scholarly journals Hydrothermal Synthesis of Graphene Quantum Dots Supported on Three-Dimensional Graphene for Supercapacitors

Nanomaterials ◽  
2019 ◽  
Vol 9 (2) ◽  
pp. 201 ◽  
Author(s):  
Peihui Luo ◽  
Xiangfeng Guan ◽  
Yunlong Yu ◽  
Xiaoyan Li ◽  
Fengpo Yan
Keyword(s):  
Quantum Dots ◽  
Graphene Quantum Dots ◽  
Three Dimensional ◽  
Electrochemical Stability ◽  
Structure And Properties ◽  
Initial Value ◽  
One Step ◽  
Improved Performance ◽  
Functional Components ◽  
Electrodes For Supercapacitors

Incorporation of new functional components into a three-dimensional graphene (3DG) framework improves the performance of supercapacitors based on 3DG as electrodes by tailoring the framework’s structure and properties. In this work, graphene quantum dots (GQDs) were incorporated into 3DG via one-step hydrothermal treatment of GQDs and graphene oxide (GO). By simply adjusting the GQDs/GO feeding ratio by weight, various GQDs/3DG composites were formed. The maximum feeding ratio was 80%, and the prepared composites possessed saturated GQDs loading on the 3DG framework, whereas composites obtained with a GQDs/GO feeding ratio of 40% as electrodes exhibited optimal specific capacitance of 242 F·g−1 for supercapacitors, an increase of 22% compared with that of pure 3DG electrodes (198 F·g−1). This improved performance was mainly due to better electrical conductivity and larger surface area for GQDs/3DG composites with moderate GQDs content. The fabricated GQDs/3DG composites as electrodes for supercapacitors revealed high electrochemical stability. Their capacitance kept 93% of the initial value after 10,000 charge-discharge cycles.

Graphene aerogel-supported and graphene quantum dots-modified γ-MnOOH nanotubes as a highly efficient electrocatalyst for oxygen reduction reaction

RSC Advances ◽  
2016 ◽  
Vol 6 (49) ◽  
pp. 43116-43126 ◽  
Author(s):  
Yisi Liu ◽  
Wenzhang Li ◽  
Jie Li ◽  
Haibo Shen ◽  
Yaomin Li ◽  
...  
Keyword(s):  
Quantum Dots ◽  
Oxygen Reduction Reaction ◽  
Oxygen Reduction ◽  
Graphene Quantum Dots ◽  
Three Dimensional ◽  
Reduction Reaction ◽  
Graphene Aerogel ◽  
3D Graphene ◽  
Highly Efficient

In this work, we demonstrate a facile strategy to synthesize a novel three-dimensional (3D) graphene aerogel-supported and graphene quantum dots-modified γ-MnOOH nanotubes as a highly efficient electrocatalyst.

One step electro-oxidative preparation of graphene quantum dots from wood charcoal as a peroxidase mimetic

Talanta ◽  
2017 ◽  
Vol 173 ◽  
pp. 36-43 ◽  
Author(s):  
Narsingh R. Nirala ◽  
Gaurav Khandelwal ◽  
Brijesh Kumar ◽  
Vinita ◽  
Rajiv Prakash ◽  
...  
Keyword(s):  
Quantum Dots ◽  
Graphene Quantum Dots ◽  
Wood Charcoal ◽  
Peroxidase Mimetic ◽  
One Step

scholarly journals One-Step Synthesis of Diamine-Functionalized Graphene Quantum Dots from Graphene Oxide and Their Chelating and Antioxidant Activities

Nanomaterials ◽  
2020 ◽  
Vol 10 (1) ◽  
pp. 104 ◽  
Author(s):  
Rabeb El-Hnayn ◽  
Laetitia Canabady-Rochelle ◽  
Christophe Desmarets ◽  
Lavinia Balan ◽  
Hervé Rinnert ◽  
...  
Keyword(s):  
Quantum Dots ◽  
Graphene Oxide ◽  
Colloidal Stability ◽  
Antioxidant Activities ◽  
Graphene Quantum Dots ◽  
Average Diameter ◽  
Functionalized Graphene ◽  
One Step ◽  
Low Cytotoxicity ◽  
Health Applications

2,2’-(Ethylenedioxy)bis(ethylamine)-functionalized graphene quantum dots (GQDs) were prepared under mild conditions from graphene oxide (GO) via oxidative fragmentation. The as-prepared GQDs have an average diameter of ca. 4 nm, possess good colloidal stability, and emit strong green-yellow light with a photoluminescence (PL) quantum yield of 22% upon excitation at 375 nm. We also demonstrated that the GQDs exhibit high photostability and the PL intensity is poorly affected while tuning the pH from 1 to 8. Finally, GQDs can be used to chelate Fe(II) and Cu(II) cations, scavenge radicals, and reduce Fe(III) into Fe(II). These chelating and reducing properties that associate to the low cytotoxicity of GQDs show that these nanoparticles are of high interest as antioxidants for health applications.

scholarly journals Graphene hybrid materials? The role of graphene materials in the final structure of hydrogels

Nanoscale ◽  
2019 ◽  
Vol 11 (11) ◽  
pp. 4822-4830 ◽  
Author(s):  
Cristina Martín ◽  
Ana Martín-Pacheco ◽  
Alicia Naranjo ◽  
Alejandro Criado ◽  
Sonia Merino ◽  
...  
Keyword(s):  
Quantum Dots ◽  
Graphene Oxide ◽  
Hybrid Materials ◽  
Graphene Quantum Dots ◽  
Three Dimensional ◽  
Final Structure ◽  
Polymeric Network

Graphene (G), graphene oxide (GO) and graphene quantum dots (GQDs) have been introduced into a three-dimensional polymeric network based on polyacrylamide in order to ascertain the role of each nanomaterial in hydrogels.

