German Nuclear High-Level Waste Program - Key Research Areas

1985 ◽  
Vol 50 ◽  
Author(s):  
Helmut Geipel

AbstractBased on more than 10 years of research and development, vitrification and high level waste disposal have reached the status of demonstration projects in the Federal Republic of Germany: hot operation of the PAMELA vitrification plant is scheduled for october 1985, and a disposal test with 30 canisters of high active glass is being prepared in the ASSE salt mine. Safety studies for a model repository led to a good understanding of the relevant phenomena; they will continue using sitespezific parameters. Modelling and computer codes will be further developed in international cooperation. In addition to reprocessing, the technology for direct disposal of spent fuel will be developed and demonstrated in the next years.

1997 ◽  
Vol 506 ◽  
Author(s):  
J.W. Schneider ◽  
P. Zuidema ◽  
P.A. Smith ◽  
P. Gribi ◽  
M. Hugi ◽  
...  

This paper discusses the results of post-closure safety studies for two different waste streams that, according to current Swiss waste-management concepts, may be co-disposed in a single deep geological repository. The waste streams are:• directly disposed spent UO2 and mixed-oxide (MOX) fuel• vitrified high-level waste from the reprocessing of spent fuelThe inventories are based on a consideration of the anticipated arisings from nuclear power generation in Switzerland. A part (at least) of these arisings will be reprocessed, with the resultant vitrified high-level waste and long-lived intermediate-level waste returned to Switzerland. The Swiss electricity utilities have placed contracts with BNFL (UK) and COGEMA (France) for the reprocessing of about one third of the total arisings of spent fuel from nuclear power generation, assuming an electricity production scenario of 120 GWa(e). The decision as to whether to reprocess the remainder is currently left open, implying that up to two thirds of the arisings could be in the form of unreprocessed spent fuel for direct disposal. For the purposes of the present study, however, it is assumed that the arisings from the full 120 GWa scenario will be either directly disposed or reprocessed.


Author(s):  
Sidik Permana ◽  
Mitsutoshi Suzuki

The embodied challenges for introducing closed fuel cycle are utilizing advanced fuel reprocessing and fabrication facilities as well as nuclear nonproliferation aspect. Optimization target of advanced reactor design should be maintained properly to obtain high performance of safety, fuel breeding and reducing some long-lived and high level radioactivity of spent fuel by closed fuel cycle options. In this paper, the contribution of loading trans-uranium to the core performance, fuel production, and reduction of minor actinide in high level waste (HLW) have been investigated during reactor operation of large fast breeder reactor (FBR). Excess reactivity can be reduced by loading some minor actinide in the core which affect to the increase of fuel breeding capability, however, some small reduction values of breeding capability are obtained when minor actinides are loaded in the blanket regions. As a total composition, MA compositions are reduced by increasing operation time. Relatively smaller reduction value was obtained at end of operation by blanket regions (9%) than core regions (15%). In addition, adopting closed cycle of MA obtains better intrinsic aspect of nuclear nonproliferation based on the increase of even mass plutonium in the isotopic plutonium composition.


1986 ◽  
Vol 84 ◽  
Author(s):  
V. M. Oversby

AbstractPerformance assessment calculations are required for high level waste repositories for a period of 10,000 years under NRC and EPA regulations. In addition, the Siting Guidelines (IOCFR960) require a comparison of sites following site characterization and prior to final site selection to be made over a 100,000 year period. In order to perform the required calculations, a detailed knowledge of the physical and chemical processes that affect waste form performance will be needed for each site. While bounding calculations might be sufficient to show compliance with the requirements of IOCFR60 and 40CFRI91, the site comparison for 100,000 years will need to be based on expected performance under site specific conditions. The only case where detailed knowledge of waste form characteristics in the repository would not be needed would be where radionuclide travel times to the accessible environment can be shown to exceed 100,000 years. This paper will review the factors that affect the release of radionuclides from spemt fuel under repository conditions, summarize our present state of knowledge, and suggest areas where more work is needed in order to support the performance assessment calculations.


2019 ◽  
Vol 482 (1) ◽  
pp. 205-212 ◽  
Author(s):  
T. Ishii ◽  
M. Kawakubo ◽  
H. Asano ◽  
I. Kobayashi ◽  
P. Sellin ◽  
...  

