Studies on radionuclide transport behaviour–The next generation of in-situ experiments at the Grimsel Test Site

2009 ◽  
Vol 1193 ◽  
Author(s):  
Andrew James Martin ◽  
Ingo Blechschmidt
Keyword(s):  
Shear Zone ◽  
Diffusion Processes ◽  
Test Site ◽  
Core Material ◽  
Laboratory Studies ◽  
Grimsel Test Site ◽  
And Migration ◽  
Colloid Formation

AbstractTwo recent ongoing major projects at the Grimsel Test Site (GTS) (www.grimsel.com) that were initiated to simulate the long-term behaviour of radionuclides in the repository near-field and the surrounding host rock are presented: the Colloid Formation and Migration (CFM) project, which focuses on colloid generation and migration from a bentonite source doped with radionuclides and the Long-Term Diffusion (LTD) project, which aims at in-situ verification and understanding of the processes that control the long-term diffusion of repository-relevant radionuclides. So far, the CFM project has principally involved: development and implementation of a state-of-the-art sealing concept to control hydraulic gradients in a shear zone to imitate repository-relevant conditions; extensive laboratory studies to examine bentonite erosion and colloid formation in a shear zone; and, development of models to estimate colloid formation and migration. The next stage will be to assess the behavior of bentonite colloids generated from a radionuclide spiked bentonite source-term emplaced into the controlled flow field of the shear zone. This will be coupled with further extensive laboratory studies in order to refine and evaluate the colloid models currently used in performance assessments. The LTD project consists of: a monopole diffusion experiment where weakly sorbing and non-sorbing radionuclides (3H, 22Na, 131I, 134Cs) have been circulating and diffusing into undisturbed rock matrix since June 2007; experiments to characterise pore space geometry, including determination of in-situ porosity with 14C doped MMA resin for comparison with laboratory derived data; a study of natural tracers to elucidate evidence of long-term diffusion processes; and, an investigation of the in-situ matrix diffusion paths in core material from earlier GTS experiments. Future experiments will focus on diffusion processes starting from a water-conducting feature under realistic boundary conditions.

Grimsel Test Site - Phase VI: Review of Accomplishments and Next Generation of In-Situ Experiments Under Repository Relevant Boundary Conditions

2008 ◽  
Vol 1107 ◽  
Author(s):  
Ingo Blechschmidt ◽  
Stratis Vomvoris ◽  
Joerg Rueedi ◽  
Andrew James Martin
Keyword(s):  
Near Field ◽  
Planning Horizon ◽  
Test Site ◽  
Low Ph ◽  
Swiss Alps ◽  
In Situ Experiments ◽  
Grimsel Test Site ◽  
And Migration

AbstractThe Grimsel Test Site owned and operated by Nagra is located in the Swiss Alps (www.grimsel.com). The Sixth Phase of investigations was started in 2003 with a ten-year planning horizon. With the investigations and projects of Phase VI the focus has shifted more towards projects assessing perturbation effects of repository implementation and projects evaluating and demonstrating engineering and operational aspects of the repository system. More than 17 international partners participate in the various projects, which form the basic organisational “elements” of Phase VI. Scientific and engineering interaction among the different projects is ensured via an annual meeting and several experimental team meetings throughout the year. On-going projects include: evaluation of full-scale engineered systems under simulated heat production and long-term natural saturation (NF-Pro/FEBEX), gas migration through engineered barrier systems (GMT, finished this year), emplacement of a shotcrete low-pH plug (ESDRED/Module IV), testing and evaluation of standard monitoring techniques (TEM).Numerous in-situ experiments with inactive tracers and radionuclides were successfully carried out over the past few years at the Grimsel Test Site (GTS). For the GTS Phase VI, three major projects have been initiated to simulate the long-term behaviour of contamination plumes in the repository near-field and the surrounding host rock:•The CFM (Colloid Formation and Migration) project, which focuses on colloid generation and migration from a bentonite source doped with radionuclides•The LCS (Long-Term Cement Studies) project, which aims at improving the understanding of low-pH cement interaction effects in water conducting features•The LTD (Long-Term Diffusion) project, which aims at in-situ verification of long-term diffusion concepts for radionuclidesAs Phase VI approaches its mid-term point, what are the next steps planned? The accomplishments assessed to date and the opportunities with the on-going projects as well as new projects – currently under discussion – are presented herein