Graphene quantum dots–three-dimensional graphene composites for high-performance supercapacitors

2014 ◽  
Vol 16 (36) ◽  
pp. 19307-19313 ◽  
Author(s):  
Qing Chen ◽  
Yue Hu ◽  
Chuangang Hu ◽  
Huhu Cheng ◽  
Zhipan Zhang ◽  
...  
Keyword(s):  
Quantum Dots ◽  
High Performance ◽  
Graphene Quantum Dots ◽  
Three Dimensional ◽  
Term Stability ◽  
Long Term Stability

Graphene quantum dots boost the capacitance of the graphene supercapacitor by more than 90% and with an excellent long-term stability.

Synthesis of N-doped graphene quantum dots by pulsed laser ablation with diethylenetriamine (DETA) and their photoluminescence

2017 ◽  
Vol 19 (33) ◽  
pp. 22395-22400 ◽  
Author(s):  
S. R. M. Santiago ◽  
T. N. Lin ◽  
C. H. Chang ◽  
Y. A. Wong ◽  
C. A. J. Lin ◽  
...  
Keyword(s):  
Quantum Dots ◽  
Laser Ablation ◽  
Graphene Quantum Dots ◽  
Pulsed Laser ◽  
Pulsed Laser Ablation ◽  
Doped Graphene ◽  
One Step

We report a facile, fast, and one-step approach to prepare N-doped graphene quantum dots (GQDs) using pulsed laser ablation with diethylenetriamine (DETA).

scholarly journals One-Step Preparation of Nitrogen-Doped Graphene Quantum Dots With Anodic Electrochemiluminescence for Sensitive Detection of Hydrogen Peroxide and Glucose

2021 ◽  
Vol 9 ◽  
Author(s):  
Zheng Yanyan ◽  
Jing Lin ◽  
Liuhong Xie ◽  
Hongliang Tang ◽  
Kailong Wang ◽  
...  
Keyword(s):  
Hydrogen Peroxide ◽  
Quantum Dots ◽  
Limit Of Detection ◽  
Hydrothermal Process ◽  
Graphene Quantum Dots ◽  
Sensitive Detection ◽  
Uniform Size ◽  
Nitrogen Doped ◽  
Nitrogen Doped Graphene ◽  
One Step

Simple and efficient synthesis of graphene quantum dots (GQDs) with anodic electrochemiluminescence (ECL) remains a great challenge. Herein, we present an anodic ECL-sensing platform based on nitrogen-doped GQDs (N-GQDs), which enables sensitive detection of hydrogen peroxide (H2O2) and glucose. N-GQDs are easily prepared using one-step molecular fusion between carbon precursor and a dopant in an alkaline hydrothermal process. The synthesis is simple, green, and has high production yield. The as-prepared N-GQDs exhibit a single graphene-layered structure, uniform size, and good crystalline. In the presence of H2O2, N-GQDs possess high anodic ECL activity owing to the functional hydrazide groups. With N-GQDs being ECL probes, sensitive detection of H2O2 in the range of 0.3–100.0 μM with a limit of detection or LOD of 63 nM is achieved. As the oxidation of glucose catalyzed by glucose oxidase (GOx) produces H2O2, sensitive detection of glucose is also realized in the range of 0.7–90.0 μM (LOD of 96 nM).

scholarly journals One-step synthesis of sulfur-incorporated graphene quantum dots using pulsed laser ablation for enhancing optical properties

2020 ◽  
Vol 28 (15) ◽  
pp. 21659 ◽  
Author(s):  
Sukhyun Kang ◽  
Young Kyu Jeong ◽  
Kyung Hwan Jung ◽  
Yong Son ◽  
Won Rae Kim ◽  
...  
Keyword(s):  
Quantum Dots ◽  
Optical Properties ◽  
Laser Ablation ◽  
Graphene Quantum Dots ◽  
Pulsed Laser ◽  
Pulsed Laser Ablation ◽  
One Step

Synthesis of white-light-emitting graphene quantum dots via a one-step reduction and their interfacial characteristics-dependent luminescence properties

2017 ◽  
Vol 4 (4) ◽  
pp. 712-718 ◽  
Author(s):  
Pei Dong ◽  
Bang-Ping Jiang ◽  
Wen-Qian Liang ◽  
Yong Huang ◽  
Zujin Shi ◽  
...  
Keyword(s):  
Quantum Dots ◽  
White Light ◽  
Graphene Quantum Dots ◽  
Luminescence Properties ◽  
Light Emitting ◽  
One Step ◽  
Interfacial Characteristics

Graphene quantum dots (GQDs) have attracted great attention because of their possible applications in various fields.

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