scholarly journals Removal of hydrogen sulfide gas using coal fly ash – blast furnace cement composite

Author(s):  
Satoshi Asaoka ◽  
Hiroyuki Saito ◽  
Tsuyoshi Ichinari ◽  
Shinjiro Hayakawa ◽  
Takahito Oikawa

Abstract The number of complaints regarding offensive odors from service industries, such as restaurants and garages, has recently increased. In this study, we aimed to develop an adsorbent for hydrogen sulfide gas derived from domestic wastewater and reveal the mechanisms of its removal. The adsorbent used for hydrogen sulfide gas removal was prepared by mixing coal fly ash and blast furnace cement with a mixing ratio of 87:13 by mass percentage. The optimum calcination temperature of the adsorbent was 700 °C to achieve a high removal performance for both dry and humid hydrogen sulfide gas. The X-ray absorption fine structure analysis revealed that hydrogen sulfide was removed on the adsorbent by oxidizing to sulfate. A pilot-scale experiment was conducted to evaluate the removal performance of hydrogen sulfide gas derived from domestic wastewater using the developed adsorbent. For a week, the average removal percentage of hydrogen sulfide gas derived from domestic wastewater remained at 99.1%. Therefore, the developed adsorbent for hydrogen sulfide gas is promising and cost-effective for promoting the recycling of coal fly ash.

Chemosphere ◽  
2017 ◽  
Vol 168 ◽  
pp. 384-389 ◽  
Author(s):  
Satoshi Asaoka ◽  
Hideo Okamura ◽  
Kyunghoi Kim ◽  
Yuzuru Hatanaka ◽  
Kenji Nakamoto ◽  
...  

2021 ◽  
Vol 406 ◽  
pp. 124780
Author(s):  
Satoshi Asaoka ◽  
Kohei Kawakami ◽  
Hiroyuki Saito ◽  
Tsuyoshi Ichinari ◽  
Hideaki Nohara ◽  
...  

2017 ◽  
Vol 29 (8) ◽  
pp. 313-321
Author(s):  
Rimvydas Kaminskas ◽  
Vytautas Cesnauskas ◽  
Raimonda Kubiliute

Minerals ◽  
2018 ◽  
Vol 8 (11) ◽  
pp. 493 ◽  
Author(s):  
Farrah Hanum ◽  
Erda Desfitri ◽  
Yukio Hayakawa ◽  
Shinji Kambara

The application of paper sludge ash as an additive in controlling the leaching of trace elements has been satisfactorily effective to date. Previous studies have found that paper sludge ash has a promising effect in controlling the leaching of arsenic, selenium and boron. The content of calcium oxide in paper sludge ash is believed to be one of the important factors in decreasing the concentration of trace elements in leachate. Therefore, this study aimed to verify the effect of paper sludge ash in the leaching process and to propose an effective and applicable suppressing material that can control the leaching of As, Se, B and F simultaneously. In light of this aim, Ca(OH)2, PS ash 8 and blast furnace cement (BF cement) were tested as single and mixed additives in two different coal fly ashes (FA C and FA H). The results indicate that the application of a mixture of additives is necessary to control the leaching of trace elements. A mixture of PS ash 8, Ca(OH)2 and blast furnace cement (BF cement) was proposed to be an applicable and suitable additive that could suppress arsenic, selenium, boron, and fluorine leaching simultaneously.


2017 ◽  
Vol 464 ◽  
pp. 76-83 ◽  
Author(s):  
Weiling Sun ◽  
Jay E. Renew ◽  
Wenlong Zhang ◽  
Yuanzhi Tang ◽  
Ching-Hua Huang

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