scholarly journals DMS emissions from the Arctic marginal ice zone

Elem Sci Anth ◽  
2021 ◽  
Vol 9 (1) ◽  
Author(s):  
Martí Galí ◽  
Martine Lizotte ◽  
David J. Kieber ◽  
Achim Randelhoff ◽  
Rachel Hussherr ◽  
...  

Phytoplankton blooms in the Arctic marginal ice zone (MIZ) can be prolific dimethylsulfide (DMS) producers, thereby influencing regional aerosol formation and cloud radiative forcing. Here we describe the distribution of DMS and its precursor dimethylsulfoniopropionate (DMSP) across the Baffin Bay receding ice edge in early summer 2016. Overall, DMS and total DMSP (DMSPt) increased towards warmer waters of Atlantic origin concurrently with more advanced ice-melt and bloom stages. Relatively high DMS and DMSPt (medians of 6.3 and 70 nM, respectively) were observed in the surface layer (0–9 m depth), and very high values (reaching 74 and 524 nM, respectively) at the subsurface biomass maximum (15–30 m depth). Microscopic and pigment analyses indicated that subsurface DMS and DMSPt peaks were associated with Phaeocystis pouchetii, which bloomed in Atlantic-influenced waters and reached unprecedented biomass levels in Baffin Bay. In surface waters, DMS concentrations and DMS:DMSPt ratios were higher in the MIZ (medians of 12 nM and 0.15, respectively) than in fully ice-covered or ice-free conditions, potentially associated with enhanced phytoplanktonic DMSP release and bacterial DMSP cleavage (high dddP:dmdA gene ratios). Mean sea–air DMS fluxes (µmol m–2 d–1) increased from 0.3 in ice-covered waters to 10 in open waters (maximum of 26) owing to concurrent trends in near-surface DMS concentrations and physical drivers of gas exchange. Using remotely sensed sea-ice coverage and a compilation of sea–air DMS flux data, we estimated that the pan-Arctic DMS emission from the MIZ (EDMS, MIZ) was 5–13 Gg S yr–1. North of 80°N, EDMS, MIZ might have increased by around 10 ± 4% yr–1 between 2003 and 2014, likely exceeding open-water emissions in June and July. We conclude that EDMS, MIZ must be taken into account to evaluate plankton-climate feedbacks in the Arctic.

Elem Sci Anth ◽  
2016 ◽  
Vol 4 ◽  
Author(s):  
Seth Zippel ◽  
Jim Thomson

Abstract The importance of waves in the Arctic Ocean has increased with the significant retreat of the seasonal sea-ice extent. Here, we use wind, wave, turbulence, and ice measurements to evaluate the response of the ocean surface to a given wind stress within the marginal ice zone, with a focus on the local wind input to waves and subsequent ocean surface turbulence. Observations are from the Beaufort Sea in the summer and early fall of 2014, with fractional ice cover of up to 50%. Observations showed strong damping and scattering of short waves, which, in turn, decreased the wind energy input to waves. Near-surface turbulent dissipation rates were also greatly reduced in partial ice cover. The reductions in waves and turbulence were balanced, suggesting that a wind-wave equilibrium is maintained in the marginal ice zone, though at levels much less than in open water. These results suggest that air-sea interactions are suppressed in the marginal ice zone relative to open ocean conditions at a given wind forcing, and this suppression may act as a feedback mechanism in expanding a persistent marginal ice zone throughout the Arctic.


2021 ◽  
Vol 12 (1) ◽  
Author(s):  
Jennifer A. MacKinnon ◽  
Harper L. Simmons ◽  
John Hargrove ◽  
Jim Thomson ◽  
Thomas Peacock ◽  
...  

AbstractUnprecedented quantities of heat are entering the Pacific sector of the Arctic Ocean through Bering Strait, particularly during summer months. Though some heat is lost to the atmosphere during autumn cooling, a significant fraction of the incoming warm, salty water subducts (dives beneath) below a cooler fresher layer of near-surface water, subsequently extending hundreds of kilometers into the Beaufort Gyre. Upward turbulent mixing of these sub-surface pockets of heat is likely accelerating sea ice melt in the region. This Pacific-origin water brings both heat and unique biogeochemical properties, contributing to a changing Arctic ecosystem. However, our ability to understand or forecast the role of this incoming water mass has been hampered by lack of understanding of the physical processes controlling subduction and evolution of this this warm water. Crucially, the processes seen here occur at small horizontal scales not resolved by regional forecast models or climate simulations; new parameterizations must be developed that accurately represent the physics. Here we present novel high resolution observations showing the detailed process of subduction and initial evolution of warm Pacific-origin water in the southern Beaufort Gyre.


2003 ◽  
Vol 81 (8) ◽  
pp. 1298-1305 ◽  
Author(s):  
Mads Peter Heide-Jørgensen ◽  
Rune Dietz ◽  
Kristin L Laidre ◽  
Pierre Richard ◽  
Jack Orr ◽  
...  

