scholarly journals Assessing Carbon Dioxide Removal Through Global and Regional Ocean Alkalization under High and Low Emission Pathways

Author(s):  
Andrew Lenton ◽  
Richard J. Matear ◽  
David P. Keller ◽  
Vivian Scott ◽  
Naomi E. Vaughan

Abstract. Atmospheric CO2 levels continue to rise, increasing the risk of severe impacts on the Earth system, and on the ecosystem services that it provides. Artificial Ocean Alkalization (AOA) is capable of reducing atmospheric CO2 concentrations, surface warming and addressing ocean acidification. Here we simulate global and regional responses to alkalinity addition (0.25 PmolAlk/year) using the CSIRO-Mk3L-COAL Earth System Model in the period 2020–2100, under high (RCP8.5) and low (RCP2.6) emissions. While regionally there are large changes associated with locations of AOA, globally we see only a very weak dependence on where and when AOA is applied. We see that under RCP2.6, while the carbon uptake associated with AOA is only ~ 60 % of the total under RCP8.5, the relative changes in temperature are larger, as are the changes in pH (1.4×) and aragonite saturation (1.7×). The results of this modelling study are significant as they demonstrate that AOA is more effective under lower emissions, and the higher the emissions the more AOA required to achieve the same reduction in global warming and ocean acidification. Finally, our simulations show AOA in the period 2020–2100 is capable of offsetting global warming and ameliorating ocean acidification increases due to low emissions, but regionally the response is more variable.

2009 ◽  
Vol 22 (22) ◽  
pp. 6066-6088 ◽  
Author(s):  
V. K. Arora ◽  
G. J. Boer ◽  
J. R. Christian ◽  
C. L. Curry ◽  
K. L. Denman ◽  
...  

Abstract The simulation of atmospheric–land–ocean CO2 exchange for the 1850–2000 period offers the possibility of testing and calibrating the carbon budget in earth system models by comparing the simulated changes in atmospheric CO2 concentration and in land and ocean uptake with observation-based information. In particular, some of the uncertainties associated with the treatment of land use change (LUC) and the role of down regulation in affecting the strength of CO2 fertilization for terrestrial photosynthesis are assessed using the Canadian Centre for Climate Modelling and Analysis Earth System Model (CanESM1). LUC emissions may be specified as an external source of CO2 or calculated interactively based on estimated changes in crop area. The evidence for photosynthetic down regulation is reviewed and an empirically based representation is implemented and tested in the model. Four fully coupled simulations are performed: with and without terrestrial photosynthesis down regulation and with interactively determined or specified LUC emissions. Simulations without terrestrial photosynthesis down regulation yield 15–20 ppm lower atmospheric CO2 by the end of the twentieth century, compared to observations, regardless of the LUC approach used because of higher carbon uptake by land. Implementation of down regulation brings simulated values of atmospheric CO2 and land and ocean carbon uptake closer to observation-based values. The use of specified LUC emissions yields a large source in the tropics during the 1981–2000 period, which is inconsistent with studies suggesting the tropics to be near-neutral or small carbon sinks. The annual cycle of simulated global averaged CO2, dominated by the Northern Hemisphere terrestrial photosynthesis and respiration cycles, is reasonably well reproduced, as is the latitudinal distribution of CO2 and the dependence of interhemispheric CO2 gradient on fossil fuel emissions. The empirical approach used here offers a reasonable method of implementing down regulation in coupled carbon–climate models in the absence of a more explicit biogeochemical representation.


2014 ◽  
Vol 11 (10) ◽  
pp. 14551-14585 ◽  
Author(s):  
P. R. Halloran ◽  
B. B. B. Booth ◽  
C. D. Jones ◽  
F. H. Lambert ◽  
D. J. McNeall ◽  
...  

