scholarly journals Impact of the choice of the satellite aerosol optical depth product in a sub-regional dust emission inversion

2017 ◽  
Author(s):  
Jerónimo Escribano ◽  
Olivier Boucher ◽  
Frédéric Chevallier ◽  
Nicolás Huneeus

Abstract. Mineral dust is the major continental contributor to the global atmospheric aerosol burden with important effects on the climate system. Regionally, a large fraction of the emitted dust is produced in North Africa, however the total emission flux from this region is still highly uncertain. In order to reduce these uncertainties, emission estimates through top-down approaches (i.e., usually models constrained by observations) had been successfully developed and implemented. Such studies usually rely on a single observational dataset and propagate the possible observational errors of this dataset onto the emission estimates. In this study, aerosol optical depth (AOD) products from five different satellites are assimilated one by one in a source inversion system to estimate dust emission fluxes over northern Africa and the Arabian Peninsula. We estimate mineral dust emissions for the year 2006 and discuss the impact of the assimilated dataset on the analysis. We find a relatively large dispersion in flux estimates among the five experiments, which can likely be attributed to differences in the assimilated observation datasets and their associated error statistics. We also show how the assimilation of a variety of AOD products can help to identify systematic errors in models.

2017 ◽  
Vol 17 (11) ◽  
pp. 7111-7126 ◽  
Author(s):  
Jerónimo Escribano ◽  
Olivier Boucher ◽  
Frédéric Chevallier ◽  
Nicolás Huneeus

Abstract. Mineral dust is the major continental contributor to the global atmospheric aerosol burden with important effects on the climate system. Regionally, a large fraction of the emitted dust is produced in northern Africa; however, the total emission flux from there is still highly uncertain. In order to reduce these uncertainties, emission estimates through top-down approaches (i.e. usually models constrained by observations) have been successfully developed and implemented. Such studies usually rely on a single observational dataset and propagate the possible observational errors of this dataset onto the emission estimates. In this study, aerosol optical depth (AOD) products from five different satellites are assimilated one by one in a source inversion system to estimate dust emission fluxes over northern Africa and the Arabian Peninsula. We estimate mineral dust emissions for the year 2006 and discuss the impact of the assimilated dataset on the analysis. We find a relatively large dispersion in flux estimates among the five experiments, which can likely be attributed to differences in the assimilated observation datasets and their associated error statistics.


2012 ◽  
Vol 12 (1) ◽  
pp. 3075-3130 ◽  
Author(s):  
N. Huneeus ◽  
F. Chevallier ◽  
O. Boucher

Abstract. This study estimates the emission fluxes of a range of aerosol species and aerosol precursor at the global scale. These fluxes are estimated by assimilating daily total and fine mode aerosol optical depth (AOD) at 550 nm from the Moderate Resolution Imaging Spectroradiometer (MODIS) into a global aerosol model of intermediate complexity. Monthly emissions are fitted homogenously for each species over a set of predefined regions. The performance of the assimilation is evaluated by comparing the AOD after assimilation against the MODIS observations and against independent observations. The system is effective in forcing the model towards the observations, for both total and fine mode AOD. Significant improvements for the root mean square error and correlation coefficient against both the assimilated and independent datasets are observed as well as a significant decrease in the mean bias against the assimilated observations. The assimilation is more efficient over land than over ocean. The impact of the assimilation of fine mode AOD over ocean demonstrates potential for further improvement by including fine mode AOD observations over continents. The Angström exponent is also improved in African, European and dusty stations. The estimated emission flux for black carbon is 14.5 Tg yr−1, 119 Tg yr−1 for organic matter, 17 Pg yr−1 for sea salt, 82.7 TgS yr−1 for SO2 and 1383 Tg yr−1 for desert dust. They represent a difference of +45%, +40%, +26%, +13% and −39% respectively, with respect to the a priori values. The initial errors attributed to the emission fluxes are reduced for all estimated species.


