized impurity and acoustic phonon scattering. A significant improvement in Hall mobility from ∼16 to ∼81 cm2⋅V−1⋅s−1 is obtained, thus leading to a notably enhanced power factor of ∼13 μW⋅cm−1⋅K−2 from ∼5 μW⋅cm−1⋅K−2. A simultaneous reduction in thermal conductivity is also achieved. Collectively, a figure of merit (ZT) of ∼1.7 is obtained at 773 K in Mg3.1Co0.1Sb1.5Bi0.49Te0.01. The concept of manipulating the carrier scattering mechanism to improve the mobility should also be applicable to other material systems.


2020 ◽  
Vol 12 (17) ◽  
pp. 19693-19700 ◽  
Author(s):  
Hongwei Ming ◽  
Chen Zhu ◽  
Xiaoying Qin ◽  
Jian Zhang ◽  
Di Li ◽  
...  

2017 ◽  
Vol 5 (1) ◽  
pp. 47-53 ◽  
Author(s):  
Jian Zhao ◽  
Dongxing Tan ◽  
Guangming Chen

The dependence of the PEDOT nanostructure’s thermoelectric performance on post-treatments with acid (H2SO4) and chemical reduction (Na2SO3) was reported.


Carbon ◽  
2020 ◽  
Vol 170 ◽  
pp. 191-198 ◽  
Author(s):  
Yang Zhao ◽  
Ying Li ◽  
Jixiang Qiao ◽  
Song Jiang ◽  
Pengyan Mao ◽  
...  

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