Abstract. The oceans currently take up around a quarter of the carbon dioxide (CO2) emitted by human activity. While stored in the ocean, this CO2 is not influencing Earth's radiation budget; the ocean CO2 sink therefore plays an important role in mitigating global warming. CO2 uptake by the oceans is heterogeneous, with the subpolar North Atlantic being the strongest CO2 sink region. Observations over the last two decades have indicated that CO2 uptake by the subpolar North Atlantic sink can vary rapidly. Given the importance of this sink and its apparent variability, it is critical that we understand the mechanisms behind its operation. Here we explore subpolar North Atlantic CO2 uptake across a large ensemble of Earth System Model simulations, and find that models show a peak in sink strength around the middle of the century after which CO2 uptake begins to decline. We identify different drivers of change on interannual and multidecadal timescales. Short-term variability appears to be driven by fluctuations in regional seawater temperature and alkalinity, whereas the longer-term evolution throughout the coming century is largely occurring through a counterintuitive response to rising atmospheric CO2 concentrations. At high atmospheric CO2 concentrations the contrasting Ravelle factors between the subtropical and subpolar gyres, combined with the transport of surface waters from the subtropical to subpolar gyre, means that the subpolar CO2 uptake capacity is largely satisfied from its southern boundary rather than through air–sea CO2 flux. Our findings indicate that: (i) we can explain the mechanisms of subpolar North Atlantic CO2 uptake variability across a broad range of Earth System Models, (ii) a focus on understanding the mechanisms behind contemporary variability may not directly tell us about how the sink will change in the future, (iii) to identify long-term change in the North Atlantic CO2 sink we should focus observational resources on monitoring subtropical as well as the subpolar seawater CO2, (iv) recent observations of a weakening subpolar North Atlantic CO2 sink suggests that the sink strength is already in long-term decline.


2017 ◽  
Vol 14 (15) ◽  
pp. 3633-3648 ◽  
Author(s):  
Jörg Schwinger ◽  
Jerry Tjiputra ◽  
Nadine Goris ◽  
Katharina D. Six ◽  
Alf Kirkevåg ◽  
...  

Abstract. We estimate the additional transient surface warming ΔTs caused by a potential reduction of marine dimethyl sulfide (DMS) production due to ocean acidification under the high-emission scenario RCP8.5 until the year 2200. Since we use a fully coupled Earth system model, our results include a range of feedbacks, such as the response of marine DMS production to the additional changes in temperature and sea ice cover. Our results are broadly consistent with the findings of a previous study that employed an offline model set-up. Assuming a medium (strong) sensitivity of DMS production to pH, we find an additional transient global warming of 0.30 K (0.47 K) towards the end of the 22nd century when DMS emissions are reduced by 7.3 Tg S yr−1 or 31 % (11.5 Tg S yr−1 or 48 %). The main mechanism behind the additional warming is a reduction of cloud albedo, but a change in shortwave radiative fluxes under clear-sky conditions due to reduced sulfate aerosol load also contributes significantly. We find an approximately linear relationship between reduction of DMS emissions and changes in top of the atmosphere radiative fluxes as well as changes in surface temperature for the range of DMS emissions considered here. For example, global average Ts changes by −0. 041 K per 1 Tg S yr−1 change in sea–air DMS fluxes. The additional warming in our model has a pronounced asymmetry between northern and southern high latitudes. It is largest over the Antarctic continent, where the additional temperature increase of 0.56 K (0.89 K) is almost twice the global average. We find that feedbacks are small on the global scale due to opposing regional contributions. The most pronounced feedback is found for the Southern Ocean, where we estimate that the additional climate change enhances sea–air DMS fluxes by about 9 % (15 %), which counteracts the reduction due to ocean acidification.


2018 ◽  
Vol 9 (2) ◽  
pp. 339-357 ◽  
Author(s):  
Andrew Lenton ◽  
Richard J. Matear ◽  
David P. Keller ◽  
Vivian Scott ◽  
Naomi E. Vaughan

Abstract. Atmospheric carbon dioxide (CO2) levels continue to rise, increasing the risk of severe impacts on the Earth system, and on the ecosystem services that it provides. Artificial ocean alkalinization (AOA) is capable of reducing atmospheric CO2 concentrations and surface warming and addressing ocean acidification. Here, we simulate global and regional responses to alkalinity (ALK) addition (0.25 PmolALK yr−1) over the period 2020–2100 using the CSIRO-Mk3L-COAL Earth System Model, under high (Representative Concentration Pathway 8.5; RCP8.5) and low (RCP2.6) emissions. While regionally there are large changes in alkalinity associated with locations of AOA, globally we see only a very weak dependence on where and when AOA is applied. On a global scale, while we see that under RCP2.6 the carbon uptake associated with AOA is only ∼ 60 % of the total, under RCP8.5 the relative changes in temperature are larger, as are the changes in pH (140 %) and aragonite saturation state (170 %). The simulations reveal AOA is more effective under lower emissions, therefore the higher the emissions the more AOA is required to achieve the same reduction in global warming and ocean acidification. Finally, our simulated AOA for 2020–2100 in the RCP2.6 scenario is capable of offsetting warming and ameliorating ocean acidification increases at the global scale, but with highly variable regional responses.


2017 ◽  
Author(s):  
Jörg Schwinger ◽  
Jerry Tjiputra ◽  
Nadine Goris ◽  
Katharina Six ◽  
Alf Kirkevåg ◽  
...  

