scholarly journals Defining Processing Times for Accelerator Produced 225Ac and Other Isotopes from Proton Irradiated Thorium

Molecules ◽  
2019 ◽  
Vol 24 (6) ◽  
pp. 1095 ◽  
Author(s):  
Jonathan Fitzsimmons ◽  
Justin Griswold ◽  
Dmitri Medvedev ◽  
Cathy Cutler ◽  
Leonard Mausner

During the purification of radioisotopes, decay periods or time dependent purification steps may be required to achieve a certain level of radiopurity in the final product. Actinum-225 (Ac-225), Silver-111 (Ag-111), Astatine-211 (At-211), Ruthenium-105 (Ru-105), and Rhodium-105 (Rh-105) are produced in a high energy proton irradiated thorium target. Experimentally measured cross sections, along with MCNP6-generated cross sections, were used to determine the quantities of Ac-225, Ag-111, At-211, Ru-105, Rh-105, and other co-produced radioactive impurities produced in a proton irradiated thorium target at Brookhaven Linac Isotope Producer (BLIP). Ac-225 and Ag-111 can be produced with high radiopurity by the proton irradiation of a thorium target at BLIP.

2021 ◽  
Vol 1024 ◽  
pp. 95-101
Author(s):  
Yosuke Iwamoto ◽  
Makoto Yoshida ◽  
Hiroki Matsuda ◽  
Shin Ichiro Meigo ◽  
Daiki Satoh ◽  
...  

For validating the number of displacements per atom (dpa) for tungsten under high-energy proton irradiation, we measured displacement cross sections related to defect-induced electrical resistivity changes in a tungsten wire sample under irradiation with 389-MeV protons under 10 K. The Gifford–McMahon cryocooler was used to cool the sample using a conductive coolant via thermal conduction plates of oxygen-free high-conductivity copper and electrical insulation sheets of aluminum nitride ceramic. In this experiment, the displacement cross section was 1612 ± 371 b for tungsten at 389 MeV. A comparison of the experimental displacement cross sections of tungsten with the calculated results obtained using Norgett–Robinson–Torrens (NRT) dpa and athermal recombination-corrected (arc) dpa cross sections indicates that arc-dpa was in better agreement with the experimental data than NRT-dpa; this is similar to the displacement cross sections of copper. From the measurements of damage recovery of the accumulated defects in tungsten through isochronal annealing, which is related to the defect concentration of the sample, approximately 20% of the damage was recovered at 60 K. This trend was similar to those observed in other experimental results for reactor neutrons.


2020 ◽  
Vol 1 (6) ◽  
pp. 2068-2073
Author(s):  
Walter O. Herrera Martínez ◽  
Paula Giudici ◽  
Natalia B. Correa Guerrero ◽  
M. Luján Ibarra ◽  
M. Dolores Perez

10 MeV proton irradiation of a MAPbI3 thin film causes PbO formation when the surface is exposed to an O2 atmosphere.


1990 ◽  
Vol 56 (24) ◽  
pp. 2456-2458 ◽  
Author(s):  
E. L. Venturini ◽  
J. C. Barbour ◽  
D. S. Ginley ◽  
R. J. Baughman ◽  
B. Morosin

2018 ◽  
Vol 33 (40) ◽  
pp. 1850242 ◽  
Author(s):  
L. Stodolsky

The description of very high energy proton–proton cross-sections in terms of a “black disc” with an “edge” allows a simple generalization to highest energy proton–nucleus cross-sections. This results in a leading ln2W term and a ln W term whose coefficient depends linearly on the radius of the nucleus (W the c.m. energy). The necessary parameters are determined from the fits to p–p data. Since the coefficient of the ln W term is rather large, it is doubtful that the regime of ln2W dominance can be reached with available energies in accelerators or cosmic rays. However, the ln W term can be relevant for highest energy cosmic rays in the atmosphere, where a large increase for the cross-section on nitrogen is expected. Tests of the theory should be possible by studying the coefficient of ln W at p-nucleus colliders.


2020 ◽  
Vol 1 (1) ◽  
pp. 45-53
Author(s):  
Julie V. Logan ◽  
Elias B. Frantz ◽  
Lilian K. Casias ◽  
Michael P. Short ◽  
Christian P. Morath ◽  
...  

High energy proton irradiation produces long-lived p-type doping in GaN and Ga2O3.


The main features of the C. E. R. N. Intersecting Storage Rings (I. S. R.) are reviewed, together with results obtained in 1971 and 1972 on elastic scattering and total cross-sections. The main result is a 10% increase of the total proton-proton cross-section in the I. S. R. energy range. The simplest picture of high energy proton-proton scattering which emerges from this and the other data, is briefly discussed.


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