2010 ◽  
Vol 10 (3) ◽  
pp. 7553-7599 ◽  
Author(s):  
T. Stanelle ◽  
B. Vogel ◽  
H. Vogel ◽  
D. Bäumer ◽  
Ch. Kottmeier

Abstract. We used the comprehensive model system COSMO-ART to quantify the impact of mineral dust on the radiative fluxes, the temperature and the feedback between dust particles and their emissions. We simulated two dust storms over West Africa in March 2006 and in June 2007. Simulations with and without coupling of the actual dust concentration with the radiative fluxes and the thermodynamics were carried out for each case. The model results for the 2006 case were compared with observations of the AMMA campaign. At the surface the shortwave radiative effect of mineral dust can be described by a linear relation between the changes in net surface radiation and the aerosol optical depth. For an aerosol optical depth (AOD) at 450 nm of 1 the average shortwave radiation reduction amounts −130 W m−2 during noon. The longwave radiative effect of mineral dust is nonlinear, with an average increase of +70 W m−2 for an AOD (450 nm) of 1. At the top of the atmosphere the effect of the dust layer with an AOD of 1 on radiative fluxes is not as significant as at the surface. It is slightly positive for the shortwave and approximately 26 W m−2 for the longwave radiation. The height range and the extension of the dust layer determine the effect of dust particles on the 2 m temperature. When the dust layer is attached to the surface and lasts for several days it leads to an increase of the surface temperature even during daytime. In case of an elevated dust layer there is a decrease in 2 m temperature of up to 4 K during noon. It is shown, that the temperature changes caused by mineral dust may result in horizontal temperature gradients which also modify near surface winds. Since surface wind thresholds decide the uptake of dust from the surface, a feedback on total emission fluxes is established. The coupled model provides an increase in the total emission fluxes of dust particles by about 16% during the dust storm in March 2006 and 25% during the dust episode in June 2007.


2012 ◽  
Vol 12 (10) ◽  
pp. 4585-4606 ◽  
Author(s):  
N. Huneeus ◽  
F. Chevallier ◽  
O. Boucher

Abstract. This study estimates the emission fluxes of a range of aerosol species and one aerosol precursor at the global scale. These fluxes are estimated by assimilating daily total and fine mode aerosol optical depth (AOD) at 550 nm from the Moderate Resolution Imaging Spectroradiometer (MODIS) into a global aerosol model of intermediate complexity. Monthly emissions are fitted homogenously for each species over a set of predefined regions. The performance of the assimilation is evaluated by comparing the AOD after assimilation against the MODIS observations and against independent observations. The system is effective in forcing the model towards the observations, for both total and fine mode AOD. Significant improvements for the root mean square error and correlation coefficient against both the assimilated and independent datasets are observed as well as a significant decrease in the mean bias against the assimilated observations. These improvements are larger over land than over ocean. The impact of the assimilation of fine mode AOD over ocean demonstrates potential for further improvement by including fine mode AOD observations over continents. The Angström exponent is also improved in African, European and dusty stations. The estimated emission flux for black carbon is 15 Tg yr−1, 119 Tg yr−1 for particulate organic matter, 17 Pg yr−1 for sea salt, 83 TgS yr−1 for SO2 and 1383 Tg yr−1 for desert dust. They represent a difference of +45 %, +40 %, +26 %, +13 % and −39 % respectively, with respect to the a priori values. The initial errors attributed to the emission fluxes are reduced for all estimated species.


2020 ◽  
Vol 16 (1) ◽  
pp. 1-14
Author(s):  
Monim Jiboori ◽  
Nadia Abed ◽  
Mohamed Abdel Wahab

2016 ◽  
Vol 9 (1) ◽  
pp. 53-62 ◽  
Author(s):  
R. D. García ◽  
O. E. García ◽  
E. Cuevas ◽  
V. E. Cachorro ◽  
A. Barreto ◽  
...  

