scholarly journals Direct Measurement of Plutonium in Spent Fuel with X-ray Fluoresence

2011 ◽  
Author(s):  
Catherine E Romano ◽  
Allisa Stafford ◽  
Alexander A Solodov ◽  
Michael H Ehinger
Keyword(s):  
2000 ◽  
Vol 27 (7) ◽  
pp. 1490-1502 ◽  
Author(s):  
Masao Matsumoto ◽  
Akihide Yamamoto ◽  
Ikuko Honda ◽  
Akira Taniguchi ◽  
Hitoshi Kanamori

2019 ◽  
Vol 622 ◽  
pp. A61 ◽  
Author(s):  
R. Staubert ◽  
J. Trümper ◽  
E. Kendziorra ◽  
D. Klochkov ◽  
K. Postnov ◽  
...  

Cyclotron lines, also called cyclotron resonant scattering features are spectral features, generally appearing in absorption, in the X-ray spectra of objects containing highly magnetized neutron stars, allowing the direct measurement of the magnetic field strength in these objects. Cyclotron features are thought to be due to resonant scattering of photons by electrons in the strong magnetic fields. The main content of this contribution focusses on electron cyclotron lines as found in accreting X-ray binary pulsars (XRBP) with magnetic fields on the order of several 1012Gauss. Also, possible proton cyclotron lines from single neutron stars with even stronger magnetic fields are briefly discussed. With regard to electron cyclotron lines, we present an updated list of XRBPs that show evidence of such absorption lines. The first such line was discovered in a 1976 balloon observation of the accreting binary pulsar Hercules X-1, it is considered to be the first direct measurement of the magnetic field of a neutron star. As of today (end 2018), we list 35 XRBPs showing evidence of one ore more electron cyclotron absorption line(s). A few have been measured only once and must be confirmed (several more objects are listed as candidates). In addition to the Tables of objects, we summarize the evidence of variability of the cyclotron line as a function of various parameters (especially pulse phase, luminosity and time), and add a discussion of the different observed phenomena and associated attempts of theoretical modeling. We also discuss our understanding of the underlying physics of accretion onto highly magnetized neutron stars. For proton cyclotron lines, we present tables with seven neutron stars and discuss their nature and the physics in these objects.


1959 ◽  
Vol 37 (1) ◽  
pp. 20-28 ◽  
Author(s):  
G. L. Smithson ◽  
R. L. Eager ◽  
A. B. VanCleave

X-Ray fluorescence has been applied to the analysis of flotation concentrates obtained from pegmatitic uranium ores occurring in Northern Saskatchewan. Approximate uranium analyses can be obtained by direct measurement on flotation concentrates but more accurate results are obtained by using an internal standard such as strontium or yttrium. The time required for an analysis, as compared to that of conventional chemical or fluorimetric methods, is considerably reduced and flotation pilot plant operations can therefore be more effectively controlled. The method has been extended to include the analysis of sulphate leach liquors obtained from the leaching of pegmatitic ores and their flotation concentrates. Organic phases obtained in liquid – liquid extraction studies can also be rapidly analyzed for uranium by X-ray fluorescence.


2000 ◽  
Vol 84 (4) ◽  
pp. 773-776 ◽  
Author(s):  
J. C. Woicik ◽  
E. J. Nelson ◽  
P. Pianetta

2018 ◽  
Vol 20 (24) ◽  
pp. 16469-16476 ◽  
Author(s):  
P. T. P. Ryan ◽  
Z. Jakub ◽  
J. Balajka ◽  
J. Hulva ◽  
M. Meier ◽  
...  

The normal incidence X-ray standing wave (NIXSW) technique has been used to follow the evolution of the adsorption geometry of Ni adatoms on the Fe3O4(001)-(√2 × √2)R45° surface as a function of temperature.


1979 ◽  
Vol 23 ◽  
pp. 163-176
Author(s):  
D. C. Camp ◽  
W. D. Ruhter

In the event that nuclear fuel from light water reactors (LWR) is reprocessed to reclaim the uranium or plutonium, several analytical techniques will be used for product accountability. Generally, the isotopic content of both the plutonium and uranium in the reprocessed product will have to be accurately determined. One plan for the reprocessing of LWR spent fuel incorporates the following scheme. After separation from both the fission products and transplutonium actinides (including neptunium and americium), part of the uranium and all of the plutonium in a nitrate solution will merge together to form a coprocessed stream. This solution will be concentrated by evaporation and sent to a hold tank for accountability. Input concentrations into the hold tank could be up to 350 g U/ℓ and nearly 50 g Pu/ℓ. The variation to be expected in these concentrations is not known. The remaining uranium fraction will be further purified and sent to a separate storage tank. Its expected stream concentration will be about 60 g U/ℓ. These two relatively high actinide stream concentrations can be monitored rapidly, quantitatively, and nondestructively using the technique of energy-dispersive x-ray fluorescence analysis(XRFA).


2017 ◽  
Vol 12 (02) ◽  
pp. P02005-P02005 ◽  
Author(s):  
S. Ihle ◽  
P. Holl ◽  
D. Kalok ◽  
R. Hartmann ◽  
H. Ryll ◽  
...  

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