scholarly journals Biogenic Aerosol in the Artic from Eight Years of MSA Data from Ny Ålesund (Svalbard Islands) and Thule (Greenland)

Atmosphere ◽  
2019 ◽  
Vol 10 (7) ◽  
pp. 349 ◽  
Author(s):  
Silvia Becagli ◽  
Alessandra Amore ◽  
Laura Caiazzo ◽  
Tatiana Di Iorio ◽  
Alcide di Sarra ◽  
...  

In remote marine areas, biogenic productivity and atmospheric particulate are coupled through dimethylsulfide (DMS) emission by phytoplankton. Once in the atmosphere, the gaseous DMS is oxidized to produce H2SO4 and methanesulfonic acid (MSA); both species can affect the formation of cloud condensation nuclei. This study analyses eight years of biogenic aerosol evolution and variability at two Arctic sites: Thule (76.5° N, 68.8° W) and Ny Ålesund (78.9° N, 11.9° E). Sea ice plays a key role in determining the MSA concentration in polar regions. At the beginning of the melting season, in April, up to June, the biogenic aerosol concentration appears inversely correlated with sea ice extent and area, and positively correlated with the extent of the ice-free area in the marginal ice zone (IF-MIZ). The upper ocean stratification induced by sea ice melting might have a role in these correlations, since the springtime formation of this surface layer regulates the accumulation of phytoplankton and nutrients, allowing the DMS to escape from the sea to the atmosphere. The multiyear analysis reveals a progressive decrease in MSA concentration in May at Thule and an increase in July August at Ny Ålesund. Therefore, while the MSA seasonal evolution is mainly related with the sea ice retreat in April, May, and June, the IF-MIZ extent appears as the main factor affecting the longer-term behavior of MSA.

2013 ◽  
Vol 13 (6) ◽  
pp. 17087-17121 ◽  
Author(s):  
J. Browse ◽  
K. S. Carslaw ◽  
G. W. Mann ◽  
C. E. Birch ◽  
S. R. Arnold ◽  
...  

Abstract. Loss of summertime Arctic sea ice will lead to a large increase in the emission of aerosols and precursor gases from the ocean surface. It has been suggested that these enhanced emissions will exert substantial aerosol radiative forcings, dominated by the indirect effect of aerosol on clouds. Here, we investigate the potential for these indirect forcings using a global aerosol microphysics model evaluated against aerosol observations from the ASCOS campaign to examine the response of Arctic cloud condensation nuclei (CCN) to sea-ice retreat. In response to a complete loss of summer ice, we find that north of 70° N emission fluxes of sea-salt, marine primary organic aerosol (OA) and dimethyl sulphide increase by a factor of ~10, ~4 and ~15, respectively. However, the CCN response is weak, with negative changes over the central Arctic ocean. The weak response is due to the efficient scavenging of aerosol by extensive drizzling stratocumulus clouds. In the scavenging-dominated Arctic environment, the production of condensable vapour from oxidation of dimethyl sulphide grows particles to sizes where they can be scavenged. This loss is not sufficiently compensated by new particle formation, due to the suppression of nucleation by the large condensation sink resulting from sea-salt and primary OA emissions. Thus, our results suggest that increased aerosol emissions will not cause a climate feedback through changes in cloud microphysical and radiative properties.


2012 ◽  
Vol 25 (13) ◽  
pp. 4736-4743 ◽  
Author(s):  
M. Årthun ◽  
T. Eldevik ◽  
L. H. Smedsrud ◽  
Ø. Skagseth ◽  
R. B. Ingvaldsen

Abstract The recent Arctic winter sea ice retreat is most pronounced in the Barents Sea. Using available observations of the Atlantic inflow to the Barents Sea and results from a regional ice–ocean model the authors assess and quantify the role of inflowing heat anomalies on sea ice variability. The interannual variability and longer-term decrease in sea ice area reflect the variability of the Atlantic inflow, both in observations and model simulations. During the last decade (1998–2008) the reduction in annual (July–June) sea ice area was 218 × 103 km2, or close to 50%. This reduction has occurred concurrent with an increase in observed Atlantic heat transport due to both strengthening and warming of the inflow. Modeled interannual variations in sea ice area between 1948 and 2007 are associated with anomalous heat transport (r = −0.63) with a 70 × 103 km2 decrease per 10 TW input of heat. Based on the simulated ocean heat budget it is found that the heat transport into the western Barents Sea sets the boundary of the ice-free Atlantic domain and, hence, the sea ice extent. The regional heat content and heat loss to the atmosphere scale with the area of open ocean as a consequence. Recent sea ice loss is thus largely caused by an increasing “Atlantification” of the Barents Sea.


