Analysis Of Congruent Matrix Release, Precipitation, And Time-Distributed Containment Failure On Spent Fuel Performance

1987 ◽  
Vol 112 ◽  
Author(s):  
Michael J. Apted ◽  
David W. Engel
Keyword(s):  
Source Term ◽  
Spent Fuel ◽  
Release Rates ◽  
Waste Package ◽  
Regulatory Limits ◽  
Lower Solubility ◽  
Fractional Abundance ◽  
Congruent Dissolution ◽  
Cesium 137 ◽  
Term Evaluation

AbstractThe Analytical Repository Source-Term (AREST) code has been developed for source-term evaluation of spent fuel as a final waste form in geologic repositories. AREST contains a set of analytical equations for the timedependent diffusional mass transport of both solubility-limited and inventory-limited radionuclides from a spent fuel in a failed container surrounded by a shell of packing or other porous material imbedded in a porous host rock. Three factors that affect release performance are examined: 1) congruent dissolution of the UO2 matrix, 2) chemical instability of the UO2 matrix, with precipitation of a more stable uranium phase within the waste package, and 3) the attenuation of release rate by distribution of containment failures with time.For congruent matrix dissolution, the release rates of included nuclides are proportional to the product of solubility-limited release of uranium and the fractional abundance of the nuclide. For certain conditions, congruent release rates are calculated to be up to 10 orders of magnitude lower than release rates assuming individual solubility-limits. Precipitation of a more stable, lower solubility uranium phase within the waste package is shown to increase release rates from the UO2 matrix compared to the non-precipitation case, in agreement with previous calculations. During the first 300 to 1000 years after repository closure, the distribution of containment failures with time will act to attenuate the peak average release rates of soluble, longlived nuclides, such as iodine-129, to values smaller than release rates below regulatory limits. However, for soluble nuclides with short half-lives, such as cesium-137, a broader distribution of containment failure with constant mean time of failure can actually cause an increase In the peak average release rates.

Source-Term Comparison Using the Arest and Syvac-Vault Models: Effects of Decay-Chain In-Growth and Precipitation

1988 ◽  
Vol 127 ◽  
Author(s):  
M. J. Apted ◽  
D. W. Engel ◽  
N. C. Garisto ◽  
D. M. Leneveu
Keyword(s):  
Boundary Conditions ◽  
Source Term ◽  
Spent Nuclear Fuel ◽  
Decay Chain ◽  
Release Rates ◽  
Waste Package ◽  
Uranium Series ◽  
Enhancement Factors ◽  
Radionuclide Release ◽  
Good Agreement

ABSTRACTA series of calculations of radionuclide release was performed with the AREST and SYVAC-Vault models (SVM) in order to assess concurrance. Specifically, the effects of precipitation and decay chain in-growth on the predicted release of nuclides from waste packages containing spent nuclear fuel were compared between each code. The results for maximum release rates generally agreed within a factor of 10. The differences in results can be explained based on the differences in geometry and boundary conditions between the two codes. Both codes showed nearly identical enhancement factors in release rates of uranium-series nuclides (U-238, U-234, Th-230, Ra-226) arising from the effect of decay-chain in-growth. Calculated enhancement factors in release rates for precipitation of a new uranium-bearing solid within the waste package were also in good agreement between AREST and SVM.

The Effect of Waste Package Components on Radionuclides Released from Spent Fuel Under Hydrothermal Conditions

1987 ◽  
Vol 112 ◽  
Author(s):  
Shirley A. Rawson ◽  
William L. Neal ◽  
James R. Burnell
Keyword(s):  
Low Carbon Steel ◽  
Fission Products ◽  
Nuclear Waste Repository ◽  
Low Carbon ◽  
Spent Fuel ◽  
Hydrothermal Conditions ◽  
Waste Package ◽  
Dissolved Species ◽  
Radionuclide Release ◽  
Time Invariant

AbstractThe Basalt Waste Isolation Project has conducted a series of hydrothermal experiments to characterize waste/barrier/rock interactions as a part of its study of the Columbia River basalts as a potential medium for a nuclear waste repository. Hydrothermal tests of 3–15 months duration were performed with light water reactor spent fuel and simulated groundwater, in combination with candidate container materials (low-carbon steel or copper) and/or basalt, in order to evaluate the effect of waste package materials on spent fuel radionuclide release behavior. Solutions were filtered through 400 and 1.8 nm filters to distinguish colloidal from dissolved species. In all experiments, 14C, 129I, and 137Cs occurred only as dissolved species, whereas the actinides occurred in 400 nm filtrates primarily as spent fuel particles. Actinide concentrations in 1.8 nm filtrates were below detection in steel-bearing experiments. In the system spent fuel + copper, apparent time-invariant concentrations of 14C and 137Cs were obtained, but in the spent fuel + steel system, the concentrations of 14C and 137Cs increased gradually throughout the experiments. In experiments containing basalt or steel + basalt, 137Cs concentrations decreased with time. In tests with copper + basalt, 14C and 129I concentrations attained time-invariant values and 137Cs concentrations decreased. Concentrations for the actinides and fission products measured in these experiments were below those calculated from Federal regulations governing radionuclide release.