Modeling of an in-situ diffusion experiment in granite at the Grimsel Test Site

2014 ◽  
Vol 1665 ◽  
pp. 85-91 ◽  
Author(s):  
Josep M. Soler ◽  
Jiri Landa ◽  
Vaclava Havlova ◽  
Yukio Tachi ◽  
Takanori Ebina ◽  
...  
Keyword(s):  
Effective Diffusion ◽  
Test Site ◽  
Diffusion Experiment ◽  
Bulk Rock ◽  
Disturbed Zone ◽  
Mean Grain Size ◽  
Grimsel Test Site ◽  
In Situ Diffusion

ABSTRACTMatrix diffusion is a key process for radionuclide retention in crystalline rocks. Within the LTD project (Long-Term Diffusion), an in-situ diffusion experiment in unaltered non-fractured granite was performed at the Grimsel Test Site (www.grimsel.com, Switzerland). The tracers included 3H as HTO, 22Na+, 134Cs+ and 131I- with stable I- as carrier.The dataset (except for 131I- because of complete decay) was analyzed with different diffusion-sorption models by different teams (NAGRA / IDAEA-CSIC, UJV-Rez, JAEA, Univ. Poitiers) using different codes, with the goal of obtaining effective diffusion coefficients (De) and porosity (ϕ) or rock capacity (α) values. A Borehole Disturbed Zone (BDZ), which was observed in the rock profile data for 22Na+ and 134Cs+, had to be taken into account to fit the experimental observations. The extension of the BDZ (1-2 mm) was about the same magnitude as the mean grain size of the quartz and feldspar grains.De and α values for the different tracers in the BDZ are larger than the respective values in the bulk rock. Capacity factors in the bulk rock are largest for Cs+ (strong sorption) and smallest for 3H (no sorption). However, 3H seems to display large α values in the BDZ. This phenomenon will be investigated in more detail in a second test starting in 2013.

The Excavation Project in the Grimsel Test Site: In Situ High-Resolution Gamma and Alpha Spectrometry of 60Co, 75Se, 113Sn, 152Eu, 235U, and 237Np/233Pa

1997 ◽  
Vol 506 ◽  
Author(s):  
J. Eikenberg ◽  
M. Ruethi ◽  
W.R. Alexander ◽  
B. Frieg ◽  
T. Fierz
Keyword(s):  
High Resolution ◽  
Shear Zone ◽  
Test Site ◽  
Breakthrough Curves ◽  
Laboratory Measurements ◽  
Radionuclide Migration ◽  
Grimsel Test Site ◽  
On Line ◽  
Comprehensive Study

ABSTRACTFull excavation of a water-conducting shear zone used for radionuclide migration experiments is part of a comprehensive study to physically determine the sites of in-situ radionuclide retardation. Prior to the excavation, multi-tracer solutions containing strongly sorbing y- and αemitting nuclides were injected into the shear zone and the water extracted was analyzed on-line using in situ, high-resolution y-spectrometry. In addition, water samples were collected to compare quantitatively the on-line data with subsequent laboratory measurements α- and γ- spectrometry) and also to analyze samples with activities below the detection limits of the in-situ analysis. The breakthrough curves indicate that Se had passed through the fracture with a velocity comparable to a conservatively behaving dye (uranine), but very strong retardation of Co. Eu and Sn was observed. The recoveries of these nuclides were found to be in the order of only a few percent when the dipole flow-field was interrupted about one month after radionuclide injection and the fracture was sealed off for excavation. Significant retardation was also obtained for the oxemitters U, Np and Pa. Almost identical breakthrough curves for these actinides were measured, suggesting a similar spatial distribution in the fracture at any given time.