Abstract. This paper presents the reconstruction of a 73-year time series of the aerosol optical depth (AOD) at 500 nm at the subtropical high-mountain Izaña Atmospheric Observatory (IZO) located in Tenerife (Canary Islands, Spain). For this purpose, we have combined AOD estimates from artificial neural networks (ANNs) from 1941 to 2001 and AOD measurements directly obtained with a Precision Filter Radiometer (PFR) between 2003 and 2013. The analysis is limited to summer months (July–August–September), when the largest aerosol load is observed at IZO (Saharan mineral dust particles). The ANN AOD time series has been comprehensively validated against coincident AOD measurements performed with a solar spectrometer Mark-I (1984–2009) and AERONET (AErosol RObotic NETwork) CIMEL photometers (2004–2009) at IZO, obtaining a rather good agreement on a daily basis: Pearson coefficient, R, of 0.97 between AERONET and ANN AOD, and 0.93 between Mark-I and ANN AOD estimates. In addition, we have analysed the long-term consistency between ANN AOD time series and long-term meteorological records identifying Saharan mineral dust events at IZO (synoptical observations and local wind records). Both analyses provide consistent results, with correlations  >  85 %. Therefore, we can conclude that the reconstructed AOD time series captures well the AOD variations and dust-laden Saharan air mass outbreaks on short-term and long-term timescales and, thus, it is suitable to be used in climate analysis.


2021 ◽  
Vol 13 (6) ◽  
pp. 1096
Author(s):  
Soi Ahn ◽  
Sung-Rae Chung ◽  
Hyun-Jong Oh ◽  
Chu-Yong Chung

This study aimed to generate a near real time composite of aerosol optical depth (AOD) to improve predictive model ability and provide current conditions of aerosol spatial distribution and transportation across Northeast Asia. AOD, a proxy for aerosol loading, is estimated remotely by various spaceborne imaging sensors capturing visible and infrared spectra. Nevertheless, differences in satellite-based retrieval algorithms, spatiotemporal resolution, sampling, radiometric calibration, and cloud-screening procedures create significant variability among AOD products. Satellite products, however, can be complementary in terms of their accuracy and spatiotemporal comprehensiveness. Thus, composite AOD products were derived for Northeast Asia based on data from four sensors: Advanced Himawari Imager (AHI), Geostationary Ocean Color Imager (GOCI), Moderate Infrared Spectroradiometer (MODIS), and Visible Infrared Imaging Radiometer Suite (VIIRS). Cumulative distribution functions were employed to estimate error statistics using measurements from the Aerosol Robotic Network (AERONET). In order to apply the AERONET point-specific error, coefficients of each satellite were calculated using inverse distance weighting. Finally, the root mean square error (RMSE) for each satellite AOD product was calculated based on the inverse composite weighting (ICW). Hourly AOD composites were generated (00:00–09:00 UTC, 2017) using the regression equation derived from the comparison of the composite AOD error statistics to AERONET measurements, and the results showed that the correlation coefficient and RMSE values of composite were close to those of the low earth orbit satellite products (MODIS and VIIRS). The methodology and the resulting dataset derived here are relevant for the demonstrated successful merging of multi-sensor retrievals to produce long-term satellite-based climate data records.


Author(s):  
Qijiao Xie ◽  
Qi Sun

Aerosols significantly affect environmental conditions, air quality, and public health locally, regionally, and globally. Examining the impact of land use/land cover (LULC) on aerosol optical depth (AOD) helps to understand how human activities influence air quality and develop suitable solutions. The Landsat 8 image and Moderate Resolution Imaging Spectroradiometer (MODIS) aerosol products in summer in 2018 were used in LULC classification and AOD retrieval in this study. Spatial statistics and correlation analysis about the relationship between LULC and AOD were performed to examine the impact of LULC on AOD in summer in Wuhan, China. Results indicate that the AOD distribution expressed an obvious “basin effect” in urban development areas: higher AOD values concentrated in water bodies with lower terrain, which were surrounded by the high buildings or mountains with lower AOD values. The AOD values were negatively correlated with the vegetated areas while positively correlated to water bodies and construction lands. The impact of LULC on AOD varied with different contexts in all cases, showing a “context effect”. The regression correlations among the normalized difference vegetation index (NDVI), normalized difference built-up index (NDBI), normalized difference water index (NDWI), and AOD in given landscape contexts were much stronger than those throughout the whole study area. These findings provide sound evidence for urban planning, land use management and air quality improvement.


