scholarly journals Differences in the Evolution of Pyrocumulonimbus and Volcanic Stratospheric Plumes as Observed by CATS and CALIOP Space-Based Lidars

Atmosphere ◽  
2020 ◽  
Vol 11 (10) ◽  
pp. 1035
Author(s):  
Kenneth Christian ◽  
John Yorks ◽  
Sampa Das
Keyword(s):  
Pacific Northwest ◽  
Stratospheric Aerosol ◽  
Volcanic Aerosol ◽  
Volcanic Plumes ◽  
Size And Shape ◽  
Altitude Dependence ◽  
Volcanic Events ◽  
Spatial Propagation ◽  
Depolarization Ratios

Recent fire seasons have featured volcanic-sized injections of smoke aerosols into the stratosphere where they persist for many months. Unfortunately, the aging and transport of these aerosols are not well understood. Using space-based lidar, the vertical and spatial propagation of these aerosols can be tracked and inferences can be made as to their size and shape. In this study, space-based CATS and CALIOP lidar were used to track the evolution of the stratospheric aerosol plumes resulting from the 2019–2020 Australian bushfire and 2017 Pacific Northwest pyrocumulonimbus events and were compared to two volcanic events: Calbuco (2015) and Puyehue (2011). The pyrocumulonimbus and volcanic aerosol plumes evolved distinctly, with pyrocumulonimbus plumes rising upwards of 10 km after injection to altitudes of 30 km or more, compared to small to modest altitude increases in the volcanic plumes. We also show that layer-integrated depolarization ratios in these large pyrocumulonimbus plumes have a strong altitude dependence with more irregularly shaped particles in the higher altitude plumes, unlike the volcanic events studied.

Seasonally Modulated Tropical Drought Induced by Volcanic Aerosol

2011 ◽  
Vol 24 (8) ◽  
pp. 2045-2060 ◽  
Author(s):  
Renu Joseph ◽  
Ning Zeng
Keyword(s):  
Heat Capacity ◽  
Internal Variability ◽  
Stratospheric Aerosol ◽  
Volcanic Aerosol ◽  
Equatorial Africa ◽  
Precipitation Response ◽  
Volcanic Events ◽  
Clear Identification ◽  
Volcanic Impact ◽  
The Difference

Abstract Major volcanic events with a high loading of stratospheric aerosol have long been known to cause cooling, but their impact on precipitation has only recently been emphasized, especially as an analog for potential geoengineering of climate. Here, the authors use a coupled atmosphere–ocean–land–vegetation model in conjunction with observations to study the effects of volcanic aerosol on the tropical and subtropical precipitation. The small internal variability in the model enables a clear identification of the volcanic impact, which is broadly supported by observations, especially for the large Pinatubo event. Area averaged rainfall over land between 40°S and 40°N decreases by about 0.15 mm day−1, 4–5 months after the height of a major volcanic aerosol loading, such as from Pinatubo, with regional changes as large as 0.6 mm day−1 or higher, such as over the Amazon and equatorial Africa. These anomalies migrate seasonally, following the movement of monsoon rainfall. This is because the low heat capacity of the land leads to rapid response of rainfall there, owing to the energy imbalance caused by volcanic aerosol cooling. In contrast, precipitation response over the ocean is much slower and considerably damped because of the much larger heat capacity. In addition, the difference in heat capacities over land and over ocean leads to an anomalous land–sea thermal contrast, which could further contribute to the reduction of rainfall over land. The volcano-induced drought may have significant impact on the ecosystem, agriculture, and the carbon cycle, especially in the monsoon regions.

scholarly journals Effect of volcanic aerosol on stratospheric NO<sub>2</sub> and N<sub>2</sub>O<sub>5</sub> from 2002–2014 as measured by Odin-OSIRIS and Envisat-MIPAS