scholarly journals RADIONUCLIDE CHARACTERISTICS OF RDE SPENT FUELS

2018 ◽  
Vol 20 (2) ◽  
pp. 69 ◽  
Author(s):  
Ihda Husnayani ◽  
Pande Made Udiyani
Keyword(s):  
Thermal Power ◽  
Neutron Production ◽  
Cooling Time ◽  
Spent Fuel ◽  
Release Rates ◽  
Radiation Dose Rate ◽  
The Core ◽  
Spent Fuel Storage ◽  
Fuel Storage

Reaktor Daya Eksperimental (RDE) is a 10 MWth pebble-bed High Temperature Gas-cooled Reactor that is planned to be constructed by National Nuclear Energy Agency of Indonesia (BATAN) in Puspiptek complex, Tangerang Selatan. RDE utilizes low enriched UO2 fuel coated by TRISO layers and loaded into the core by means of multipass loading scheme. Determination of radionuclide characteristics of RDE spent fuel; such as activity, thermal power, neutron and photon release rates; are very important because those characteristics are crucial to be used as a base for evaluating the safety of spent fuel handling system and storage tank. This study is aimed to investigate the radionuclide characteristics of RDE spent fuel at the end of cycle and during the first 5 years cooling time in spent fuel storage. The method used to investigate the radionuclide characteristics is burnup calculation using ORIGEN2.1 code. In performing the ORIGEN2.1 calculation, one pebble fuel was assumed to be irradiated in the core for 5 cycles and then decayed for 5 years. At the end of the fifth cycle, it is obtained that the total activity, thermal power, neutron production, and photon release rates from all radionuclides inside one spent fuel are approximately 105.68 curies, 0.41 watts, 2.65 x 103 neutrons/second, and 1.79 x 104 photons/second, respectively. The results for the radionuclides characteristics during the first 5 years cooling time in the spent fuel storage show that the radioactivity characteristics from all radionuclides are rapidly decreasing at the first year and then slowly decreasing at the second until the fifth year of cooling time. The results obtained in this study can provide data for safety evaluation of fuel handling and spent fuel storage, such as the calculation of sourceterm, radiation dose rate, and the determination of radiation shielding.Keywords: RDE, spent fuel, radionuclide activity, thermal power, neutron production, photon releaserates KARAKTERISTIK RADIONUKLIDA DI DALAM BAHAN BAKAR RDE. Reaktor Daya Eksperimental (RDE) adalah reaktor tipe Reaktor Temperatur Tinggi Berpendingin Gas dengan daya termal 10MW yang akan dibangun oleh BadanTenagaNuklirNasional (BATAN) di kawasanPuspiptek, Tangerang Selatan. RDE menggunakan bahan bakar UO2 yang dilapisi dengan lapisan TRISO dan dimasukkan ke dalam teras RDE menurut skema multipass (5 siklus). Penentuan karakteristik radionuklida di dalam bahan bakar RDE; seperti aktivitas, daya termal, laju produksi neutron dan pelepasan foton; adalah sangat penting karena informasi karakteristik ini diperlukan sebagai dasar untuk melakukan evaluasi keselamatan system penanganan dan penyimpanan bahan bakar bekas. Penelitian ini bertujuan untuk menganalisis karakteristik radionuklida bahanbakar RDE setelah 5 siklus dan pada 5 tahun pertama pendinginan ditempat penyimpanan bahan bakar bekas. Metode yang digunakan dalam menghitung karakteristik radionuklida adalah menggunakan program ORIGEN2.1. Satu bola bahan bakar RDE diasumsikan diiradiasi selama 5 siklus dan kemudian meluruh selama 5 tahun. Pada akhir siklus, diperoleh hasil aktivitas total, daya termal, laju produksi neutron dan pelepasan foton dari seluruh radionuklida di dalam satu bola bahan bakar RDE sebesar 105,68 curies, 0,41 watts, 2,65 x 103 neutron/detik, dan 1,79 x 104 foton/detik. Hasil untuk karakteristik radionuklida selama 5 tahun penyimpanan menunjukkan bahwa karakteristik radioktivitas radionuklida menurun dengan cepat pada tahun pertama dan kemudian menurun lebih lambat pada tahun kedua hingga tahun kelima. Hasil perhitungan karakteristik radionuklida dari penelitian ini dapat digunakan sebagai basis untuk analisis keselamatan penanganan dan penyimpanan bahan bakarbekas RDE.Kata kunci:RDE, bahan bakar bekas, aktivitas radionuklida, daya termal, produksi neutron, laju foton

Evaluation of source term parameters for spent fuel disposal in foreign countries

2016 ◽  
Vol 23 (1) ◽  
pp. 31-54
Author(s):  
Masanobu NAGATA ◽  
Takahiro CHIKAZAWA ◽  
Kuniaki AKAHORI ◽  
Akira KITAMURA ◽  
Yukio TACHI
Keyword(s):  
Source Term ◽  
Spent Fuel ◽  
Foreign Countries
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