Sixteen female narwhals (Monodon monoceros) were tracked by satellite in 2000 and 2001 from their summering ground near Somerset Island in the Canadian High Arctic to their wintering ground in central Baffin Bay. The wintering ground location was spatially discrete from another narwhal wintering ground in southern Baffin Bay. Area extent of the summering ground was approximately 9464 km2 and area extent of the wintering ground was 25 846 km2. Two of the narwhals were tracked for more than 12 consecutive months. These whales used three focal areas between their spring and autumn migration: a coastal area in the open-water season in August in the Canadian High Arctic, a wintering area from November through April in the consolidated pack ice of Baffin Bay, and an early summer area in front of the receding fast ice edge in Lancaster Sound. The whales showed remarkable site fidelity to summering grounds and had specific migratory routes that followed sea ice formation and recession.


2017 ◽  
Vol 17 (14) ◽  
pp. 8757-8770 ◽  
Author(s):  
Roghayeh Ghahremaninezhad ◽  
Ann-Lise Norman ◽  
Betty Croft ◽  
Randall V. Martin ◽  
Jeffrey R. Pierce ◽  
...  

Abstract. Vertical distributions of atmospheric dimethyl sulfide (DMS(g)) were sampled aboard the research aircraft Polar 6 near Lancaster Sound, Nunavut, Canada, in July 2014 and on pan-Arctic flights in April 2015 that started from Longyearbyen, Spitzbergen, and passed through Alert and Eureka, Nunavut, and Inuvik, Northwest Territories. Larger mean DMS(g) mixing ratios were present during April 2015 (campaign mean of 116  ±  8 pptv) compared to July 2014 (campaign mean of 20  ±  6 pptv). During July 2014, the largest mixing ratios were found near the surface over the ice edge and open water. DMS(g) mixing ratios decreased with altitude up to about 3 km. During April 2015, profiles of DMS(g) were more uniform with height and some profiles showed an increase with altitude. DMS reached as high as 100 pptv near 2500 m. Relative to the observation averages, GEOS-Chem (www.geos-chem.org) chemical transport model simulations were higher during July and lower during April. Based on the simulations, more than 90 % of the July DMS(g) below 2 km and more than 90 % of the April DMS(g) originated from Arctic seawater (north of 66° N). During April, 60 % of the DMS(g), between 500 and 3000 m originated from Arctic seawater. During July 2014, FLEXPART (FLEXible PARTicle dispersion model) simulations locate the sampled air mass over Baffin Bay and the Canadian Arctic Archipelago 4 days back from the observations. During April 2015, the locations of the air masses 4 days back from sampling were varied: Baffin Bay/Canadian Archipelago, the Arctic Ocean, Greenland and the Pacific Ocean. Our results highlight the role of open water below the flight as the source of DMS(g) during July 2014 and the influence of long-range transport (LRT) of DMS(g) from further afield in the Arctic above 2500 m during April 2015.


2016 ◽  
Author(s):  
S. Kern ◽  
A. Rösel ◽  
L. T. Pedersen ◽  
N. Ivanova ◽  
R. Saldo ◽  
...  

Abstract. The sea ice concentration (SIC) derived from satellite microwave brightness temperature (TB) data are known to be less accurate during summer melt conditions – in the Arctic Ocean primarily because of the impact of melt ponds on sea ice. Using data from June to August 2009, we investigate how TBs and SICs vary as a function of the ice surface fraction (ISF) computed from open water fraction and melt pond fraction both derived from satellite optical reflectance data. SIC is computed from TBs using a set of eight different retrieval algorithms and applying a consistent set of tie points. We find that TB values change during sea ice melt non-linearly and not monotonically as a function of ISF for ISF of 50 to 100 %. For derived parameters such as the polarization ratio at 19 GHz the change is monotonic but substantially smaller than theoretically expected. Changes in ice/snow radiometric properties during melt also contribute to the TB changes observed; these contributions are functions of frequency and polarization and have the potential to partly counter-balance the impact of changing ISF on the observed TBs. All investigated SIC retrieval algorithms overestimate ISF when using winter tie points. The overestimation varies among the algorithms as a function of ISF such that the SIC retrieval algorithms could be categorized into two different classes. These reveal a different degree of ISF overestimation at high ISF and an opposite development of ISF over-estimation as ISF decreases. For one class, correlations between SIC and ISF are ≥ 0.85 and the associated linear regression lines suggest an exploitable relationship between SIC and ISF if reliable summer sea ice tie points can be established. This study shows that melt ponds are interpreted as open water by the SIC algorithms, while the concentration of ice between the melt ponds is in general being overestimated. These two effects may cancel each other out and thus produce seemingly correct SIC for the wrong reasons. This cancelling effect will in general only be "correct" at one specific value of MPF. Based on our findings we recommend to not correct SIC algorithms for the impact of melt ponds as this seems to violate physical principles. Users should be aware that the SIC algorithms available at the moment retrieve a combined parameter presented by SIC in winter and ISF in summer.


