scholarly journals Emission State Structure and Linewidth Broadening Mechanisms in Type-II CdSe/CdTe Core–Crown Nanoplatelets: A Combined Theoretical–Single Nanocrystal Optical Study

2020 ◽  
Vol 124 (31) ◽  
pp. 17352-17363
Author(s):  
Violette Steinmetz ◽  
Juan I. Climente ◽  
Raj Pandya ◽  
Josep Planelles ◽  
Florent Margaillan ◽  
...  
2016 ◽  
Vol 2 (1) ◽  
pp. 174-181 ◽  
Author(s):  
Qiuyang Li ◽  
Boyang Zhou ◽  
James R. McBride ◽  
Tianquan Lian

2021 ◽  
Vol 96 (12) ◽  
pp. 125867
Author(s):  
Worasak Sukkabot

Abstract Utilizing the atomistic tight-binding theory, the impact of the lateral and vertical potential confinement by the coated shell on the CdSe/CdTe core/crown and core/shell nanoplatelets (NPLs) is attained. The spatial charge separation and encapsulated shell have a noteworthy impact on the electronic structures and optical properties because of the type-II band profile. The reduced band gaps with the growing laterally and vertically passivated shell thicknesses are due to the quantum confinement phenomena. The optical band gaps adjusted across the visible light are achieved by the shell thickness change. The excitonic binding energies of CdSe/CdTe core/shell NPLs are larger than those of CdSe/CdTe core/crown NPLs. Thanks to the spatial charge separation, a shortening of the oscillation strengths is concomitant with an increase of the radiative lifetimes. Overall, this scientific research underlines the importance of the theoretical understanding and practical control by lateral and vertical confinement of heterostructure NPLs.


1991 ◽  
Vol 59 (1) ◽  
pp. 96-98 ◽  
Author(s):  
Satoshi Sasaki ◽  
Noboru Miura ◽  
Yoshiji Horikoshi

2017 ◽  
Vol 90 (1) ◽  
pp. 52-58 ◽  
Author(s):  
Taichi Watanabe ◽  
Kohji Takahashi ◽  
Kunio Shimura ◽  
Hang-Beom Bu ◽  
Kim Hyeon-Deuk ◽  
...  

Author(s):  
Nguyen Xuan Ca ◽  
Nguyen Thi Hien

The CdSe, type-II CdSe/CdTe core/shell and type-II/type-I CdSe/CdTe/ZnS core/shell/shell  quantum dots (QDs) were successfully synthesized in a noncoordinating solvent. The phonon characterizations, optical properties and structures of the synthesized QDs were characterized by Raman scattering (RS) spectra, photoluminescence (PL) spectroscopy, PL-decay lifetime, absorption spectroscopy (Abs), and X-ray diffraction (XRD). The growth of QDs was monitored by using RS, which demonstrated the formation of correct of the core/shell and core/shell/shell structures. Observation results from XRD reveal that all QDs crystallize in the cubic phase with zinc-blende structure. The typical characteristics of spatially indirect recombination for type-II QDs were observed through Abs and PL spectroscopy. The ZnS shell significantly enhanced the PL quantum yeild (QY), the optical durability, the chemical stability and separating CdSe/CdTe QDs from the surroundings. The effect of excitation power on the PL properties of the CdSe core,  CdSe/CdTe and CdSe/CdTe/ZnS QDs has been investigated.


Nanoscale ◽  
2015 ◽  
Vol 7 (6) ◽  
pp. 2698-2707 ◽  
Author(s):  
Partha Maity ◽  
Tushar Debnath ◽  
Uday Chopra ◽  
Hirendra Nath Ghosh

For the first time ultrafast cascading hole and electron transfer dynamics in a CdS/CdTe type II core–shell sensitized with a molecular adsorbate (Br-PGR) have been demonstrated using transient absorption spectroscopy.


2014 ◽  
Vol 136 (46) ◽  
pp. 16430-16438 ◽  
Author(s):  
Silvia Pedetti ◽  
Sandrine Ithurria ◽  
Hadrien Heuclin ◽  
Gilles Patriarche ◽  
Benoit Dubertret
Keyword(s):  
Type Ii ◽  

2015 ◽  
Vol 119 (4) ◽  
pp. 2177-2185 ◽  
Author(s):  
Yusuf Kelestemur ◽  
Murat Olutas ◽  
Savas Delikanli ◽  
Burak Guzelturk ◽  
Mehmet Zafer Akgul ◽  
...  
Keyword(s):  
Type Ii ◽  

2016 ◽  
Vol 4 (30) ◽  
pp. 7223-7229 ◽  
Author(s):  
Qingli Lin ◽  
Bin Song ◽  
Hongzhe Wang ◽  
Fengjuan Zhang ◽  
Fei Chen ◽  
...  

Highly efficient deep-red light-emitting diodes (LEDs) fabricated by using type-II CdTe/CdSe quantum dots.


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