scholarly journals Fostering multidisciplinary research on interactions between chemistry, biology, and physics within the coupled cryosphere-atmosphere system

Elem Sci Anth ◽  
2019 ◽  
Vol 7 ◽  
Author(s):  
Jennie L. Thomas ◽  
Jochen Stutz ◽  
Markus M. Frey ◽  
Thorsten Bartels-Rausch ◽  
Katye Altieri ◽  
...  
Keyword(s):  
Atmospheric Chemistry ◽  
Global Climate ◽  
Atmospheric Composition ◽  
Multidisciplinary Research ◽  
Frozen Ground ◽  
Alpine Regions ◽  
Atmosphere System ◽  
Cryospheric Change ◽  
New Research ◽  
Atmospheric Inputs

The cryosphere, which comprises a large portion of Earth’s surface, is rapidly changing as a consequence of global climate change. Ice, snow, and frozen ground in the polar and alpine regions of the planet are known to directly impact atmospheric composition, which for example is observed in the large influence of ice and snow on polar boundary layer chemistry. Atmospheric inputs to the cryosphere, including aerosols, nutrients, and contaminants, are also changing in the anthropocene thus driving cryosphere-atmosphere feedbacks whose understanding is crucial for understanding future climate. Here, we present the Cryosphere and ATmospheric Chemistry initiative (CATCH) which is focused on developing new multidisciplinary research approaches studying interactions of chemistry, biology, and physics within the coupled cryosphere – atmosphere system and their sensitivity to environmental change. We identify four key science areas: (1) micro-scale processes in snow and ice, (2) the coupled cryosphere-atmosphere system, (3) cryospheric change and feedbacks, and (4) improved decisions and stakeholder engagement. To pursue these goals CATCH will foster an international, multidisciplinary research community, shed light on new research needs, support the acquisition of new knowledge, train the next generation of leading scientists, and establish interactions between the science community and society.

The Earth energy imbalance – new advances and remaining challenges

2021 ◽  
Author(s):  
Karina von Schuckmann
Keyword(s):  
Global Climate ◽  
Research Effort ◽  
Atmospheric Composition ◽  
Multidisciplinary Research ◽  
Energy Imbalance ◽  
The Past ◽  
The Earth ◽  
Multiple Measurements ◽  
Composition Changes ◽  
Past Half

<p>Human-induced atmospheric composition changes cause a radiative imbalance at the top of the atmosphere which is driving global warming. This simple number, the Earth energy imbalance (EEI), is the most fundamental metric that the scientific community and public must be aware of as the measure of how well the world is doing in the task of bringing climate change under control. Combining multiple measurements and approaches in an optimal way holds considerable promise for estimating EEI and continued quantification and reduced uncertainties can be best achieved through the maintenance of the current global climate observing system, its extension into areas of gaps in the sampling, advance on instrumental limitations, and the establishment of an international framework for concerted multidisciplinary research effort. This talk will provide an overview on the different approaches and their challenges for estimating the EEI. A particular emphasis will be drawn on the heat gain of the Earth system over the past half of a century – and particularly how much and where the heat is distributed – which is fundamental to understanding how this affects warming ocean, atmosphere and land; rising surface temperature; sea level; and loss of grounded and floating ice, which are critical concerns for society.</p><p> </p>

Global Climate Change and Aesthetics

2021 ◽  
Author(s):  
Emily Brady
Keyword(s):  
Climate Change ◽  
Global Climate Change ◽  
Research Agenda ◽  
Global Climate ◽  
Ethical Values ◽  
Global Crisis ◽  
Aesthetic Experiences ◽  
New Research ◽  
The Relationship

What kinds of issues does the global crisis of climate change present to aesthetics, and how will they challenge the field to respond? This paper argues that a new research agenda is needed for aesthetics with respect to global climate change (GCC) and outlines a set of foundational issues which are especially pressing: (1) attention to environments that have been neglected by philosophers, for example, the cryosphere and aerosphere; (2) negative aesthetics of environment, in order to grasp aesthetic experiences, meanings, and dis/values in light of the catastrophic effects of GCC; (3) bringing intergenerational thinking into aesthetics through concepts of temporality and ‘future aesthetics’ (4) understanding the relationship between aesthetic and ethical values as they arise in regard to GCC.