Abstract. We estimate the additional transient surface warming ΔTs caused by a potential reduction of marine dimethyl sulfide (DMS) production due to ocean-acidification under the high emission scenario RCP8.5 until the year 2200. Since we use a fully coupled Earth system model, our results include a range of feedbacks, such as the response of marine DMS-production to the additional changes in temperature and sea-ice cover. Our results are broadly consistent with the findings of a previous study that employed an off-line model set-up. Assuming a medium (strong) sensitivity of DMS-production to pH, we find an additional transient global warming of 0.30 K (0.47 K) towards the end of the 22nd century when DMS-emission are reduced by 7.3 Tg S yr−1 or 31 % (11.5 Tg S yr−1 or 48 %). The main mechanism behind the additional warming is a reduction of cloud albedo, but a change in short-wave radiative fluxes under clear-sky conditions due to reduced sulfate aerosol load also contributes significantly. We find an approximately linear relationship between reduction of DMS-emissions and changes in top of the atmosphere radiative fluxes as well as changes in surface temperature for the range of DMS-emissions considered here. For example, global average Ts changes by −0.041 K per 1 Tg S yr−1 change in sea-air DMS-fluxes. The additional warming in our model has a pronounced asymmetry between northern and southern high latitudes. It is largest over the Antarctic continent, where the additional temperature increase of 0.56 K (0.89 K) is almost twice the global average. We find that feedbacks are small on the global scale due to opposing regional contributions. The most pronounced feedback is found for the Southern Ocean, where we estimate that the additional climate change enhances sea-air DMS-fluxes by about 9 % (15 %), which counteracts the reduction due to ocean acidification.


2014 ◽  
Vol 5 (2) ◽  
pp. 991-1012 ◽  
Author(s):  
P. Shao ◽  
X. Zeng ◽  
X. Zeng

Abstract. The influence of prognostic and prescribed atmospheric CO2 concentrations ([CO2]) on the carbon uptake and temperature is investigated using all eight Earth System Models (ESMs) with relevant output variables from the Coupled Model Intercomparison Project Phase 5 (CMIP5). Under the RCP8.5 scenario, the projected [CO2] differences in 2100 vary from −19.7 to +207.3 ppm in emission-driven ESMs. Incorporation of the interactive concentrations also increases the range of global warming, computed as the 20 year average difference between 2081–2100 and 1850–1869/1861–1880, by 49% from 2.36 K (i.e. ranging from 3.11 to 5.47 K) in the concentration-driven simulations to 3.51 K in the emission-driven simulations. The observed seasonal amplitude of global [CO2] from 1980–2011 is about 1.2–5.3 times as large as those from the eight emission-driven ESMs, while the [CO2] seasonality is simply neglected in concentration-driven ESMs, suggesting the urgent need of ESM improvements in this area. The temperature-concentration feedback parameter α is more sensitive to [CO2] (e.g. during 1980–2005 versus 2075–2100) than how [CO2] is handled (i.e. prognostic versus prescribed). This sensitivity can be substantially reduced by using a more appropriate parameter α' computed from the linear regression of temperature change versus that of the logarithm of [CO2]. However, the inter-model relative variations of both α and α' remain large, suggesting the need of more detailed studies to understand and hopefully reduce these discrepancies.


2016 ◽  
Vol 7 (4) ◽  
pp. 783-796 ◽  
Author(s):  
Vera Heck ◽  
Jonathan F. Donges ◽  
Wolfgang Lucht

Abstract. The planetary boundaries framework provides guidelines for defining thresholds in environmental variables. Their transgression is likely to result in a shift in Earth system functioning away from the relatively stable Holocene state. As the climate system is approaching critical thresholds of atmospheric carbon, several climate engineering methods are discussed, aiming at a reduction of atmospheric carbon concentrations to control the Earth's energy balance. Terrestrial carbon dioxide removal (tCDR) via afforestation or bioenergy production with carbon capture and storage are part of most climate change mitigation scenarios that limit global warming to less than 2 °C. We analyse the co-evolutionary interaction of societal interventions via tCDR and the natural dynamics of the Earth's carbon cycle. Applying a conceptual modelling framework, we analyse how the degree of anticipation of the climate problem and the intensity of tCDR efforts with the aim of staying within a "safe" level of global warming might influence the state of the Earth system with respect to other carbon-related planetary boundaries. Within the scope of our approach, we show that societal management of atmospheric carbon via tCDR can lead to a collateral transgression of the planetary boundary of land system change. Our analysis indicates that the opportunities to remain in a desirable region within carbon-related planetary boundaries only exist for a small range of anticipation levels and depend critically on the underlying emission pathway. While tCDR has the potential to ensure the Earth system's persistence within a carbon-safe operating space under low-emission pathways, it is unlikely to succeed in a business-as-usual scenario.