2016 ◽  
Author(s):  
Cristen Adams ◽  
Adam E. Bourassa ◽  
Chris A. McLinden ◽  
Chris E. Sioris ◽  
Thomas von Clarmann ◽  
...  
Keyword(s):  
Infrared Imaging ◽  
Pearson Correlation ◽  
Michelson Interferometer ◽  
Correlation Coefficients ◽  
Volcanic Eruptions ◽  
Stratospheric Aerosol ◽  
Volcanic Aerosol ◽  
Quasi Biennial Oscillation ◽  
El Chichón ◽  
El Chichon

Abstract. Following the large volcanic eruptions of Pinatubo in 1991 and El Chichón in 1982, decreases in stratospheric NO2 associated with enhanced aerosol were observed. The Optical Spectrograph and InfraRed Imaging Spectrometer (OSIRIS) likewise measured widespread enhancements of stratospheric aerosol following seven volcanic eruptions between 2002 and 2014, although the magnitudes of these eruptions were all much smaller than the Pinatubo and El Chichón eruptions. In order to isolate and quantify the relationship between volcanic aerosol and NO2, NO2 anomalies were calculated using measurements from OSIRIS and the Michelson Interferometer for Passive Atmospheric Sounding (MIPAS). In the tropics, variability due to the quasi-biennial oscillation was subtracted from the timeseries. OSIRIS profile measurements indicate that the strongest relationships between NO2 and volcanic aerosol extinction were for the layer ~ 3–7 km above the tropopause, where OSIRIS stratospheric NO2 partial columns for ~ 3–7 km above the tropopause were found to be smaller than baseline levels during these aerosol enhancements by up to ~ 60 % with typical Pearson correlation coefficients of R ~ −0.7. MIPAS also observed decreases in NO2 partial columns during periods of affected by volcanic aerosol, with percent differences of up to ~ 25 %. An even stronger relationship was observed between OSIRIS aerosol optical depth and MIPAS N2O5 partial columns, with R ~ −0.9, although no link with MIPAS HNO3 was observed. The variation of OSIRIS NO2 with increasing aerosol was found to be quantitatively consistent with simulations from a photochemical box model in terms of both magnitude and degree of non-linearity.

scholarly journals Ship-borne lidar measurements showing the progression of the tropical reservoir of volcanic aerosol after the June 1991 Pinatubo eruption

2020 ◽  
Author(s):  
Juan-Carlos Antuña-Marrero ◽  
Graham W. Mann ◽  
Philippe Keckhut ◽  
Sergey Avdyushin ◽  
Bruno Nardi ◽  
...  
Keyword(s):  
Lower Layer ◽  
Extinction Ratio ◽  
Stratospheric Aerosol ◽  
Original Text ◽  
Aerosol Extinction ◽  
Volcanic Aerosol ◽  
Tropical Reservoir ◽  
Aerosol Cloud ◽  
Pinatubo Eruption ◽  
The Tropics

Abstract. A key limitation of volcanic forcing datasets for the Pinatubo period, is the large uncertainty that remains with respect to the extent of the optical depth of the Pinatubo aerosol cloud in the first year after the eruption, the saturation of the SAGE-II instrument restricting it to only be able to measure the upper part of the aerosol cloud in the tropics. Here we report the recovery of stratospheric aerosol measurements from two ship-borne lidars, both of which measured the tropical reservoir of volcanic aerosol produced by the June 1991 Mount Pinatubo eruption. The lidars were on-board two Soviet vessels, each ship crossing the Atlantic, their measurement datasets providing unique observational transects of the Pinatubo cloud across the tropics from Europe to the Caribbean (~ 40° N to 8° N) from July to September 1991 (the Prof Zubov ship) and from Europe to south of the Equator (8° S to ~ 40° N) between January and February 1992 (the Prof Vize ship). Our philosophy with the data recovery is to follow the same algorithms and parameters appearing in the two peer-reviewed articles that presented these datasets in the same issue of GRL in 1993, and here we provide all 48 lidar soundings made from the Prof. Zubov, and 11 of the 20 conducted from the Prof. Vize, ensuring we have reproduced the aerosols backscatter and extinction values in the Figures of those two papers. These original approaches used thermodynamic properties from the CIRA-86 standard atmosphere to derive the molecular backscattering, vertically and temporally constant values applied for the aerosol backscatter to extinction ratio and the correction factor of the aerosols backscattering wavelength dependence. We demonstrate this initial validation of the recovered stratospheric aerosol extinction profiles, providing full details of each dataset in this paper's Supplement S1, the original text files of the backscatter ratio, the calculated aerosols backscatter and extinction profiles. We anticipate the data providing potential new observational case studies for modelling analyses, including a 1-week series of consecutive soundings (in September 1991) at the same location showing the progression of the entrainment of part of the Pinatubo plume into the upper troposphere and the formation of an associated cirrus cloud. The Zubov lidar dataset illustrates how the tropically confined Pinatubo aerosol cloud transformed from a highly heterogeneous vertical structure in August 1991, maximum aerosol extinction values around 19 km for the lower layer and 23–24 for the upper layer, to a more homogeneous and deeper reservoir of volcanic aerosol in September 1991. We encourage modelling groups to consider new analyses of the Pinatubo cloud, comparing to the recovered datasets, with the potential to increase our understanding of the evolution of the Pinatubo aerosol cloud and its effects. Data described in this work are available at https://doi.pangaea.de/10.1594/PANGAEA.912770 (Antuña-Marrero et al., 2020).