scholarly journals Clean air in the Anthropocene

2017 ◽  
Vol 200 ◽  
pp. 693-703 ◽  
Author(s):  
Jos Lelieveld
Keyword(s):  
Air Pollution ◽  
Sustainable Development ◽  
Air Quality ◽  
Human Health ◽  
Atmospheric Chemistry ◽  
Clean Energy ◽  
Atmospheric Composition ◽  
Anthropogenic Sources ◽  
Years Of Life Lost ◽  
Clean Air

In atmospheric chemistry, interactions between air pollution, the biosphere and human health, often through reaction mixtures from both natural and anthropogenic sources, are of growing interest. Massive pollution emissions in the Anthropocene have transformed atmospheric composition to the extent that biogeochemical cycles, air quality and climate have changed globally and partly profoundly. It is estimated that mortality attributable to outdoor air pollution amounts to 4.33 million individuals per year, associated with 123 million years of life lost. Worldwide, air pollution is the major environmental risk factor to human health, and strict air quality standards have the potential to strongly reduce morbidity and mortality. Preserving clean air should be considered a human right, and is fundamental to many sustainable development goals of the United Nations, such as good health, climate action, sustainable cities, clean energy, and protecting life on land and in the water. It would be appropriate to adopt “clean air” as a sustainable development goal.

scholarly journals A 250-year periodicity in Southern Hemisphere westerly winds over the last 2600 years

2016 ◽  
Vol 12 (2) ◽  
pp. 189-200 ◽  
Author(s):  
C. S. M. Turney ◽  
R. T. Jones ◽  
C. Fogwill ◽  
J. Hatton ◽  
A. N. Williams ◽  
...  
Keyword(s):  
Southern Hemisphere ◽  
Global Climate Change ◽  
Late Holocene ◽  
Global Climate ◽  
Falkland Islands ◽  
The Core ◽  
Atmosphere System ◽  
Westerly Winds ◽  
Ocean Atmosphere ◽  
Southern Hemisphere Westerly Winds

Abstract. Southern Hemisphere westerly airflow has a significant influence on the ocean–atmosphere system of the mid- to high latitudes with potentially global climate implications. Unfortunately, historic observations only extend back to the late 19th century, limiting our understanding of multi-decadal to centennial change. Here we present a highly resolved (30-year) record of past westerly wind strength from a Falkland Islands peat sequence spanning the last 2600 years. Situated within the core latitude of Southern Hemisphere westerly airflow (the so-called furious fifties), we identify highly variable changes in exotic pollen and charcoal derived from South America which can be used to inform on past westerly air strength. We find a period of high charcoal content between 2000 and 1000 cal. years BP, associated with increased burning in Patagonia, most probably as a result of higher temperatures and stronger westerly airflow. Spectral analysis of the charcoal record identifies a pervasive ca. 250-year periodicity that is coherent with radiocarbon production rates, suggesting that solar variability has a modulating influence on Southern Hemisphere westerly airflow. Our results have important implications for understanding global climate change through the late Holocene.

scholarly journals Isoprene emissions from a tundra ecosystem

2013 ◽  
Vol 10 (2) ◽  
pp. 871-889 ◽  
Author(s):  
M. J. Potosnak ◽  
B. M. Baker ◽  
L. LeStourgeon ◽  
S. M. Disher ◽  
K. L. Griffin ◽  
...  
Keyword(s):  
Atmospheric Chemistry ◽  
Global Climate ◽  
Common Species ◽  
Emission Rates ◽  
Arctic Ecosystems ◽  
Field Station ◽  
Isoprene Emission ◽  
Tundra Ecosystem ◽  
Leaf Level ◽  
Field Campaigns

Abstract. Whole-system fluxes of isoprene from a moist acidic tundra ecosystem and leaf-level emission rates of isoprene from a common species (Salix pulchra) in that same ecosystem were measured during three separate field campaigns. The field campaigns were conducted during the summers of 2005, 2010 and 2011 and took place at the Toolik Field Station (68.6° N, 149.6° W) on the north slope of the Brooks Range in Alaska, USA. The maximum rate of whole-system isoprene flux measured was over 1.2 mg C m−2 h−1 with an air temperature of 22 °C and a PAR level over 1500 μmol m−2 s−1. Leaf-level isoprene emission rates for S. pulchra averaged 12.4 nmol m−2 s−1 (27.4 μg C gdw−1 h−1) extrapolated to standard conditions (PAR = 1000 μmol m−2 s−1 and leaf temperature = 30 °C). Leaf-level isoprene emission rates were well characterized by the Guenther algorithm for temperature with published coefficients, but less so for light. Chamber measurements from a nearby moist acidic tundra ecosystem with little S. pulchra emitted significant amounts of isoprene, but at lower rates (0.45 mg C m−2 h−1) suggesting other significant isoprene emitters. Comparison of our results to predictions from a global model found broad agreement, but a detailed analysis revealed some significant discrepancies. An atmospheric chemistry box model predicts that the observed isoprene emissions have a significant impact on Arctic atmospheric chemistry, including a reduction of hydroxyl radical (OH) concentrations. Our results support the prediction that isoprene emissions from Arctic ecosystems will increase with global climate change.

