scholarly journals Utilizing Electroplex Emission to Achieve External Quantum Efficiency up to 18.1% in Nondoped Blue OLED

Research ◽  
2020 ◽  
Vol 2020 ◽  
pp. 1-13
Author(s):  
Xuejun Zhan ◽  
Zhongbin Wu ◽  
Yanbin Gong ◽  
Jin Tu ◽  
Yujun Xie ◽  
...  

For the first time, electroplex emission is utilized to enhance the performance of nondoped blue organic light-emitting diodes (OLEDs). By decorating the twisted blue-emitting platform and adjusting the electronic structure, three molecules of 3Cz-Ph-CN, 3Cz-mPh-CN, and 3Ph-Cz-CN with a donor-acceptor structure are synthesized and investigated. When external voltage is applied, electroplex emission, which contributes to the emission performance of OLED, can be realized at the interface between the emitting layer and the electron-transporting layer. Accordingly, high external quantum efficiency of 18.1% can be achieved, while the emission wavelength of the device can be controlled in the blue region. Our results provide the possibility to enhance the performance of OLED through electroplex emission, in addition to the generally investigated thermally activated delayed fluorescence (TADF). Excitedly, when 3Ph-Cz-CN is used as host material in orange-emitting phosphorous OLEDs (PO-01 as the dopant), unprecedented high external quantum efficiency of 27.4% can also be achieved.

2018 ◽  
Vol 6 (20) ◽  
pp. 5363-5368 ◽  
Author(s):  
Ji Han Kim ◽  
Dong Ryun Lee ◽  
Si Hyun Han ◽  
Jun Yeob Lee

Highly efficient red thermally activated delayed fluorescence organic light-emitting diodes were developed using a reverse intersystem crossing activating host derived from phenylcarbazole and pyridofuropyridine.


RSC Advances ◽  
2019 ◽  
Vol 9 (8) ◽  
pp. 4336-4343 ◽  
Author(s):  
Ikbal Marghad ◽  
Fatima Bencheikh ◽  
Chao Wang ◽  
Sophia Manolikakes ◽  
Alice Rérat ◽  
...  

A novel TADF emitter showing dual emission is synthesized and applied to OLEDs with an external quantum efficiency of 11.5%.


2016 ◽  
Vol 4 (43) ◽  
pp. 10205-10208 ◽  
Author(s):  
Xin He ◽  
Tong Shan ◽  
Xiangyang Tang ◽  
Yu Gao ◽  
Jinyu Li ◽  
...  

DPAC–DBTDO possesses a very small ΔEST of 0.10 eV between S1 and T1. A high external quantum efficiency of 13.1% is achieved in multi-layered OLEDs.


2020 ◽  
Vol 8 (5) ◽  
pp. 1736-1745 ◽  
Author(s):  
Kyung Hyung Lee ◽  
Soon Ok Jeon ◽  
Yeon Sook Chung ◽  
Masaki Numata ◽  
Hasup Lee ◽  
...  

A molecular design platform of blue thermally activated delayed fluorescence (TADF) emitters to boost the external quantum efficiency and efficiency roll-off of blue TADF organic light-emitting diodes (OLEDs) was developed.


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