A global perspective on Bromine monoxide composition in volcanic plumes derived from three years of S5-P/TROPOMI data

2021 ◽  
Author(s):  
Simon Warnach ◽  
Holger Sihler ◽  
Christian Borger ◽  
Nicole Bobrowski ◽  
Stefan Schmitt ◽  
...  
Keyword(s):  
Global Perspective ◽  
Coefficient Of Determination ◽  
Optical Absorption Spectroscopy ◽  
Polar Regions ◽  
Volcanic Gas ◽  
Volcanic Plumes ◽  
Molar Ratios ◽  
Volcanic Events ◽  
Global Coverage

&lt;p&gt;Bromine monoxide (BrO) is a halogen radical capable of influencing atmospheric chemical processes, in particular the abundance of ozone, e. g. in the troposphere of polar regions, the stratosphere as well as in volcanic plumes. Furthermore, the molar bromine to sulphur ratio in volcanic gas emissions is a proxy for the magmatic composition of a volcano and potentially an eruption forecast parameter.&lt;/p&gt;&lt;p&gt;The high spatial resolution of the S5-P/TROPOMI instrument (up to 3.5x5.5km&lt;sup&gt;2&lt;/sup&gt;) and its daily global coverage offer the potential to detect BrO even during minor eruptions and also to determine BrO/SO&lt;sub&gt;2&lt;/sub&gt; ratios during continuous passive degassing.&lt;/p&gt;&lt;p&gt;Here, we present a global overview of BrO/SO&lt;sub&gt;2&lt;/sub&gt; molar ratios in volcanic plumes derived from a systematic long-term investigation of three years of TROPOMI data.&lt;/p&gt;&lt;p&gt;We retrieved column densities of BrO and SO&lt;sub&gt;2&lt;/sub&gt; using Differential Optical Absorption Spectroscopy (DOAS) and calculated mean BrOSO&lt;sub&gt;2&lt;/sub&gt; molar ratios for each volcano. As expected, the calculated BrO/SO&lt;sub&gt;2&lt;/sub&gt; molar ratios differ strongly between different volcanoes ranging from several 10&lt;sup&gt;-5&lt;/sup&gt; up to several 10&lt;sup&gt;-4&lt;/sup&gt;. In our study of three years of S5P/TROPOMI data we successfully recorded elevated BrO column densities for more than 100 volcanic events and were able to derive meaningful (coefficient of determination, R&lt;sup&gt;2&lt;/sup&gt; exceeding 0.5) BrO/SO&lt;sub&gt;2&lt;/sub&gt; ratios for multiple volcanoes.&lt;/p&gt;

scholarly journals Easy Volcanic Aerosol (EVA v1.0): An idealized forcing generator for climate simulations