Radionuclide geochemistry evolution in the Long-term In-situ Test (LIT) at Grimsel Test Site (Switzerland)

2021 ◽  
pp. 127733
Author(s):  
Vanessa Montoya ◽  
Ulrich Noseck ◽  
Felix Mattick ◽  
Susan Britz ◽  
Ingo Blechschmidt ◽  
...  
Keyword(s):  
Test Site ◽  
In Situ Test ◽  
Grimsel Test Site

Grimsel Test Site — Phase VI: Review of Accomplishments and Next Steps

2007 ◽  
Author(s):  
Stratis Vomvoris ◽  
Wolfgang Kickmaier
Keyword(s):  
Ad Hoc ◽  
Field Testing ◽  
Planning Horizon ◽  
Test Site ◽  
Swiss Alps ◽  
Tracer Transport ◽  
Geophysical Investigation ◽  
Grimsel Test Site

The Grimsel Test Site owned and operated by Nagra is located in the Swiss Alps (www.grimsel.com). The sixth Phase of investigations was started in 2003 with a ten-year planning horizon. With the investigations and projects of Phase VI the focus is shifted more towards projects assessing perturbation effects of repository implementation and projects evaluating and demonstrating engineering and operational aspects of the repository system. More than 17 international partners participate in the various projects, which form the basic organisational ‘elements’ of Phase VI, each one further structured in field-testing, laboratory studies, design and modelling tasks, as appropriate. Each project phase is planned with a duration of 3 to 5 years, to facilitate all practical and administrative aspects, ensuring flexibility for updating the overall plan with the recent findings. Scientific and engineering interaction among the different projects is ensured via the annual international meeting and ad-hoc meetings, as appropriate. As Phase VI approaches its mid-term point, a review of the accomplishments to date is performed to provide a sound basis for the detailed planning of the next steps. The accomplishments to date are described and assessed below; the opportunities with the on-going projects as well as new projects – currently under discussion – are also presented and discussed. The on-going projects include: studies of the long-term diffusion with emphasis on the processes in the rock matrix (LTD); colloid studies under in-situ generation conditions and migration velocities closer to velocities expected in an actual repository site (CFM); studies of the long-term cement interactions with natural systems (LCS); evaluation of full-scale engineered systems under simulated heat production and long-term natural saturation (NF-Pro/FEBEX); gas migration through engineered barrier systems (GMT); emplacement of shotcrete low-pH plug (ESDRED/Module IV); test and evaluation of monitoring systems (TEM). In addition, various shorter term projects assessing, for example, new geophysical investigation tools, wireless transmission, testing new tools and training for in-situ tracer transport studies have been performed and/or are planned for the near future.

scholarly journals The seismo-hydro-mechanical behaviour during deep geothermal reservoir stimulations: open questions tackled in a decameter-scale in-situ stimulation experiment

2017 ◽  
Author(s):  
Florian Amann ◽  
Valentin Gischig ◽  
Keith Evans ◽  
Joseph Doetsch ◽  
Reza Jalali ◽  
...  
Keyword(s):  
Rock Mass ◽  
Geothermal Energy ◽  
Numerical Models ◽  
Test Site ◽  
Crystalline Rock ◽  
Coupled Processes ◽  
Small Scale ◽  
Intermediate Scale ◽  
Grimsel Test Site

Abstract. In this contribution we present a review of scientific research results that address seismo-hydro-mechanical coupled processes relevant for the development of a sustainable heat exchanger in low permeability crystalline rock and introduce the design of the In-situ Stimulation and Circulation (ISC) experiment at the Grimsel Test Site dedicated to study such processes under controlled conditions. The review shows that research on reservoir stimulation for deep geothermal energy exploitation has been largely based on laboratory observations, large-scale projects and numerical models. Observations of full-scale reservoir stimulations have yielded important results. However, the limited access to the reservoir and limitations in the control on the experimental conditions during deep reservoir stimulations is insufficient to resolve the details of the hydro-mechanical processes that would enhance process understanding in a way that aids future stimulation design. Small scale laboratory experiments provide a fundamental insights into various processes relevant for enhanced geothermal energy, but suffer from 1) difficulties and uncertainties in upscaling the results to the field-scale and 2) relatively homogeneous material and stress conditions that lead to an over-simplistic fracture flow and/or hydraulic fracture propagation behaviour that is not representative for a heterogeneous reservoir. Thus, there is a need for intermediate-scale hydraulic stimulation experiments with high experimental control that bridge the various scales, and for which access to the target rock mass with a comprehensive monitoring system is possible. Only few intermediate-scale hydro-shearing and hydro-fracturing experiments have recently been performed in a densely instrumented rock mass. No such measurements have been performed on faults in crystalline basement rocks. The In-situ Stimulation and Circulation (ISC) experiment currently performed in a naturally fractured and faulted crystalline rock mass at the Grimsel Test Site (Switzerland) is designed to address open research questions, which could not be investigated in the required detail so far. Two hydraulic injection phases were executed to enhance the permeability of the rock mass: a hydro-shearing phase and then a hydraulic fracturing phase. During the injection phases the rock mass deformation across fractures and within intact rock, the pore pressure distribution and propagation and the micro-seismic response were monitored at a high spatial and temporal resolution.

