Influence of CO2 Nucleation Rate Towards Cryogenic Separation Technologies in Bulk CO2 Separation from Natural Gas

Author(s):  
A.A. Md Jalil ◽  
K. Rostani ◽  
R. Ahmad Samawe ◽  
N.A. Othman ◽  
M.A. Esa
2014 ◽  
Author(s):  
A.A. Md Jalil ◽  
K. Rostani ◽  
R. Ahmad Samawe ◽  
N.A. Othman ◽  
M.A. Esa

Author(s):  
Stéphanie Hoffmann ◽  
Michael Bartlett ◽  
Matthias Finkenrath ◽  
Andrei Evulet ◽  
Tord Peter Ursin

This paper presents the results of an evaluation of advanced combined cycle gas turbine plants with precombustion capture of CO2 from natural gas. In particular, the designs are carried out with the objectives of high efficiency, low capital cost, and low emissions of carbon dioxide to the atmosphere. The novel cycles introduced in this paper are comprised of a high-pressure syngas generation island, in which an air-blown partial oxidation reformer is used to generate syngas from natural gas, and a power island, in which a CO2-lean syngas is burnt in a large frame machine. In order to reduce the efficiency penalty of natural gas reforming, a significant effort is spent evaluating and optimizing alternatives to recover the heat released during the process. CO2 is removed from the shifted syngas using either CO2 absorbing solvents or a CO2 membrane. CO2 separation membranes, in particular, have the potential for considerable cost or energy savings compared with conventional solvent-based separation and benefit from the high-pressure level of the syngas generation island. A feasibility analysis and a cycle performance evaluation are carried out for large frame gas turbines such as the 9FB. Both short-term and long-term solutions have been investigated. An analysis of the cost of CO2 avoided is presented, including an evaluation of the cost of modifying the combined cycle due to CO2 separation. The paper describes a power plant reaching the performance targets of 50% net cycle efficiency and 80% CO2 capture, as well as the cost target of 30$ per ton of CO2 avoided (2006 Q1 basis). This paper indicates a development path to this power plant that minimizes technical risks by incremental implementation of new technology.


2011 ◽  
Vol 369 (1-2) ◽  
pp. 490-498 ◽  
Author(s):  
Imona C. Omole ◽  
Dhaval A. Bhandari ◽  
Stephen J. Miller ◽  
William J. Koros

Fuel ◽  
2014 ◽  
Vol 122 ◽  
pp. 206-217 ◽  
Author(s):  
Marvin Ricaurte ◽  
Christophe Dicharry ◽  
Xavier Renaud ◽  
Jean-Philippe Torré

2019 ◽  
Vol 21 (39) ◽  
pp. 21685-21688 ◽  
Author(s):  
Kwanghee Jeong ◽  
Peter J. Metaxas ◽  
Joel Chan ◽  
Temiloluwa O. Kuteyi ◽  
Zachary M. Aman ◽  
...  

We present the first quantitative measurements of hydrate formation probability, nucleation rate and growth on a water droplet suspended within a high pressure natural gas by acoustic levitation.


2018 ◽  
Vol 54 (90) ◽  
pp. 12671-12685 ◽  
Author(s):  
Hongshuai Gao ◽  
Lu Bai ◽  
Jiuli Han ◽  
Bingbing Yang ◽  
Suojiang Zhang ◽  
...  

It is imperative to develop efficient, reversible and economic technologies for separating CO2 which mainly comes from flue gas, natural gas and syngas.


Author(s):  
Maurizio Spinelli ◽  
Stefano Campanari ◽  
Stefano Consonni ◽  
Matteo C. Romano ◽  
Thomas Kreutz ◽  
...  

The state-of-the-art conventional technology for postcombustion capture of CO2 from fossil-fueled power plants is based on chemical solvents, which requires substantial energy consumption for regeneration. A promising alternative, available in the near future, is the application of molten carbonate fuel cells (MCFC) for CO2 separation from postcombustion flue gases. Previous studies related to this technology showed both high efficiency and high carbon capture rates, especially when the fuel cell is thermally integrated in the flue gas path of a natural gas-fired combined cycle or an integrated gasification combined cycle plant. This work compares the application of MCFC-based CO2 separation process to pulverized coal fired steam cycles (PCC) and natural gas combined cycles (NGCC) as a “retrofit” to the original power plant. Mass and energy balances are calculated through detailed models for both power plants, with fuel cell behavior simulated using a 0D model calibrated against manufacturers' specifications and based on experimental measurements, specifically carried out to support this study. The resulting analysis includes a comparison of the energy efficiency and CO2 separation efficiency as well as an economic comparison of the cost of CO2 avoided (CCA) under several economic scenarios. The proposed configurations reveal promising performance, exhibiting very competitive efficiency and economic metrics in comparison with conventional CO2 capture technologies. Application as a MCFC retrofit yields a very limited (<3%) decrease in efficiency for both power plants (PCC and NGCC), a strong reduction (>80%) in CO2 emission and a competitive cost for CO2 avoided (25–40 €/ton).


2014 ◽  
Author(s):  
R. Ahmad Samawe ◽  
K. Rostani ◽  
A. Mohd Jalil ◽  
M. Esa ◽  
N. Othman

Author(s):  
Maurizio Spinelli ◽  
Stefano Campanari ◽  
Matteo C. Romano ◽  
Stefano Consonni ◽  
Thomas G. Kreutz ◽  
...  

The state-of-the-art conventional technology for post combustion capture of CO2 from fossil-fuelled power plants is based on chemical solvents, which requires substantial energy consumption for regeneration. Apromising alternative, available in the near future, is the application of Molten Carbonate Fuel Cells (MCFC) for CO2 separation from post-combustion flue gases. Previous studies related to this technology showed both high efficiency and high carbon capture rates, especially when the fuel cell is thermally integrated in the flue gas path of a natural gas-fired combined cycle or an integrated gasification combined cycle plant. This work compares the application of MCFC based CO2 separation process to pulverized coal fired steam cycles (PCC) and natural gas combined cycles (NGCC) as a ‘retrofit’ to the original power plant. Mass and energy balances are calculated through detailed models for both power plants, with fuel cell behaviour simulated using a 0D model calibrated against manufacturers’ specifications and based on experimental measurements, specifically carried out to support this study. The resulting analysis includes a comparison of the energy efficiency and CO2 separation efficiency as well as an economic comparison of the cost of CO2 avoided under several economic scenarios. The proposed configurations reveal promising performance, exhibiting very competitive efficiency and economic metrics in comparison with conventional CO2 capture technologies. Application as a MCFC retrofit yields a very limited (<3%) decrease in efficiency for both power plants (PCC and NGCC), a strong reduction (>80%) in CO2 emission and a competitive cost for CO2 avoided (25–40 €/ton).


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