2016 ◽  
Author(s):  
Matthew Toohey ◽  
Bjorn Stevens ◽  
Hauke Schmidt ◽  
Claudia Timmreck
Keyword(s):  
Time Scale ◽  
Climate Models ◽  
Single Scattering ◽  
Stratospheric Aerosol ◽  
Asymmetry Factor ◽  
Volcanic Aerosol ◽  
Climate Simulations ◽  
Simple Scaling ◽  
Millennial Time Scale ◽  
Aerosol Properties

Abstract. The Easy Volcanic Aerosol (EVA) forcing generator produces stratospheric aerosol optical properties as a function of time, latitude, height and wavelength for a given input list of volcanic eruption attributes. EVA is based on a parameterized three-box model of stratospheric transport, and simple scaling relationships used to derive mid-visible (550 nm) aerosol optical depth and aerosol effective radius from stratospheric sulfate mass. Pre-calculated look up tables computed from Mie theory are used to produce wavelength dependent aerosol extinction, single scattering albedo and scattering asymmetry factor values. The structural form of EVA, and the tuning of its parameters, are chosen to produce best agreement with the satellite-based reconstruction of stratospheric aerosol properties following the 1991 Pinatubo eruption, and with prior millennial-time scale forcing reconstructions including the 1815 eruption of Tambora. EVA can be used to produce volcanic forcing for climate models which is based on recent observations and physical understanding, but internally self-consistent over any time-scale of choice. In addition, EVA is constructed so as to allow for easy modification of different aspects of aerosol properties, in order to be used in model experiments to help advance understanding of what aspects of the volcanic aerosol are important for the climate system.

scholarly journals Long-range isentropic transport of stratospheric aerosols over Southern Hemisphere following the Calbuco eruption in April 2015

2017 ◽  
Author(s):  
Nelson Bègue ◽  
Damien Vignelles ◽  
Gwenaël Berthet ◽  
Thierry Portafaix ◽  
Guillaume Payen ◽  
...  
Keyword(s):  
Southern Hemisphere ◽  
Transient Behavior ◽  
Stratospheric Aerosol ◽  
Aerosol Layer ◽  
Reunion Island ◽  
Volcanic Aerosol ◽  
Réunion Island ◽  
One Year ◽  
The Impact ◽  
Aerosol Plume

Abstract. After 43 years of inactivity, the Calbuco volcano which is located in the southern part of Chile erupted on 22 April 2015. The space-time evolutions (distribution and transport) of its aerosol plume are investigated by combining satellite (CALIOP, IASI, OMPS), in situ aerosol counting (LOAC OPC) and lidar observations, and the MIMOSA advection model. The Calbuco aerosol plume reached the Indian Ocean 1 week after the eruption. Over the Reunion Island site (21° S; 55.5° E), the aerosol signal was unambiguously enhanced in comparison with "background" conditions with a volcanic aerosol layer extending from 18 km to 21 km during the May–July period. All the data reveal an increase by a factor of ~ 2 in the SAOD (Stratospheric Aerosol Optical Depth) with respect to values observed before the eruption. The aerosol e-folding time is approximately 90 days. Microphysical measurements obtained before, during and after the eruption reflecting the impact of the Calbuco eruption on the lower stratospheric aerosol content have been analyzed over Reunion site. During the passage of the plume, the volcanic aerosol was characterized by an effective radius of 0.16 ± 0.02 µm with an unimodal lognormal size distribution and the aerosol number concentration appears 20 times higher than before and one year after the eruption. A tendency toward "background" conditions has been observed about one year after the eruption, by April 2016. The volcanic aerosol plume is advected eastward in the Southern Hemisphere and its latitudinal extent is clearly bounded by the subtropical barrier and the polar vortex. The transient behavior of the aerosol layers observed above Reunion Island between May and July 2015 reflects an inhomogeneous geographical distribution of the plume which is controlled by the latitudinal motion of these dynamical barriers.