Late-Holocene Formation of Lake Michigan Beach Ridges Correlated with a 70-yr Oscillation in Global Climate

1996 ◽  
Vol 45 (3) ◽  
pp. 321-326 ◽  
Author(s):  
Paul A. Delcourt ◽  
William H. Petty ◽  
Hazel R. Delcourt
Keyword(s):  
Late Holocene ◽  
Lake Michigan ◽  
Global Climate ◽  
Temperature Oscillation ◽  
Beach Ridges ◽  
Climate Fluctuations ◽  
The Past ◽  
Fundamental Part ◽  
Atmosphere System ◽  
Centennial Time Scale

AbstractA radiocarbon-dated series of 75 beach ridges, formed at regular intervals averaging 72 yr over the past 5400 yr, provides further support for the existence of a 70-yr oscillation in Northern Hemisphere climate, postulated recently from instrument data representing less than two cycles of this climate oscillation. Results from this study lend support to the interpretation that internal variations in the ocean–atmosphere system are an important factor in climate fluctuations on a decadal–centennial time scale. A temperature oscillation with a period of about 70 yr has been a previously unrecognized but fundamental part of the global climate system since at least the middle Holocene.

scholarly journals A comparison of atmospheric composition using the Carbon Bond and Regional Atmospheric Chemistry Mechanisms

2013 ◽  
Vol 13 (3) ◽  
pp. 6923-6969 ◽  
Author(s):  
G. Sarwar ◽  
J. Godowitch ◽  
B. Henderson ◽  
K. Fahey ◽  
G. Pouliot ◽  
...  
Keyword(s):  
Hydrogen Peroxide ◽  
Atmospheric Chemistry ◽  
Production Efficiency ◽  
Fine Particles ◽  
Secondary Organic Aerosols ◽  
Organic Aerosols ◽  
Ozone Production ◽  
Atmospheric Composition ◽  
Organic Nitrate ◽  
Carbon Bond

Abstract. We incorporate the recently developed Regional Atmospheric Chemistry Mechanism (version 2, RACM2) into the Community Multiscale Air Quality modeling system for comparison with the existing 2005 Carbon Bond mechanism with updated toluene chemistry (CB05TU). Compared to CB05TU, RACM2 enhances the domain-wide monthly mean hydroxyl radical concentrations by 46% and nitric acid by 26%. However, it reduces hydrogen peroxide by 2%, peroxyacetic acid by 94%, methyl hydrogen peroxide by 19%, peroxyacetyl nitrate by 40%, and organic nitrate by 41%. RACM2 predictions generally agree better with the observed data than the CB05TU predictions. RACM2 enhances ozone for all ambient levels leading to higher bias at low (< 60 ppbv) concentrations but improved performance at high (>70 ppbv) concentrations. The RACM2 ozone predictions are also supported by increased ozone production efficiency that agrees better with observations. Compared to CB05TU, RACM2 enhances the domain-wide monthly mean sulfate by 10%, nitrate by 6%, ammonium by 10%, anthropogenic secondary organic aerosols by 42%, biogenic secondary organic aerosols by 5%, and in-cloud secondary organic aerosols by 7%. Increased inorganic and organic aerosols with RACM2 agree better with observed data. While RACM2 enhances ozone and secondary aerosols by relatively large margins, control strategies developed for ozone or fine particles using the two mechanisms do not differ appreciably.

scholarly journals Rapid formation of isoprene photo-oxidation products observed in Amazonia

