scholarly journals Determination of tropospheric NO2 by airborne multi axis differential optical absorption spectroscopy

2012 ◽  
Vol 61 (2) ◽  
pp. 024204
Author(s):  
Xu Jin ◽  
Xie Pin-Hua ◽  
Si Fu-Qi ◽  
Li Ang ◽  
Liu Wen-Qing
2006 ◽  
Vol 6 (5) ◽  
pp. 9273-9296
Author(s):  
A. Ladstätter-Weißenmayer ◽  
H. Altmeyer ◽  
M. Bruns ◽  
A. Richter ◽  
A. Rozanov ◽  
...  

Abstract. The INDian Ocean EXperiment (INDOEX) was an international, multi-platform field campaign to measure long-range transport of air masses from South and South-East-(SE) Asia towards the Indian Ocean. During the dry monsoon season between January and March 1999, local measurements were carried out from ground based platforms and were compared with satellite based data. The objective of this study was to characterise stratospheric and tropospheric trace gas amounts in the equatorial region, and to investigate the impact of air pollution at this remote site. For the characterisation of the chemical composition of the outflow from the S-SE-Asian region, we performed ground based dual-axis-DOAS (Differential Optical Absorption Spectroscopy) measurements at the KCO (Kaashidhoo Climate Observatory) in the Maldives (5.0° N, 73.5° E). The ground based dual-axis-DOAS measurements were conducted using two different observation modes (off-axis and zenith-sky). This technique allows the separation of the tropospheric and stratospheric columns for different trace gases like O3 and NO2. These dual-axis DOAS data were compared with O3-sonde measurements performed at KCO and satellite based GOME (Global Ozone Measuring Experiment) data during the intensive measuring phase of the INDOEX campaign in February and March 1999. From GOME observations, tropospheric and stratospheric columns for O3 and NO2 were retrieved. In addition, the analysis of the O3-sonde measurements allowed the determination of the tropospheric O3 amount. The comparison shows that the results of all three measurement systems agree within their error limits. During the INDOEX campaign, background conditions were observed most of the time, but in a single case an increase of tropospheric NO2 during a short pollution event was observed and the impact on the vertical columns was calculated. In the GOME measurements, evidence was found for large tropospheric contributions to the BrO budget, probably located in the free troposphere and present throughout the year. The latter has been investigated by the comparison of satellite pixels influenced by high and low cloud conditions based on GOME data which allows the determination of the detection limit of tropospheric BrO columns.


2009 ◽  
Vol 29 (9) ◽  
pp. 2458-2462
Author(s):  
司福祺 Si Fuqi ◽  
谢品华 Xie Pinhua ◽  
刘宇 Liu Yu ◽  
窦科 Dou Ke ◽  
徐晋 Xu Jin ◽  
...  

2019 ◽  
Vol 9 (4) ◽  
pp. 9
Author(s):  
Marilia Mitidieri Fernandes de Oliveira ◽  
Nelson Francisco Favilla Ebecken ◽  
Jorge Luiz Fernandes de Oliveira ◽  
José Maria de Castro Jr

Spectroscopic methods have played an important role in the study of chemical and physical processes related to the composition of the atmosphere and the differential optical absorption spectroscopy (DOAS) has been one of the most powerful methods to measure a wide range of trace gases. The pollutants are identified by their respective ranges of wavelengths that must be previously known. A Passive Differential Optical Absorption Spectroscopy system that uses the ultraviolet region from 400 to 480 nm of the solar radiation is presented. In this research diurnal variation of NO2 was remotely measured by means of MAX-DOAS system which uses multiple viewing angles to monitor pollutant concentrations in urban area at the city of Rio de Janeiro. The instrument was placed on the roof of a building oriented to the center of the city. Tropospheric NO2 amounts are retrieved from the measured spectra using the DOAS technique. In this paper we give a general description of the procedure and present the results from measurements during four days in winter 2017 associated with the prevailing meteorological aspects. These days were characterized by mostly sunny and dry conditions, no convection, periods of medium clouds and clear sky. The tropospheric NO2 slant column densities values are presented and the results are consistent for all three used elevation angles (5º, 10º, and 15º). The results demonstrate the capability and the potential of the MAX-DOAS technique to derive information on spatial distribution of NO2 in an urban environment.


2021 ◽  
Vol 13 (11) ◽  
pp. 2098
Author(s):  
Yuanyuan Qian ◽  
Yuhan Luo ◽  
Fuqi Si ◽  
Haijin Zhou ◽  
Taiping Yang ◽  
...  

Global measurements of total ozone are necessary to evaluate ozone hole recovery above Antarctica. The Environmental Trace Gases Monitoring Instrument (EMI) onboard GaoFen 5, launched in May 2018, was developed to measure and monitor the global total ozone column (TOC) and distributions of other trace gases. In this study, some of the first global TOC results of the EMI using the differential optical absorption spectroscopy (DOAS) method and validation with ground-based TOC measurements and data derived from Ozone Monitoring Instrument (OMI) and TROPOspheric Monitoring Instrument (TROPOMI) observations are presented. Results show that monthly average EMI TOC data had a similar spatial distribution and a high correlation coefficient (R ≥ 0.99) with both OMI and TROPOMI TOC. Comparisons with ground-based measurements from the World Ozone and Ultraviolet Radiation Data Centre also revealed strong correlations (R > 0.9). Continuous zenith sky measurements from zenith scattered light differential optical absorption spectroscopy instruments in Antarctica were also used for validation (R = 0.9). The EMI-derived observations were able to account for the rapid change in TOC associated with the sudden stratospheric warming event in October 2019; monthly average TOC in October 2019 was 45% higher compared to October 2018. These results indicate that EMI TOC derived using the DOAS method is reliable and has the potential to be used for global TOC monitoring.


2007 ◽  
Vol 7 (1) ◽  
pp. 69-79 ◽  
Author(s):  
T. Wagner ◽  
S. Beirle ◽  
T. Deutschmann ◽  
M. Grzegorski ◽  
U. Platt

Abstract. A new method for the satellite remote sensing of different types of vegetation and ocean colour is presented. In contrast to existing algorithms relying on the strong change of the reflectivity in the red and near infrared spectral region, our method analyses weak narrow-band (few nm) reflectance structures (i.e. "fingerprint" structures) of vegetation in the red spectral range. It is based on differential optical absorption spectroscopy (DOAS), which is usually applied for the analysis of atmospheric trace gas absorptions. Since the spectra of atmospheric absorption and vegetation reflectance are simultaneously included in the analysis, the effects of atmospheric absorptions are automatically corrected (in contrast to other algorithms). The inclusion of the vegetation spectra also significantly improves the results of the trace gas retrieval. The global maps of the results illustrate the seasonal cycles of different vegetation types. In addition to the vegetation distribution on land, they also show patterns of biological activity in the oceans. Our results indicate that improved sets of vegetation spectra might lead to more accurate and more specific identification of vegetation type in the future.


Sign in / Sign up

Export Citation Format

Share Document