Model comparison of volcanic aerosol forcing and climate impact of tropical and extratropical eruptions

2021 ◽  
Author(s):  
Zhihong Zhuo ◽  
Herman Fuglestvedt ◽  
Matthew Toohey ◽  
Michael J. Mills ◽  
Kirstin Krüger
Keyword(s):  
Large Scale ◽  
Model Comparison ◽  
Climate Model ◽  
Volcanic Eruptions ◽  
Climate Impact ◽  
Stratospheric Aerosol ◽  
Volcanic Aerosol ◽  
Surface Cooling ◽  
Aerosol Forcing ◽  
Central American Volcanic Arc

&lt;p&gt;Major volcanic eruptions increase sulfate aerosols in the stratosphere. This causes a large-scale dimming effect with significant surface cooling and stratosphere warming. However, the climate impact differs for tropical and extratropical eruptions, and depends on the eruption season and height, and volcanic volatiles injections. In order to study different volcanic aerosol forcing and their climate impact, we perform simulations based on the fully coupled Community Earth System Model version 2 (CESM2) with the version 6 of the Whole Atmosphere Community Climate Model (WACCM6) with prognostic stratospheric aerosol and chemistry. In this study, explosive eruptions at 14.6 N and 63.6 N in January and July injecting 17 MT and 200 MT SO&lt;sub&gt;2&lt;/sub&gt; at 24 km with and without halogens are simulated, in line with Central American Volcanic Arc and Icelandic volcanic eruptions. Simulated changes in the stratospheric sulfate and halogen burdens, and related impacts on aerosol optical depth, radiation, ozone and surface climate are analyzed. These simulated volcanic eruption cases will be compared with simulations based on the aerosol-climate model MAECHAM5-HAM.&lt;/p&gt;

Interactive Stratospheric Aerosol models response to different sulfur injection amount and altitude distribution during volcanic eruption

2021 ◽  
Author(s):  
Ilaria Quaglia ◽  
Christoph Brühl ◽  
Sandip Dhomse ◽  
Henning Franke ◽  
Anton Laakso ◽  
...  
Keyword(s):  
Volcanic Eruptions ◽  
Stratospheric Aerosol ◽  
Climate Modelling ◽  
Aerosol Layer ◽  
Volcanic Aerosol ◽  
Surface Cooling ◽  
Altitude Distribution ◽  
Aerosol Cloud ◽  
Modelling Studies ◽  
Intercomparison Project

&lt;p&gt;Large magnitude tropical volcanic eruptions emit sulphur dioxide and other gases directly into the stratosphere, creating a long-lived volcanic aerosol cloud which scatter incoming solar radiation, absorbs outgoing terrestrial radiation, and can strongly affect the composition of the stratosphere.&lt;/p&gt;&lt;p&gt;Such major volcanic enhancements of the stratospheric aerosol layer have strong &amp;#8220;direct effects&amp;#8221; on climate via these influences on radiative transfer, primarily surface cooling via the reduced insolation, but also have a range of indirect effects, due to the volcanic aerosol cloud&amp;#8217;s effects on stratospheric circulation, dynamics and chemistry.&lt;/p&gt;&lt;p&gt;In this study, we investigate the 3 largest volcanic enhancements to the stratospheric aerosol layer in the last 100 years (Mt Agung 1963; Mt El Chich&amp;#243;n 1982; Mt Pinatubo 1991), comparing co-ordinated simulations within the so-called HErSEA experiments (Historical Eruptions SO2 Emission Assessment) several national climate modelling centres carried out for the model intercomparison project ISA-MIP.&lt;/p&gt;&lt;p&gt;The HErSEA experiment saw participating models performing interactive stratospheric aerosol simulations of each of the volcanic aerosol clouds with common upper-, mid- and lower-estimate amounts and injection heights of sulfur dioxide, in order to better understand known differences among modelling studies for which initial emission gives best agreement with observations.&amp;#160;&lt;/p&gt;&lt;p&gt;First, we compare results of several models HErSEA simulations with a range of observations, with the aim to find where there is agreement between the models and where there are differences, at the different initial sulfur injection amount and altitude distribution.&lt;/p&gt;&lt;p&gt;In this way, we could understand the differences and limitations in the mechanisms that controls the dynamical, microphysical and chemical processes of stratospheric aerosol layer.&lt;/p&gt;

