scholarly journals Major Impediment to Highly Efficient, Stable and Low-Cost Perovskite Solar Cells

Metals ◽  
2018 ◽  
Vol 8 (11) ◽  
pp. 964 ◽  
Author(s):  
Yue Zhang ◽  
Haiming Zhang ◽  
Xiaohui Zhang ◽  
Lijuan Wei ◽  
Biao Zhang ◽  
...  

Organic–inorganic hybrid perovskite solar cells (PSCs) have made immense progress in recent years, owing to outstanding optoelectronic properties of perovskite materials, such as high extinction coefficient, carrier mobility, and low exciton binding energy. Since the first appearance in 2009, the efficiency of PSCs has reached 23.3%. This has made them the most promising rival to silicon-based solar cells. However, there are still several issues to resolve to promote PSCs’ outdoor applications. In this review, three crucial aspects of PSCs, including high efficiency, environmental stability, and low-cost of PSCs, are described in detail. Recent in-depth studies on different aspects are also discussed for better understanding of these issues and possible solutions.

2017 ◽  
Vol 727 ◽  
pp. 923-928
Author(s):  
Jian Hong Zhao ◽  
Lei Ming Yu ◽  
Tao Yu Zou ◽  
Zhen Fang Qiao ◽  
Li Luo ◽  
...  

Organic-inorganic hybrid perovskite materials offer the potential for realization of low-cost and flexible next-generation solar cells fabricated by low-temperature solution processing. Although efficiencies of perovskite solar cells have dramatically improved up to 22.1% within the past 6 years, there is still considerable room for further improvement in device efficiency through development of smooth and large grain size perovskite films. Commonly, the smooth perovskite layers and large grains are alternative to CH3NH3PbI3-xClx. However, the previous one-step fabrication of CH3NH3PbI3-xClx using PbCl2 needs long annealing time. Herein, the active layer, a noncontinuous CH3NH3PbI3-xClx film with micrometre-level crystalline grain, was fabricated using a one-step spin-coating process followed by high-temperature annealing and exhibited an increased efficiency of 9.93%. This finding enables the formation of larger grain size perovskite films and the demonstration of efficient perovskite heterojunction solar cells.


Author(s):  
Li Zhang ◽  
Hui Li ◽  
Jing Zhuang ◽  
Yigang Luan ◽  
Sixuan Wu ◽  
...  

The low-cost material antimony trifluoride (SbF3) was doped into the commonly used tin dioxide (SnO2) for the first time, and the SbF3-doped SnO2 as an electron transport layer (ETL) was...


2015 ◽  
Vol 2015 ◽  
pp. 1-10 ◽  
Author(s):  
Guiming Peng ◽  
Xueqing Xu ◽  
Gang Xu

The ramping solar energy to electricity conversion efficiencies of hybrid organic-inorganic perovskite solar cells during the last five years have opened new doors to low-cost solar energy. The record power conversion efficiency has climbed to 19.3% in August 2014 and then jumped to 20.1% in November. In this review, the main achievements for perovskite solar cells categorized from a viewpoint of device structure are overviewed. The challenges and prospects for future development of this field are also briefly presented.


Author(s):  
Duc

Perovskites are increasingly proved to be a promising candidate for making absorber materials for high-efficiency and low-cost next-generation solar cells. There are several models proposed for perovskite solar cells similar to the conventional solar cells; their operation also has specific characteristics and requires the development of a more general physical model to study, thus optimizing the cells and improving the performance of the panels. This paper develops such a physics-based intuitive model to consider the performance of two high-efficiency types of perovskite solar cells, taking into account heterogeneous properties, with filtered transport layers, recombination, charge selection, and voltage-dependent collector. This model would allow experimentally to estimate critical parameters of perovskite solar cells, understand the performance bottleneck, and predict the performance of perovskite solar cells and suggest further study for perovskite solar cell technology development.   


2019 ◽  
Vol 7 (18) ◽  
pp. 5235-5243 ◽  
Author(s):  
Arthur Connell ◽  
Zhiping Wang ◽  
Yen-Hung Lin ◽  
Peter C. Greenwood ◽  
Alan A. Wiles ◽  
...  

Organic hole-transporting materials (HTM) have shown excellent ability in achieving high efficiency perovskite solar cells.


RSC Advances ◽  
2020 ◽  
Vol 10 (66) ◽  
pp. 40341-40350 ◽  
Author(s):  
Tarek I. Alanazi ◽  
Onkar S. Game ◽  
Joel A. Smith ◽  
Rachel C. Kilbride ◽  
Claire Greenland ◽  
...  

The addition of alkali metal halides to hybrid perovskite materials can significantly impact their crystallisation and hence their performance when used in solar cell devices.


2019 ◽  
Vol 7 (36) ◽  
pp. 20494-20518 ◽  
Author(s):  
Bo Li ◽  
Lin Fu ◽  
Shuang Li ◽  
Hui Li ◽  
Lu Pan ◽  
...  

High-efficiency and low-cost perovskite solar cells (PSCs) are desirable candidates for addressing the scalability challenge of renewable solar energy.


Nanomaterials ◽  
2020 ◽  
Vol 10 (9) ◽  
pp. 1676
Author(s):  
Md. Shahiduzzaman ◽  
Daiki Kuwahara ◽  
Masahiro Nakano ◽  
Makoto Karakawa ◽  
Kohshin Takahashi ◽  
...  

The most frequently used n-type electron transport layer (ETL) in high-efficiency perovskite solar cells (PSCs) is based on titanium oxide (TiO2) films, involving a high-temperature sintering (>450 °C) process. In this work, a dense, uniform, and pinhole-free compact titanium dioxide (TiOx) film was prepared via a facile chemical bath deposition process at a low temperature (80 °C), and was applied as a high-quality ETL for efficient planar PSCs. We tested and compared as-deposited substrates sintered at low temperatures (< 150 °C) and high temperatures (> 450 °C), as well as their corresponding photovoltaic properties. PSCs with a high-temperature treated TiO2 compact layer (CL) exhibited power conversion efficiencies (PCEs) as high as 15.50%, which was close to those of PSCs with low-temperature treated TiOx (14.51%). This indicates that low-temperature treated TiOx can be a potential ETL candidate for planar PSCs. In summary, this work reports on the fabrication of low-temperature processed PSCs, and can be of interest for the design and fabrication of future low-cost and flexible solar modules.


RSC Advances ◽  
2020 ◽  
Vol 10 (48) ◽  
pp. 29010-29017 ◽  
Author(s):  
Muhammad Adnan ◽  
Zobia Irshad ◽  
Jae Kwan Lee

Sequential all-dip-coating processed perovskite materials was conducted in an aqueous non-halide lead precursor solution, which was followed by that in a mixed halide solution for high-efficiency perovskite solar cells.


2015 ◽  
Vol 1771 ◽  
pp. 171-179 ◽  
Author(s):  
Zonglong Zhu ◽  
Shihe Yang

ABSTRACTPerovskite solar cells have caught wide attention. High efficiency, low-cost and high stability are among the major goals, which could eventually move the perovskite solar cells to the market. To achieve these goals, interface deliberation and nanostructural engineering hold the key.


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