2017 ◽  
Vol 30 (23) ◽  
pp. 9343-9363 ◽  
Author(s):  
Richard G. Williams ◽  
Vassil Roussenov ◽  
Philip Goodwin ◽  
Laure Resplandy ◽  
Laurent Bopp

Climate projections reveal global-mean surface warming increasing nearly linearly with cumulative carbon emissions. The sensitivity of surface warming to carbon emissions is interpreted in terms of a product of three terms: the dependence of surface warming on radiative forcing, the fractional radiative forcing from CO2, and the dependence of radiative forcing from CO2 on carbon emissions. Mechanistically each term varies, respectively, with climate sensitivity and ocean heat uptake, radiative forcing contributions, and ocean and terrestrial carbon uptake. The sensitivity of surface warming to fossil-fuel carbon emissions is examined using an ensemble of Earth system models, forced either by an annual increase in atmospheric CO2 or by RCPs until year 2100. The sensitivity of surface warming to carbon emissions is controlled by a temporal decrease in the dependence of radiative forcing from CO2 on carbon emissions, which is partly offset by a temporal increase in the dependence of surface warming on radiative forcing. The decrease in the dependence of radiative forcing from CO2 is due to a decline in the ratio of the global ocean carbon undersaturation to carbon emissions, while the increase in the dependence of surface warming is due to a decline in the ratio of ocean heat uptake to radiative forcing. At the present time, there are large intermodel differences in the sensitivity in surface warming to carbon emissions, which are mainly due to uncertainties in the climate sensitivity and ocean heat uptake. These uncertainties undermine the ability to predict how much carbon may be emitted before reaching a warming target.


2020 ◽  
Vol 13 (7) ◽  
pp. 3383-3438 ◽  
Author(s):  
Veronika Eyring ◽  
Lisa Bock ◽  
Axel Lauer ◽  
Mattia Righi ◽  
Manuel Schlund ◽  
...  

Abstract. The Earth System Model Evaluation Tool (ESMValTool) is a community diagnostics and performance metrics tool designed to improve comprehensive and routine evaluation of Earth system models (ESMs) participating in the Coupled Model Intercomparison Project (CMIP). It has undergone rapid development since the first release in 2016 and is now a well-tested tool that provides end-to-end provenance tracking to ensure reproducibility. It consists of (1) an easy-to-install, well-documented Python package providing the core functionalities (ESMValCore) that performs common preprocessing operations and (2) a diagnostic part that includes tailored diagnostics and performance metrics for specific scientific applications. Here we describe large-scale diagnostics of the second major release of the tool that supports the evaluation of ESMs participating in CMIP Phase 6 (CMIP6). ESMValTool v2.0 includes a large collection of diagnostics and performance metrics for atmospheric, oceanic, and terrestrial variables for the mean state, trends, and variability. ESMValTool v2.0 also successfully reproduces figures from the evaluation and projections chapters of the Intergovernmental Panel on Climate Change (IPCC) Fifth Assessment Report (AR5) and incorporates updates from targeted analysis packages, such as the NCAR Climate Variability Diagnostics Package for the evaluation of modes of variability, the Thermodynamic Diagnostic Tool (TheDiaTo) to evaluate the energetics of the climate system, as well as parts of AutoAssess that contains a mix of top–down performance metrics. The tool has been fully integrated into the Earth System Grid Federation (ESGF) infrastructure at the Deutsches Klimarechenzentrum (DKRZ) to provide evaluation results from CMIP6 model simulations shortly after the output is published to the CMIP archive. A result browser has been implemented that enables advanced monitoring of the evaluation results by a broad user community at much faster timescales than what was possible in CMIP5.


2021 ◽  
Author(s):  
Ralf Döscher ◽  
Mario Acosta ◽  
Andrea Alessandri ◽  
Peter Anthoni ◽  
Almut Arneth ◽  
...  

Abstract. The Earth System Model EC-Earth3 for contributions to CMIP6 is documented here, with its flexible coupling framework, major model configurations, a methodology for ensuring the simulations are comparable across different HPC systems, and with the physical performance of base configurations over the historical period. The variety of possible configurations and sub-models reflects the broad interests in the EC-Earth community. EC-Earth3 key performance metrics demonstrate physical behaviour and biases well within the frame known from recent CMIP models. With improved physical and dynamic features, new ESM components, community tools, and largely improved physical performance compared to the CMIP5 version, EC-Earth3 represents a clear step forward for the only European community ESM. We demonstrate here that EC-Earth3 is suited for a range of tasks in CMIP6 and beyond.


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