Phosphate-Doped Carbon Black as Pt Catalyst Support: Co-catalytic Functionality for Dimethyl Ether and Methanol Electro-oxidation

2013 ◽  
Vol 1 (2) ◽  
pp. 448-454 ◽  
Author(s):  
Min Yin ◽  
Yunjie Huang ◽  
Qingfeng Li ◽  
Jens Oluf Jensen ◽  
Lars N. Cleemann ◽  
...  
Keyword(s):  
Carbon Black ◽  
Dimethyl Ether ◽  
Catalyst Support ◽  
Pt Catalyst ◽  
Electro Oxidation

INVESTIGATION OF THE ELECTROCHEMICAL BEHAVIOR OF HEAT-TREATED CARBON BLACKS AND Pt/C CATALYSTS

2002 ◽  
Vol 09 (03n04) ◽  
pp. 1443-1452 ◽  
Author(s):  
C. D. HUANG ◽  
Z. T. XIONG ◽  
J. Y. LIN ◽  
K. L. TAN
Keyword(s):  
Carbon Black ◽  
Electrochemical Behavior ◽  
Catalyst Support ◽  
Carbon Surface ◽  
Carbon Blacks ◽  
Heat Treated ◽  
Platinum Particles ◽  
Electro Oxidation ◽  
Treated Carbon ◽  
Xps Study

In this paper we report the electrochemical behavior of heat-treated carbon blacks and Pt/C catalysts. Cyclic voltammetry indicates that the heat-treated carbon black as catalyst support does not improve the Pt/C catalyst's activity for methanol oxidation. An XPS study of a Pt-loaded carbon black indicates that the amounts of oxidized platinum and oxygen-functional groups on catalysts are decreased when the platinum particles are deposited on the heat-treated carbon surface. These changes in the surface and crystalline structural properties of carbon materials lead to the catalytic activity change in methanol electro-oxidation.

scholarly journals Preparation and Characterization of Zirconia-Coated Nanodiamonds as a Pt Catalyst Support for Methanol Electro-Oxidation

Nanomaterials ◽  
2016 ◽  
Vol 6 (12) ◽  
pp. 234 ◽  
Author(s):  
Jing Lu ◽  
Jianbing Zang ◽  
Yanhui Wang ◽  
Yongchao Xu ◽  
Xipeng Xu
Keyword(s):  
Catalyst Support ◽  
Pt Catalyst ◽  
Electro Oxidation

Effect of Nitric Acid on Modified Mesoporous Carbon as Catalyst Support of Direct Methanol Fuel Cell

2013 ◽  
Vol 10 (5) ◽  
Author(s):  
Qiao-xia Li ◽  
Hong-min Mao ◽  
Jin-guang Li ◽  
Qun-jie Xu
Keyword(s):  
Nitric Acid ◽  
Mesoporous Carbon ◽  
Chemical Reduction ◽  
Energy Dispersive Spectrometer ◽  
Catalyst Support ◽  
Pt Catalyst ◽  
Acid Media ◽  
Composite Catalysts ◽  
Direct Methanol ◽  
Electro Oxidation

Nitric acid modified Mesoporous carbon (CMK-3) supported Pt particles have been prepared by chemical reduction with NaBH4 as a reducing agent. Energy dispersive spectrometer shows that the catalysts have some oxygenic functional groups. The activity of the composite catalysts for methanol electro-oxidation was investigated by using cyclic votammogram and chronoamperometry in acid media. The results indicated that modified mesoporous carbon can improve the catalytic ability of Pt catalyst for methanol electro-oxidation and antipoison capability for CO. The composite electrode modified by 0.23 g nitric acid has the highest electrochemical ability.

scholarly journals Synthesis of Hollow Mesoporous TiN Nanostructures as an Efficient Catalyst Support for Methanol Electro-Oxidation

Catalysts ◽  
2021 ◽  
Vol 11 (7) ◽  
pp. 763
Author(s):  
Yoon-Hee Kim ◽  
Hyeonkyeong Lee ◽  
Dong-Seop Choi ◽  
Jiyull Kim ◽  
Hyun-Sung Jang ◽  
...  
Keyword(s):  
Sol Gel ◽  
Catalyst Support ◽  
Physicochemical Characteristics ◽  
Catalytic Performance ◽  
Pt Catalyst ◽  
Pt Catalysts ◽  
Efficient Catalyst ◽  
Electro Oxidation ◽  
Sol Gel Synthesis ◽  
Nitridation Temperature

The development of efficient catalyst materials that can drive high catalytic performance is challenging. Here, we report a well-defined hollow mesoporous TiN nanostructure for use as Pt catalyst support material for methanol electro-oxidation. The hollow TiN nanostructure was synthesized by the ammonia nitridation of pre-synthesized mother hollow anatase TiO2, which was prepared by SiO2 template-assisted sol–gel synthesis followed by chemical etching, acid treatment, and sequential calcination. The variation in the ammonia nitridation temperature allowed the crystalline properties of the samples to be finely tuned. As the ammonia nitrification temperature increased, the crystallinity of the resulting hollow TiN continuously increased, and the corresponding Pt catalysts showed enhanced activity toward methanol electro-oxidation. The hollow TiN-800 sample (H-TiN-800), with a well-developed pure TiN phase, exhibited the highest electrical conductivity and the lowest resistance. The corresponding Pt/H-TiN-800 catalyst exhibited significantly enhanced catalytic activity. In this study, we systemically analyzed the physicochemical characteristics and electrochemical performance of hollow TiN samples and their corresponding Pt catalysts.

The electro-oxidation of dimethyl ether on platinum-based catalyst

2008 ◽  
Vol 53 (28) ◽  
pp. 8298-8304 ◽  
Author(s):  
Qian Zhang ◽  
Zhongfang Li ◽  
Suwen Wang ◽  
Wei Xing ◽  
Rujun Yu ◽  
...  
Keyword(s):  
Dimethyl Ether ◽  
Electro Oxidation

Electro-catalysis of carbon black or titanium sub-oxide supported Pd–Gd towards formic acid electro-oxidation

RSC Advances ◽  
2016 ◽  
Vol 6 (73) ◽  
pp. 68989-68996 ◽  
Author(s):  
Nan He ◽  
Chuanguang Qin ◽  
Rumin Wang ◽  
Shuhui Ma ◽  
Yi Wang ◽  
...  
Keyword(s):  
Aqueous Solution ◽  
Carbon Black ◽  
Formic Acid ◽  
Sodium Borohydride ◽  
Weight Percent ◽  
Reduction Reaction ◽  
Simultaneous Reduction ◽  
Electro Catalysis ◽  
Electro Oxidation ◽  
Supported Pd

Carbon black supported Pd–Gd catalysts (Pd–xGd/C, x is weight percent in catalyst) with different amounts of Gd were prepared by a simultaneous reduction reaction with sodium borohydride in aqueous solution.

Electrochemical and ATR-FTIR study of dimethyl ether and methanol electro-oxidation on sputtered Pt electrode

2007 ◽  
Vol 52 (19) ◽  
pp. 5781-5788 ◽  
Author(s):  
Yan Liu ◽  
Masashi Muraoka ◽  
Shigenori Mitsushima ◽  
Ken-Ichiro Ota ◽  
Nobuyuki Kamiya
Keyword(s):  
Dimethyl Ether ◽  
Pt Electrode ◽  
Ftir Study ◽  
Electro Oxidation
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