Stratospheric residence time and the lifetime of volcanic aerosol

2021 ◽  
Author(s):  
Matthew Toohey ◽  
Yue Jia ◽  
Susann Tegetmeier
Keyword(s):  
Residence Time ◽  
Volcanic Eruptions ◽  
Stratospheric Aerosol ◽  
Volcanic Aerosol ◽  
Aerosol Forcing ◽  
Radiative Impact ◽  
The Common ◽  
The Impact ◽  
The Relationship ◽  
Common Era

&lt;p&gt;The cumulative radiative impact of major volcanic eruptions depends strongly on the length of time volcanic sulfate aerosol remains in the stratosphere. Observations of aerosol from recent eruptions have been used to suggest that residence time depends on the latitude of the volcanic eruption, with tropical eruptions producing aerosol loading that persists longer than that from extratropical eruptions. However, the limited number of eruptions observed make it difficult to disentangle the roles of latitude and injection height in controlling aerosol lifetime. Here we use satellite observations and model experiments to explore the relationship between eruption latitude, injection height and resulting residence time of stratospheric aerosol. We find that contrary to earlier interpretations of observations, the residence time of aerosol from major tropical eruptions like Pinatubo (1991) is on the order of 24 months. Model results suggest that the residence time is greatly sensitive to the height of the sulfur injection, especially within the lowest few kilometers of the stratosphere. As injection heights and latitudes are unknown for the majority of eruptions over the common era, we estimate the impact of this uncertainty on volcanic aerosol forcing reconstructions.&amp;#160;&lt;/p&gt;

scholarly journals Effect of volcanic aerosol on stratospheric NO<sub>2</sub> and N<sub>2</sub>O<sub>5</sub> from 2002–2014 as measured by Odin-OSIRIS and Envisat-MIPAS

2017 ◽  
Vol 17 (13) ◽  
pp. 8063-8080 ◽  
Author(s):  
Cristen Adams ◽  
Adam E. Bourassa ◽  
Chris A. McLinden ◽  
Chris E. Sioris ◽  
Thomas von Clarmann ◽  
...  
Keyword(s):  
Infrared Imaging ◽  
Pearson Correlation ◽  
Michelson Interferometer ◽  
Correlation Coefficients ◽  
Volcanic Eruptions ◽  
Stratospheric Aerosol ◽  
Volcanic Aerosol ◽  
Quasi Biennial Oscillation ◽  
El Chichón ◽  
El Chichon

Abstract. Following the large volcanic eruptions of Pinatubo in 1991 and El Chichón in 1982, decreases in stratospheric NO2 associated with enhanced aerosol were observed. The Optical Spectrograph and Infrared Imaging Spectrometer (OSIRIS) measured the widespread enhancements of stratospheric aerosol following seven volcanic eruptions between 2002 and 2014, although the magnitudes of these eruptions were all much smaller than the Pinatubo and El Chichón eruptions. In order to isolate and quantify the relationship between volcanic aerosol and NO2, NO2 anomalies were calculated using measurements from OSIRIS and the Michelson Interferometer for Passive Atmospheric Sounding (MIPAS). In the tropics, variability due to the quasi-biennial oscillation was subtracted from the time series. OSIRIS profile measurements indicate that the strongest anticorrelations between NO2 and volcanic aerosol extinction were for the 5 km layer starting  ∼  3 km above the climatological mean tropopause at the given latitude. OSIRIS stratospheric NO2 partial columns in this layer were found to be smaller than background NO2 levels during these aerosol enhancements by up to  ∼  60 % with typical Pearson correlation coefficients of R ∼ −0. 7. MIPAS also observed decreases in NO2 partial columns during periods affected by volcanic aerosol, with percent differences of up to  ∼  25 % relative to background levels. An even stronger anticorrelation was observed between OSIRIS aerosol optical depth and MIPAS N2O5 partial columns, with R ∼ −0. 9, although no link with MIPAS HNO3 was observed. The variation in OSIRIS NO2 with increasing aerosol was found to be consistent with simulations from a photochemical box model within the estimated model uncertainty.

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