UV-Driven Harmonic Generation for Time-Resolved Photoelectron Spectroscopy of Polyatomic Molecules
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A single-order harmonic pulse in the vacuum-ultraviolet (VUV) is highly desirable for time-resolved photoelectron spectroscopy (TRPES) of polyatomic molecules. A high-power 9th harmonic of a Ti:sapphire laser (hv = 14 eV) is obtained using a UV driving laser at 270 nm (the 3rd harmonic). We describe our recent efforts to develop VUV TRPES combined with UV-driven harmonic generation, and present a few representative results from our recent TRPES studies.
2017 ◽
Vol 684
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pp. 397-401
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2011 ◽
Vol 82
(6)
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pp. 063114
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2003 ◽
Vol 22
(2)
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pp. 377-405
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2018 ◽
Vol 149
(14)
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pp. 144311
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