Ultrafast spin dynamics in double-magnetic-center endohedral fullerene Y2C2@C82-C2(1)

In the previous chapters we described the basic principles of density functional theory, gave examples of how accurate it is to describe static magnetic properties in general, and derived from this basis the master equation for atomistic spin-dynamics; the SLL (or SLLG) equation. However, one term was not described in these chapters, namely the damping parameter. This parameter is a crucial one in the SLL (or SLLG) equation, since it allows for energy and angular momentum to dissipate from the simulation cell. The damping parameter can be evaluated from density functional theory, and the Kohn-Sham equation, and it is possible to determine its value experimentally. This chapter covers in detail the theoretical aspects of how to calculate theoretically the damping parameter. Chapter 8 is focused, among other things, on the experimental detection of the damping, using ferromagnetic resonance.

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Strong Coupling of Electron and Nuclear Spins: Outlook and Prospects

10.1093/oso/9780198807308.003.0011 ◽

2018 ◽

Author(s):

M. M. Glazov

Keyword(s):

Energy Spectrum ◽

Charge Carrier ◽

Strong Coupling ◽

Nuclear Spin ◽

Spin Dynamics ◽

Spin Polaron ◽

Nuclear Spins ◽

Deep Impurity ◽

Impurity Centers ◽

Ordered State

In this chapter, some prospects in the field of electron and nuclear spin dynamics are outlined. Particular emphasis is put ona situation where the hyperfine interaction is so strong that it leads to a qualitative rearrangement of the energy spectrum resulting in the coherent excitation transfer between the electron and nucleus. The strong coupling between the spin of the charge carrier and of the nucleus is realized, for example in the case of deep impurity centers in semiconductors or in isotopically purified systems. We also discuss the effect of the nuclear spin polaron, that is ordered state, formation at low enough temperatures of nuclear spins, where the orientation of the carrier spin results in alignment of the spins of nucleus interacting with the electron or hole.

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Electron Spin Decoherence by Nuclei

10.1093/oso/9780198807308.003.0007 ◽

2018 ◽

Author(s):

M. M. Glazov

Keyword(s):

Electron Spin ◽

Spin Dynamics ◽

Magnetic Moments ◽

Host Lattice ◽

Spin Model ◽

Relaxation Processes ◽

Nuclear Spins ◽

Model Calculations ◽

Spin Decoherence ◽

Quantum Mechanical Approach

The discussion of the electron spin decoherence and relaxation phenomena via the hyperfine interaction with host lattice spins is presented here. The spin relaxation processes processes limit the conservation time of spin states as well as the response time of the spin system to external perturbations. The central spin model, where the spin of charge carrier interacts with the bath of nuclear spins, is formulated. We also present different methods to calculate the spin dynamics within this model. Simple but physically transparent semiclassical treatment where the nuclear spins are considered as largely static classical magnetic moments is followed by more advanced quantum mechanical approach where the feedback of electron spin dynamics on the nuclei is taken into account. The chapter concludes with an overview of experimental data and its comparison with model calculations.

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Beta-NMR and Basic Processes in Spin Dynamics

Applied Magnetic Resonance ◽

10.1007/s00723-021-01334-1 ◽

2021 ◽

Author(s):

F. S. Dzheparov ◽

A. D. Gulko ◽

D. V. Lvov

Keyword(s):

Spin Dynamics

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Collective spin dynamics under dissipative spin Hall torque

Applied Physics Letters ◽

10.1063/5.0035586 ◽

2021 ◽

Vol 118 (3) ◽

pp. 032406

Author(s):

Yaroslav Tserkovnyak ◽

Eran Maniv ◽

James G. Analytis

Keyword(s):

Spin Dynamics

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Evolution of spin excitations from bulk to monolayer FeSe

Nature Communications ◽

10.1038/s41467-021-23317-3 ◽

2021 ◽

Vol 12 (1) ◽

Author(s):

Jonathan Pelliciari ◽

Seher Karakuzu ◽

Qi Song ◽

Riccardo Arpaia ◽

Abhishek Nag ◽

...

Keyword(s):

Quantum Monte Carlo ◽

Spin Dynamics ◽

Spin Fluctuations ◽

Superconducting Transition ◽

Pairing Mechanism ◽

Range Magnetic Order ◽

X Ray Scattering ◽

Spin Excitations ◽

Order Of Magnitude ◽

Long Range Magnetic Order

AbstractIn ultrathin films of FeSe grown on SrTiO3 (FeSe/STO), the superconducting transition temperature Tc is increased by almost an order of magnitude, raising questions on the pairing mechanism. As in other superconductors, antiferromagnetic spin fluctuations have been proposed to mediate SC making it essential to study the evolution of the spin dynamics of FeSe from the bulk to the ultrathin limit. Here, we investigate the spin excitations in bulk and monolayer FeSe/STO using resonant inelastic x-ray scattering (RIXS) and quantum Monte Carlo (QMC) calculations. Despite the absence of long-range magnetic order, bulk FeSe displays dispersive magnetic excitations reminiscent of other Fe-pnictides. Conversely, the spin excitations in FeSe/STO are gapped, dispersionless, and significantly hardened relative to its bulk counterpart. By comparing our RIXS results with simulations of a bilayer Hubbard model, we connect the evolution of the spin excitations to the Fermiology of the two systems revealing a remarkable reconfiguration of spin excitations in FeSe/STO, essential to understand the role of spin fluctuations in the pairing mechanism.

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