2021 ◽  
Author(s):  
Qiaoqiao Wang ◽  
Jianwei Gu ◽  
Xurong Wang

<p>The frequent transport of Sahara dust toward Europe degrades the air quality and poses risk to human health. In this study we use GEOS-Chem (a global transport model) to examine the impact of Sahara dust on air quality and the consequent health effect in Europe for the year 2016–2017. The simualtion is conducted in a nested model with the native resolution of 0.25° × 0.3125° (Latitude × Logitude) over Europe (32.75°N–61.25°N, 15°W–40°E). The simulation on a global scale with a coarse horizontal resolution of 2° × 2.5° is also conducted to provide the boundary condition for the nested-grid simulation as well as aerosol optical depth (AOD) over the Sahara desert for model evaluation.</p><p>The model performance is evaluated by comparisons with surface observations including aerosol optical depth (AOD) from AERONET, and PM<sub>2.5</sub> and PM<sub>10</sub> concentrations from numerous air quality monitoring stations in European countries. Overall, the model well reproduces observed surface PM concentrations over most European countries with some underestimation in southern Europe. In addition, model AOD is highly correlated with AERONET data over both Sahara and European region.</p><p>The spatial distribution of dust concentrations, frequency of dust episodes, as well as the exposure and health effects are studied. The concentrations of Sahara dust decrease from 5–20 μg m<sup>-3</sup> in south to 0.5–1.0 μg m<sup>-3</sup> in north of Europe. Spain and Italy are most heavily influenced by Sahara dust in terms of both concentration levels and frequencies of occurrence. Strong dust episodes (>50 μg m<sup>-3</sup>) occur predominately in Southern Spain and Italy with frequency of 2–5%, while light dust episodes (>1 μg m<sup>-3</sup>) are often detected (5–30%) in Central and Western Europe.</p><p>The population-weighted dust concentrations are higher in Southern European countries (3.3–7.9 μg m<sup>-3</sup>) and lower in Western European countries (0.5–0.6 μg m<sup>-3</sup>). The health effects of exposure to dust is evaluated based on population attributable fraction (PAF). We use the relative risk (RR) value of 1.04 (95% confidence intervals: 1.00 – 1.09) per 10 µg m<sup>-3 </sup>of dust exposure based on the main model of Beelen et al. (2014). We estimate a total of 41884 (95% CI: 2110–81658) deaths per year attributed to the exposure to dust in the 13 European countries studied. Due to high contribution to PM<sub>10</sub> in Spain, Italy and Portugal, dust accounts for 44%, 27% and 22% of the total number of deaths linked to PM<sub>10</sub> exposure, respectively.</p>


2009 ◽  
Vol 66 (4) ◽  
pp. 1033-1040 ◽  
Author(s):  
O. E. García ◽  
A. M. Díaz ◽  
F. J. Expósito ◽  
J. P. Díaz ◽  
A. Redondas ◽  
...  

Abstract The influence of mineral dust on ultraviolet energy transfer is studied for two different mineralogical origins. The aerosol radiative forcing ΔF and the forcing efficiency at the surface ΔFeff in the range 290–325 nm were estimated in ground-based stations affected by the Saharan and Asian deserts during the dusty seasons. UVB solar measurements were taken from the World Ozone and Ultraviolet Data Center (WOUDC) for four Asian stations (2000–04) and from the Santa Cruz Observatory, Canary Islands (2002–03), under Gobi and Sahara Desert influences, respectively. The Moderate Resolution Imaging Spectroradiometer (MODIS) aerosol optical depth at 550 nm was used to characterize the aerosol load τ, whereas the aerosol index provided by the Total Ozone Mapping Spectrometer (TOMS) sensor was employed to identify the mineral dust events. The ΔF is strongly affected by the aerosol load, the values found being comparable in both regions during the dusty seasons. Under those conditions, ΔF values as large as −1.29 ± 0.53 W m−2 (τ550 = 0.48 ± 0.24) and −1.43 ± 0.38 W m−2 (τ550 = 0.54 ± 0.26) were reached under Saharan and Asian dust conditions, respectively. Nevertheless, significant differences have been observed in the aerosol radiative forcing per unit of aerosol optical depth in the slant path, τS. The maximum ΔFeff values associated with dust influences were −1.55 ± 0.20 W m−2 τS550−1 for the Saharan region and −0.95 ± 0.11 W m−2 τS550−1 in the Asian area. These results may be used as a benchmark database for establishing aerosol corrections in UV satellite products or in global climate model estimations.


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