scholarly journals Eighteen years of steel–bentonite interaction in the FEBEX in situ test at the Grimsel Test Site in Switzerland

2019 ◽  
Vol 67 (2) ◽  
pp. 111-131 ◽  
Author(s):  
Jebril Hadi ◽  
Paul Wersin ◽  
Vincent Serneels ◽  
Jean-Marc Greneche
Keyword(s):  
Test Site ◽  
In Situ Test ◽  
Grimsel Test Site

scholarly journals Formation and In Situ Treatment of High Fluoride Concentrations in Shallow Groundwater of a Semi-Arid Region: Jiaolai Basin, China

2020 ◽  
Vol 17 (21) ◽  
pp. 8075
Author(s):  
Zongjun Gao ◽  
Mengjie Shi ◽  
Hongying Zhang ◽  
Jianguo Feng ◽  
Shaoyan Fang ◽  
...  
Keyword(s):  
Shallow Groundwater ◽  
Field Investigation ◽  
River Outflow ◽  
High Fluoride ◽  
Essential Nutrient ◽  
Semi Arid Region ◽  
And Migration ◽  
Soil Fluoride

Fluorine is an essential nutrient, and excessive or deficient fluoride contents in water can be harmful to human health. The shallow groundwater of the Jiaolai Basin, China has a high fluoride content. This study aimed to (1) investigate the processes responsible for the formation of shallow high-fluoride groundwater (SHFGW); (2) identify appropriate methods for in situ treatment of SHFGW. A field investigation into the formation of SHFGW was conducted, and the results of experiments using soils from high-fluoride areas were examined to investigate the leaching and migration of fluoride. The results showed that the formation of SHFGW in the Jiaolai Basin is due to long-term geological and evaporation processes in the region. Stratums around and inside the basin act as the source of fluoride whereas the terrain promotes groundwater convergence. The hydrodynamic and hydrochemical conditions resulting from slow groundwater flow along with high evaporation and low rainfall all contribute to the enrichment of fluoride in groundwater. In situ treatment of SHFGW may be an effective approach to manage high SHFGW in the Jiaolai Basin. Since soil fluoride in high-fluoride areas can leach into groundwater and migrate with runoff, the construction of ditches can shorten the runoff of shallow groundwater and accelerate groundwater loss, resulting in the loss of SHFGW from high-fluoride areas through river outflow. The groundwater level will be reduced, thereby lowering the influence of evaporation on fluoride enrichment in shallow groundwater. The results of this study can act a reference for further research on in situ treatment for high-fluoride groundwater.

Microbial transformation of PCBs in sediments: what can we learn to solve practical problems?

1995 ◽  
Vol 31 (8) ◽  
pp. 99-107 ◽  
Author(s):  
Paul B. M. Stortelder ◽  
Jacobus E. M. Beurskens
Keyword(s):  
Sediment Quality ◽  
Microbial Transformation ◽  
Environmental Policies ◽  
Rhine River ◽  
Laboratory Studies ◽  
Complete Elimination ◽  
Anaerobic Consortium ◽  
Sediment Layers

The disappearance of several polychlorinated biphenyls (PCBs) was observed in the deeper anaerobic sediment layers of Lake Ketelmeer, a sedimentation area of the Rhine River. Laboratory studies with an anaerobic consortium from this area demonstrated the capabilities for transforming PCBs. The field and laboratory observations indicate that disappearances of PCBs in the sediment might be caused by in situ microbial dechlorination. These processes appear to have lowered the PCB toxicity of four reactive congeners by 75% during the last two decades. In addition, dechlorination reactions are the essential first steps in the only natural pathway that eventually may lead to a complete elimination of PCBs from the aquatic environment. This can only be achieved if the dechlorination products are subsequently mineralized under aerobic conditions. Several implications for environmental policies with regard to contaminated sediments are discussed. Long-term prognoses on sediment quality generated with mathematical models that include these reactions may lead to a distinct, probably less costly, sediment policy.

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