AbstractBentonite-based buffer materials play an important safety role in engineered barriers planned for use in geological disposal repositories for radioactive high-level waste (HLW) in Japan. The effectiveness of buffer materials is dependent on the status of groundwater saturation during resaturation of the repository. Accordingly, it is important to determine the behaviour of buffer materials during saturation and predict post-saturation conditions such as the distribution of residual dry density and chemical alteration.In this study, the rate of groundwater uptake into a buffer material was determined to clarify the behaviour of the material during the saturation process. As mechanical changes and chemical alteration of buffer materials are generated by groundwater permeation, knowledge of the water uptake rate is necessary for the prediction of post-permeation conditions. In the experiment reported here, one-dimensional permeation by distilled water and a NaCl water solution at a constant rate was monitored over a period of more than seven years. The results indicated that the seepage and saturation front moved in proportion to the square root of the seepage time. The coefficient of the relationships between the seepage and the saturation fronts with time of the reference bentonite used in Japan was determined.


2003 ◽  
Vol 807 ◽  
Author(s):  
Paul Wersin ◽  
Lawrence H. Johnson ◽  
Bernhard Schwyn

ABSTRACTRedox conditions were assessed for a spent fuel and high-level waste (SF/HLW) and an intermediate-level waste (ILW) repository. For both cases our analysis indicates permanently reducing conditions after a relatively short oxic period. The canister-bentonite near field in the HLW case displays a high redox buffering capacity because of expected high activity of dissolved and surface-bound Fe(II). This is contrary to the cementitious near field in the ILW case where concentrations of dissolved reduced species are low and redox reactions occur primarily via solid phase transformation processes.For the bentonite-canister near field, redox potentials of about -100 to -300 mV (SHE) are estimated, which is supported by recent kinetic data on U, Tc and Se interaction with reduced iron systems. For the cementitious near field, redox potentials of about -200 to -800 mV are estimated, which reflects the large uncertainties related to this alkaline environment.


Author(s):  
Richard E. Andrews

Abstract Sweden has chosen to manage spent fuel rods by direct encapsulation and storage in a deep level repository. Two welding processes are being investigated for the sealing of copper vessels that form the outer barrier of the disposal canisters. TWI Ltd in the UK has developed Reduced Pressure Electron Beam Welding and Friction Stir Welding for 50mm thick copper. This paper describes some of the investigations and compares the techniques. Over the past 3 years a full-size canister welding machine has been designed and built. Specialised tools have been developed for the welding of thick sections in copper with very encouraging results.


Author(s):  
H. Geiser ◽  
J. Schro¨der

The idea of using casks for interim storage of spent fuel arose at GNS after a very controversial political discussion in 1978, when total passive safety features (including aircraft crash conditions) were required for an above ground spent fuel storage facility. In the meantime, GNS has loaded more than 1000 casks at 25 different storage sites in Germany. GNS cask technology is used in 13 countries. Spent fuel assemblies of PWR, BWR, VVER, RBMK, MTR and THTR as well as vitrified high level waste containers are stored in full metal casks of the CASTOR® type. Also MOX fuel of PWR and BWR has been stored. More than two decades of storage have shown that the basic requirements (safe confinement, criticality safety, sufficient shielding and appropriate heat transfer) have been fulfilled in any case — during normal operation and in case of severe accidents, including aircraft crash. There is no indication of problems arising in the future. Of course, the experience of more than 20 years has resulted in improvements of the cask design. The CASTOR® casks have been thoroughly investigated by many experiments. There have been approx. 50 full and half scale drop tests and a significant number of fire tests, simulations of aircraft crash, investigations with anti tank weapons, and an explosion of a railway tank with liquid gas neighbouring a loaded CASTOR® cask. According to customer and site specific demands, different types of storage facilities are realized in Germany. Firstly, there are facilities for long-term storage, such as large ventilated central storage buildings away from reactor or ventilated storage buildings at the reactor site, ventilated underground tunnels or concrete platforms outside a building. Secondly, there are facilities for temporary storage, where casks have been positioned in horizontal orientation under a ventilated shielding cover outside a building.


1997 ◽  
Vol 506 ◽  
Author(s):  
V. M. Oversby

ABSTRACTThe conditions that are needed to achieve criticality in a high level waste repository for spent nuclear reactor fuel are reviewed. The effect of initial enrichment of the fuel, burnup, and of mixed oxide fuels on the conditions for criticality are discussed. The situations that produced criticality at Oklo, Gabon, 2000 million years ago are summarized. A model based on the Oklo conditions is presented for estimating the amount of fissile material that must be assembled to create a critical mass in typical granitic rocks. Mechanisms for movement of uranium and plutonium to achieve a critical configuration are discussed and compared to the conditions that are likely to occur in a repository in granite. The sequences of events needed to produce a critical assemblage are shown to be in conflict with the conditions expected in the repository and, in some cases, to require internally inconsistent assumptions to produce the postulated sequence of events. No credible scenario for achieving criticality in a high level waste repository has been found.


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