2016 ◽  
Vol 29 (24) ◽  
pp. 9179-9188 ◽  
Author(s):  
Erica Rosenblum ◽  
Ian Eisenman

Abstract The downward trend in Arctic sea ice extent is one of the most dramatic signals of climate change during recent decades. Comprehensive climate models have struggled to reproduce this trend, typically simulating a slower rate of sea ice retreat than has been observed. However, this bias has been widely noted to have decreased in models participating in phase 5 of the Coupled Model Intercomparison Project (CMIP5) compared with the previous generation of models (CMIP3). Here simulations are examined from both CMIP3 and CMIP5. It is found that simulated historical sea ice trends are influenced by volcanic forcing, which was included in all of the CMIP5 models but in only about half of the CMIP3 models. The volcanic forcing causes temporary simulated cooling in the 1980s and 1990s, which contributes to raising the simulated 1979–2013 global-mean surface temperature trends to values substantially larger than observed. It is shown that this warming bias is accompanied by an enhanced rate of Arctic sea ice retreat and hence a simulated sea ice trend that is closer to the observed value, which is consistent with previous findings of an approximately linear relationship between sea ice extent and global-mean surface temperature. Both generations of climate models are found to simulate Arctic sea ice that is substantially less sensitive to global warming than has been observed. The results imply that much of the difference in Arctic sea ice trends between CMIP3 and CMIP5 occurred because of the inclusion of volcanic forcing, rather than improved sea ice physics or model resolution.


2014 ◽  
Vol 14 (14) ◽  
pp. 7543-7557 ◽  
Author(s):  
J. Browse ◽  
K. S. Carslaw ◽  
G. W. Mann ◽  
C. E. Birch ◽  
S. R. Arnold ◽  
...  

Abstract. Loss of summertime Arctic sea ice will lead to a large increase in the emission of aerosols and precursor gases from the ocean surface. It has been suggested that these enhanced emissions will exert substantial aerosol radiative forcings, dominated by the indirect effect of aerosol on clouds. Here, we investigate the potential for these indirect forcings using a global aerosol microphysics model evaluated against aerosol observations from the Arctic Summer Cloud Ocean Study (ASCOS) campaign to examine the response of Arctic cloud condensation nuclei (CCN) to sea-ice retreat. In response to a complete loss of summer ice, we find that north of 70° N emission fluxes of sea salt, marine primary organic aerosol (OA) and dimethyl sulfide increase by a factor of ~ 10, ~ 4 and ~ 15 respectively. However, the CCN response is weak, with negative changes over the central Arctic Ocean. The weak response is due to the efficient scavenging of aerosol by extensive drizzling stratocumulus clouds. In the scavenging-dominated Arctic environment, the production of condensable vapour from oxidation of dimethyl sulfide grows particles to sizes where they can be scavenged. This loss is not sufficiently compensated by new particle formation, due to the suppression of nucleation by the large condensation sink resulting from sea-salt and primary OA emissions. Thus, our results suggest that increased aerosol emissions will not cause a climate feedback through changes in cloud microphysical and radiative properties.


2021 ◽  
Vol 2 (1) ◽  
Author(s):  
Alex Crawford ◽  
Julienne Stroeve ◽  
Abigail Smith ◽  
Alexandra Jahn

AbstractThe shrinking of Arctic-wide September sea ice extent is often cited as an indicator of modern climate change; however, the timing of seasonal sea ice retreat/advance and the length of the open-water period are often more relevant to stakeholders working at regional and local scales. Here we highlight changes in regional open-water periods at multiple warming thresholds. We show that, in the latest generation of models from the Coupled Model Intercomparison Project (CMIP6), the open-water period lengthens by 63 days on average with 2 °C of global warming above the 1850-1900 average, and by over 90 days in several Arctic seas. Nearly the entire Arctic, including the Transpolar Sea Route, has at least 3 months of open water per year with 3.5 °C warming, and at least 6 months with 5 °C warming. Model bias compared to satellite data suggests that even such dramatic projections may be conservative.


2011 ◽  
Vol 24 (20) ◽  
pp. 5325-5335 ◽  
Author(s):  
Ian Eisenman ◽  
Tapio Schneider ◽  
David S. Battisti ◽  
Cecilia M. Bitz

Abstract The Northern Hemisphere sea ice cover has diminished rapidly in recent years and is projected to continue to diminish in the future. The year-to-year retreat of Northern Hemisphere sea ice extent is faster in summer than winter, which has been identified as one of the most striking features of satellite observations as well as of state-of-the-art climate model projections. This is typically understood to imply that the sea ice cover is most sensitive to climate forcing in summertime, and previous studies have explained this by calling on factors such as the surface albedo feedback. In the Southern Hemisphere, however, it is the wintertime sea ice extent that retreats fastest in climate model projections. Here, it is shown that the interhemispheric differences in the model projections can be attributed to differences in coastline geometry, which constrain where sea ice can occur. After accounting for coastline geometry, it is found that the sea ice changes simulated in both hemispheres in most climate models are consistent with sea ice retreat being fastest in winter in the absence of landmasses. These results demonstrate that, despite the widely differing rates of ice retreat among climate model projections, the seasonal structure of the sea ice retreat is robust among the models and is uniform in both hemispheres.