2009 ◽  
Vol 9 (3) ◽  
pp. 13629-13653 ◽  
Author(s):  
T. Karl ◽  
A. Guenther ◽  
A. Turnipseed ◽  
P. Artaxo ◽  
S. Martin
Keyword(s):  
Atmospheric Chemistry ◽  
Global Climate ◽  
Oxidative Capacity ◽  
Oxidation Products ◽  
Lower Atmosphere ◽  
Peroxy Radicals ◽  
Aerosol Formation ◽  
Photo Oxidation ◽  
Voc Oxidation ◽  
Rapid Formation

Abstract. Isoprene represents the single most important reactive hydrocarbon for atmospheric chemistry in the tropical atmosphere. It plays a central role in global and regional atmospheric chemistry and possible climate feedbacks. Photo-oxidation of primary hydrocarbons (e.g. isoprene) leads to the formation of oxygenated VOCs (OVOCs). The evolution of these intermediates affects the oxidative capacity of the atmosphere (by reacting with OH) and can contribute to secondary aerosol formation, a poorly understood process. An accurate and quantitative understanding of VOC oxidation processes is needed for model simulations of regional air quality and global climate. Based on field measurements conducted during the Amazonian aerosol characterization experiment (AMAZE-08) we show that the production of certain OVOCs (e.g. hydroxyacetone) from isoprene photo-oxidation in the lower atmosphere is significantly underpredicted by standard chemistry schemes. A recently suggested novel pathway for isoprene peroxy radicals could explain the observed discrepancy and reconcile the rapid formation of these VOCs. Furthermore, if generalized our observations suggest that prompt photochemical formation of OVOCs and other uncertainties in VOC oxidation schemes could result in substantial underestimates of modelled OH reactivity that could explain a major fraction of the missing OH sink over forests which has previously been attributed to a missing source of primary biogenic VOCs.

scholarly journals Mineral protection regulates the long-term global preservation of natural organic carbon

2021 ◽  
Author(s):  
Jordon Hemingway ◽  
Daniel Rothman ◽  
Katherine Grant ◽  
Sarah Rosengard ◽  
Timothy Eglinton ◽  
...  
Keyword(s):  
Organic Carbon ◽  
Redox State ◽  
Global Climate ◽  
Atmospheric Oxygen ◽  
Atmospheric Composition ◽  
Earth Surface ◽  
Mountain Ranges ◽  
Surface Redox ◽  
Carbon Erosion

&lt;p&gt;The vast majority of organic carbon (OC) produced by life is respired back to carbon dioxide (CO&lt;sub&gt;2&lt;/sub&gt;), but roughly 0.1% escapes and is preserved over geologic timescales. By sequestering reduced carbon from Earth&amp;#8217;s surface, this &amp;#8220;slow OC leak&amp;#8221; contributes to CO&lt;sub&gt;2&lt;/sub&gt; removal and promotes the accumulation of atmospheric oxygen and oxidized minerals. Countering this, OC contained within sedimentary rocks is oxidized during exhumation and erosion of mountain ranges. By respiring previously sequestered reduced carbon, erosion consumes atmospheric oxygen and produces CO&lt;sub&gt;2&lt;/sub&gt;. The balance between these two processes&amp;#8212;preservation and respiration&amp;#8212;regulates atmospheric composition, Earth-surface redox state, and global climate. Despite this importance, the governing mechanisms remain poorly constrained. To provide new insight, we developed a method that investigates OC composition using bond-strength distributions coupled with radiocarbon ages. Here I highlight a suite of recent results using this approach, and I show that biospheric OC interacts with particles and becomes physiochemically protected during aging, thus promoting preservation. I will discuss how this mechanistic framework can help elucidate why OC preservation&amp;#8212;and thus atmospheric composition, Earth-surface redox state, and climate&amp;#8212;has varied throughout Earth history.&lt;/p&gt;

scholarly journals New Results on the Composition of the Outer Planets and Titan

2005 ◽  
Vol 13 ◽  
pp. 891-893
Author(s):  
Thierry Fouchet
Keyword(s):  
Solar System ◽  
Atmospheric Chemistry ◽  
Recent Progress ◽  
Giant Planets ◽  
Atmospheric Composition ◽  
Solar System Formation ◽  
Outer Planets ◽  
System Formation ◽  
The Impact

AbstractIn this brief summary, I present recent progress on our knowledge of the Giant Planets and Titan atmospheric composition, as well as the impact of this progress on our understanding of Solar System formation, and atmospheric chemistry.

Sign in / Sign up

Export Citation Format

Share Document