Contradictory Evidence for the Role of Temperature and Particle Size in Nanofluid Thermal Conductivity

2011 ◽  
Vol 1347 ◽  
Author(s):  
Rebecca J. Christianson ◽  
Jessica Townsend

ABSTRACTThe prospects for increased cooling capacity from the use of nanofluid coolants has created a tremendous amount of interest. However, in the years since the initial thermal conductivity measurements of nanoparticle suspensions were reported, there has been much inconsistency in data published in the literature. The International Nanofluids Benchmarking Exercise was a significant step towards creating a reliable set of data on the thermal conductivity enhancement of stable nanofluids, however there remain many unanswered questions. Most significant, perhaps, is the contradictory results on the effects of particle size and temperature. In the past year alone it is possible to find published reports on nominally identical samples claiming precisely opposing trends in thermal conductivity with decreasing particle size at room temperature. Some studies also claim an increasing enhancement at higher temperatures, sometimes linking this to small particle sizes. In this work we review the literature claims for particle size and temperature results, the theories used to support those claims, as well as presenting new data with the aim of resolving the dispute and identifying the origins of the evidence for contradictory claims.

Author(s):  
Calvin H. Li ◽  
G. P. Peterson

Experimental evidence exists that the addition of a small quantity of nanoparticles to a base fluid, can have a significant impact on the effective thermal conductivity of the resulting suspension. The causes for this are currently thought to be due to a combination of two distinct mechanisms. The first is due to the change in the thermophysical properties of the suspension, resulting from the difference in the thermal conductivity of the fluid and the particles, and the second is thought to be due to the transport of thermal energy by the particles, due to the Brownian motion of the particles. In order to better understand these phenomena, a theoretical model has been developed that examines the effect of the Brownian motion. In this model, the well-known approach first presented by Maxwell, is combined with a new expression that incorporates the effect of the Brownian motion and describes the physical phenomena that occurs because of it. The results indicate that the enhanced thermal conductivity may not in fact be due to the transport of energy by the particles, but rather, due to the stirring motion caused by the movement of the nanoparticles which enhances the heat transfer within the fluid. The resulting model shows good agreement when compared with the existing experimental data and perhaps more importantly helps to explain the trends observed from a fundamental physical perspective. In addition, it provides a possible explanation for the differences that have been observed between the previously obtained experimental data, the predictions obtained from Maxwell’s equation and the theoretical models developed by other investigators.


2006 ◽  
Vol 129 (3) ◽  
pp. 298-307 ◽  
Author(s):  
Sang Hyun Kim ◽  
Sun Rock Choi ◽  
Dongsik Kim

The thermal conductivity of water- and ethylene glycol-based nanofluids containing alumina, zinc-oxide, and titanium-dioxide nanoparticles is measured using the transient hot-wire method. Measurements are performed by varying the particle size and volume fraction, providing a set of consistent experimental data over a wide range of colloidal conditions. Emphasis is placed on the effect of the suspended particle size on the effective thermal conductivity. Also, the effect of laser-pulse irradiation, i.e., the particle size change by laser ablation, is examined for ZnO nanofluids. The results show that the thermal-conductivity enhancement ratio relative to the base fluid increases linearly with decreasing the particle size but no existing empirical or theoretical correlation can explain the behavior. It is also demonstrated that high-power laser irradiation can lead to substantial enhancement in the effective thermal conductivity although only a small fraction of the particles are fragmented.


Author(s):  
R.A. Youngman

It has been over thirty years since sintered aluminum nitride (AIN) has been the focus of many research and development activities in Japan, the U.S., and Europe. Only in the past 5 years has there been significant use of this material in microelectronics. There are many reasons for this considerable time for application including, technology needs and acceptance of a new material. Also important has been the role of materials understanding of AIN through the use of microscopy and spectroscopy. We illustrate the use of both standard and unique characterization techniques to elucidate the nature of the crystalline defects which control the important property of thermal conductivity.The thermal conductivity of pure AIN is 320 W/mK. This value has never been achieved in a sintered ceramic. In order to develop a sintered AIN with a high thermal conductivity it is necessary to understand the factors which control the thermal conductivity.


2011 ◽  
Vol 133 (4) ◽  
Author(s):  
Jing Fan ◽  
Liqiu Wang

Nanofluids—fluid suspensions of nanometer-sized particles—are a very important area of emerging technology and are playing an increasingly important role in the continuing advances of nanotechnology and biotechnology worldwide. They have enormously exciting potential applications and may revolutionize the field of heat transfer. This review is on the advances in our understanding of heat-conduction process in nanofluids. The emphasis centers on the thermal conductivity of nanofluids: its experimental data, proposed mechanisms responsible for its enhancement, and its predicting models. A relatively intensified effort has been made on determining thermal conductivity of nanofluids from experiments. While the detailed microstructure-conductivity relationship is still unknown, the data from these experiments have enabled some trends to be identified. Suggested microscopic reasons for the experimental finding of significant conductivity enhancement include the nanoparticle Brownian motion, the Brownian-motion-induced convection, the liquid layering at the liquid-particle interface, and the nanoparticle cluster/aggregate. Although there is a lack of agreement regarding the role of the first three effects, the last effect is generally accepted to be responsible for the reported conductivity enhancement. The available models of predicting conductivity of nanofluids all involve some empirical parameters that negate their predicting ability and application. The recently developed first-principles theory of thermal waves offers not only a macroscopic reason for experimental observations but also a model governing the microstructure-conductivity relationship without involving any empirical parameter.


Author(s):  
Sonya T. Smith ◽  
Mohsen Mosleh ◽  
Khosro A. Shirvani

Experimental and numerical investigations were conducted to explore the viability of single-phase nanofluids for microchannel cooling. The experiments were conducted with water/ethylene glycol-based nanofluids to investigate the thermal conductivity enhancement. In the numerical analysis, micro-channels ranged in width from 40 μm to 90 μm with the fixed channel height were considered. Thermal conductivity enhancements of nearly 14% at particle concentration of 0.1% by weight was observed in the experiments. Numerical predictions suggest that design variables (particle size and channel aspect ratio) and thermo-physical properties of the nanofluid have a significant effect on the thermal performance of micro-channel heat sinks. It was shown that at fixed Reynold number, reduction of channel width reduces the hydraulic pressure loss and the heat transfer coefficient, and utilizing nanofluids increases these parameters.


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