Evaluation of the impact of wood combustion on benzo(a)pyrene concentrations, using ambient air measurements and dispersion modelling in Helsinki, Finland
Abstract. Even though emission inventories indicate that wood combustion is a major source of PAHs, estimating its impacts on PAH concentration in ambient air is challenging. In this study effect of local small-scale wood combustion on the benzo(a)pyrene (BaP) concentrations in ambient air in the Helsinki metropolitan area in Finland was evaluated, using ambient air measurements, emission estimates and dispersion modelling. Measurements were conducted at 12 different locations during a period from 2007 to 2015. The spatial distributions of annual average benzo(a)pyrene concentrations originated from wood combustion were predicted for four years: 2008, 2011, 2013 and 2014. According to both the measurements and the dispersion modelling, the European Union target value for the annual average BaP concentrations (1 ng m−3) was clearly exceeded in part of the suburban detached house areas. However, over most of the other urban areas, including the centre of Helsinki, the concentrations were below the target value. The measured BaP concentrations were highly correlated with the measured levoglucosan concentrations at suburban detached house areas. In street canyons, the measured concentrations of BaP were at the same level as urban background, being clearly lower than those in suburban detached house areas. The predicted annual average concentrations agreed fairly well with the measured concentrations. Both measurements and modelling clearly indicated that wood combustion was the main local source of ambient air BaP in the Helsinki metropolitan area.