Nonlinear Optical Properties of Polyenes: Electron Correlation and Chain Conformation
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ABSTRACTUsing a recently developed many-electron theory of second and third order nonlinear optical susceptibilities, microscopic descriptions of γxxxx(-3ω;ω,ω,ω) are presented for two conformations of polyenes. The importance of electron correlations and the effects of variation in conformation and chain length are discussed.
2006 ◽
Vol 156
(2-4)
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pp. 154-161
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1988 ◽
Vol 160
(1)
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pp. 37-51
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2005 ◽
Vol 52
(14)
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pp. 1933-1945
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2014 ◽
Vol 57
(9)
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pp. 1235-1245
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