2014 ◽  
Vol 8 (1) ◽  
pp. 273-288 ◽  
Author(s):  
I. Eisenman ◽  
W. N. Meier ◽  
J. R. Norris

Abstract. Recent estimates indicate that the Antarctic sea ice cover is expanding at a statistically significant rate with a magnitude one third as large as the rapid rate of sea ice retreat in the Arctic. However, during the mid-2000s, with several fewer years in the observational record, the trend in Antarctic sea ice extent was reported to be considerably smaller and statistically indistinguishable from zero. Here, we show that the increase in the reported trend occurred primarily due to the effect of a previously undocumented change in the way the satellite sea ice observations are processed for the widely-used Bootstrap algorithm dataset, rather than a physical increase in the rate of ice advance. Although our analysis does not definitively identify whether this undocumented change introduced an error or removed one, the resulting difference in the trends suggests that a substantial error exists in either the current dataset or the version that was used prior to the mid-2000s, and numerous studies that have relied on these observations should be reexamined to determine the sensitivity of their results to this change in the dataset. Furthermore, a number of recent studies have investigated physical mechanisms for the observed expansion of the Antarctic sea ice cover. The results of this analysis raise the possibility that this expansion may be a spurious artifact of an error in the satellite observations, and that the actual Antarctic sea ice cover may not be expanding at all.


2019 ◽  
Vol 116 (39) ◽  
pp. 19311-19317 ◽  
Author(s):  
Martí Galí ◽  
Emmanuel Devred ◽  
Marcel Babin ◽  
Maurice Levasseur

Dimethylsulfide (DMS), a gas produced by marine microbial food webs, promotes aerosol formation in pristine atmospheres, altering cloud radiative forcing and precipitation. Recent studies suggest that DMS controls aerosol formation in the summertime Arctic atmosphere and call for an assessment of pan-Arctic DMS emission (EDMS) in a context of dramatic ecosystem changes. Using a remote sensing algorithm, we show that summertime EDMS from ice-free waters increased at a mean rate of 13.3 ± 6.7 Gg S decade−1 (∼33% decade−1) north of 70°N between 1998 and 2016. This trend, mostly explained by the reduction in sea-ice extent, is consistent with independent atmospheric measurements showing an increasing trend of methane sulfonic acid, a DMS oxidation product. Extrapolation to an ice-free Arctic summer could imply a 2.4-fold (±1.2) increase in EDMS compared to present emission. However, unexpected regime shifts in Arctic geo- and ecosystems could result in future EDMS departure from the predicted range. Superimposed on the positive trend, EDMS shows substantial interannual changes and nonmonotonic multiyear trends, reflecting the interplay between physical forcing, ice retreat patterns, and phytoplankton productivity. Our results provide key constraints to determine whether increasing marine sulfur emissions, and resulting aerosol–cloud interactions, will moderate or accelerate Arctic warming in the context of sea-ice retreat and increasing low-level cloud cover.


2014 ◽  
Vol 11 (7) ◽  
pp. 1705-1716 ◽  
Author(s):  
A. Fujiwara ◽  
T. Hirawake ◽  
K. Suzuki ◽  
I. Imai ◽  
S.-I. Saitoh

Abstract. This study assesses the response of phytoplankton assemblages to recent climate change, especially with regard to the shrinking of sea ice in the northern Chukchi Sea of the western Arctic Ocean. Distribution patterns of phytoplankton groups in the late summers of 2008–2010 were analysed based on HPLC pigment signatures and, the following four major algal groups were inferred via multiple regression and cluster analyses: prasinophytes, diatoms, haptophytes and dinoflagellates. A remarkable interannual difference in the distribution pattern of the groups was found in the northern basin area. Haptophytes dominated and dispersed widely in warm surface waters in 2008, whereas prasinophytes dominated in cold water in 2009 and 2010. A difference in the onset date of sea ice retreat was evident among years–the sea ice retreat in 2008 was 1–2 months earlier than in 2009 and 2010. The spatial distribution of early sea ice retreat matched the areas in which a shift in algal community composition was observed. Steel-Dwass's multiple comparison tests were used to assess the physical, chemical and biological parameters of the four clusters. We found a statistically significant difference in temperature between the haptophyte-dominated cluster and the other clusters, suggesting that the change in the phytoplankton communities was related to the earlier sea ice retreat in 2008 and the corollary increase in sea surface temperatures. Longer periods of open water during the summer, which are expected in the future, may affect food webs and biogeochemical cycles in the western Arctic due to shifts in phytoplankton community structure.


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