scholarly journals Graphene-Based Nanomaterials as the Cathode for Lithium-Sulfur Batteries

Molecules ◽  
2021 ◽  
Vol 26 (9) ◽  
pp. 2507
Author(s):  
Jingkun Tian ◽  
Fei Xing ◽  
Qiqian Gao

The global energy crisis and environmental problems are becoming increasingly serious. It is now urgent to vigorously develop an efficient energy storage system. Lithium-sulfur batteries (LSBs) are considered to be one of the most promising candidates for next-generation energy storage systems due to their high energy density. Sulfur is abundant on Earth, low-cost, and environmentally friendly, which is consistent with the characteristics of new clean energy. Although LSBs possess numerous advantages, they still suffer from numerous problems such as the dissolution and diffusion of sulfur intermediate products during the discharge process, the expansion of the electrode volume, and so on, which severely limit their further development. Graphene is a two-dimensional crystal material with a single atomic layer thickness and honeycomb bonding structure formed by sp2 hybridization of carbon atoms. Since its discovery in 2004, graphene has attracted worldwide attention due to its excellent physical and chemical properties. Herein, this review summarizes the latest developments in graphene frameworks, heteroatom-modified graphene, and graphene composite frameworks in sulfur cathodes. Moreover, the challenges and future development of graphene-based sulfur cathodes are also discussed.

RSC Advances ◽  
2020 ◽  
Vol 10 (34) ◽  
pp. 20173-20183
Author(s):  
Yasai Wang ◽  
Guilin Feng ◽  
Yang Wang ◽  
Zhenguo Wu ◽  
Yanxiao Chen ◽  
...  

Lithium–sulfur batteries are considered to be promising energy storage devices owing to their high energy density, relatively low price and abundant resources.


2018 ◽  
Vol 6 (17) ◽  
pp. 7375-7381 ◽  
Author(s):  
Zhibin Cheng ◽  
Hui Pan ◽  
Zhubing Xiao ◽  
Dejian Chen ◽  
Xiaoju Li ◽  
...  

A new lithium polysulfide (PS) trapping strategy based on electrostatic attraction between imidazolium groups and PSs has been demonstrated. Simple introduction of main-chain imidazolium-based ionic polymers into sulfur cathodes results in effective suppression of the PS shuttle effect, thus significantly improving cycling stability of lithium–sulfur batteries.


2015 ◽  
Vol 5 (16) ◽  
pp. 1402290 ◽  
Author(s):  
Dongping Lv ◽  
Jianming Zheng ◽  
Qiuyan Li ◽  
Xi Xie ◽  
Seth Ferrara ◽  
...  

2016 ◽  
Vol 52 (73) ◽  
pp. 10964-10967 ◽  
Author(s):  
Long Qie ◽  
Arumugam Manthiram

Long-term cycling stability with high-loading sulfur cathodes has been achieved using N,O-codoped carbon hollow fibers as the current collector and Li2S6 as the starting active material.


Author(s):  
Menghua Yang ◽  
Xuewei Wang ◽  
Jinfeng Wu ◽  
Yue Tian ◽  
Xingyu Huang ◽  
...  

Lithium sulfur (Li-S) batteries has been investigated as the ideal candidates for future high-density energy storage system with the advantages of abundant reserves, high energy density and competitive cost. The...


Author(s):  
Song Huang ◽  
Huixiang Ang ◽  
Yang Yang ◽  
Minghui Ye ◽  
Yufei Zhang ◽  
...  

Owing to promising applications in aircraft, military field and submarine etc., lithium-sulfur (Li-S) batteries with high energy density (2500 Wh·kg-1) are emerging as the next-generation energy storage system at low...


2019 ◽  
Vol 422 ◽  
pp. 104-112 ◽  
Author(s):  
Min-Seop Kim ◽  
Mun Sek Kim ◽  
Vandung Do ◽  
Yongyao Xia ◽  
Woong Kim ◽  
...  

2021 ◽  
Author(s):  
Srikanth Ponnada ◽  
Maryam Sadat Kiai ◽  
Demudu Babu Gorle ◽  
Nowduri Annapurna

One of the most promising alternatives in the energy storage sector is the lithium-sulfur battery, which has a high energy density and theoretical capacity. However, the low electrical conductivity of...


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