2020 ◽  
Vol 20 (13) ◽  
pp. 8139-8156
Author(s):  
Tobias Donth ◽  
Evelyn Jäkel ◽  
André Ehrlich ◽  
Bernd Heinold ◽  
Jacob Schacht ◽  
...  

Abstract. The magnitude of solar radiative effects (cooling or warming) of black carbon (BC) particles embedded in the Arctic atmosphere and surface snow layer was explored on the basis of case studies. For this purpose, combined atmospheric and snow radiative transfer simulations were performed for cloudless and cloudy conditions on the basis of BC mass concentrations measured in pristine early summer and more polluted early spring conditions. The area of interest is the remote sea-ice-covered Arctic Ocean in the vicinity of Spitsbergen, northern Greenland, and northern Alaska typically not affected by local pollution. To account for the radiative interactions between the black-carbon-containing snow surface layer and the atmosphere, an atmospheric and snow radiative transfer model were coupled iteratively. For pristine summer conditions (no atmospheric BC, minimum solar zenith angles of 55∘) and a representative BC particle mass concentration of 5 ng g−1 in the surface snow layer, a positive daily mean solar radiative forcing of +0.2 W m−2 was calculated for the surface radiative budget. A higher load of atmospheric BC representing early springtime conditions results in a slightly negative mean radiative forcing at the surface of about −0.05 W m−2, even when the low BC mass concentration measured in the pristine early summer conditions was embedded in the surface snow layer. The total net surface radiative forcing combining the effects of BC embedded in the atmosphere and in the snow layer strongly depends on the snow optical properties (snow specific surface area and snow density). For the conditions over the Arctic Ocean analyzed in the simulations, it was found that the atmospheric heating rate by water vapor or clouds is 1 to 2 orders of magnitude larger than that by atmospheric BC. Similarly, the daily mean total heating rate (6 K d−1) within a snowpack due to absorption by the ice was more than 1 order of magnitude larger than that of atmospheric BC (0.2 K d−1). Also, it was shown that the cooling by atmospheric BC of the near-surface air and the warming effect by BC embedded in snow are reduced in the presence of clouds.


2016 ◽  
Vol 29 (24) ◽  
pp. 8721-8744 ◽  
Author(s):  
Georgia Sotiropoulou ◽  
Michael Tjernström ◽  
Joseph Sedlar ◽  
Peggy Achtert ◽  
Barbara J. Brooks ◽  
...  

Abstract The Arctic Clouds in Summer Experiment (ACSE) was conducted during summer and early autumn 2014, providing a detailed view of the seasonal transition from ice melt into freeze-up. Measurements were taken over both ice-free and ice-covered surfaces near the ice edge, offering insight into the role of the surface state in shaping the atmospheric conditions. The initiation of the autumn freeze-up was related to a change in air mass, rather than to changes in solar radiation alone; the lower atmosphere cooled abruptly, leading to a surface heat loss. During melt season, strong surface inversions persisted over the ice, while elevated inversions were more frequent over open water. These differences disappeared during autumn freeze-up, when elevated inversions persisted over both ice-free and ice-covered conditions. These results are in contrast to previous studies that found a well-mixed boundary layer persisting in summer and an increased frequency of surface-based inversions in autumn, suggesting that knowledge derived from measurements taken within the pan-Arctic area and on the central ice pack does not necessarily apply closer to the ice edge. This study offers an insight into the atmospheric processes that occur during a crucial period of the year; understanding and accurately modeling these processes is essential for the improvement of ice-extent predictions and future Arctic climate projections.


2007 ◽  
Vol 7 (19) ◽  
pp. 5043-5059 ◽  
Author(s):  
S. E. Bauer ◽  
D. Koch ◽  
N. Unger ◽  
S. M. Metzger ◽  
D. T. Shindell ◽  
...  

Abstract. Nitrate aerosols are expected to become more important in the future atmosphere due to the expected increase in nitrate precursor emissions and the decline of ammonium-sulphate aerosols in wide regions of this planet. The GISS climate model is used in this study, including atmospheric gas- and aerosol phase chemistry to investigate current and future (2030, following the SRES A1B emission scenario) atmospheric compositions. A set of sensitivity experiments was carried out to quantify the individual impact of emission- and physical climate change on nitrate aerosol formation. We found that future nitrate aerosol loads depend most strongly on changes that may occur in the ammonia sources. Furthermore, microphysical processes that lead to aerosol mixing play a very important role in sulphate and nitrate aerosol formation. The role of nitrate aerosols as climate change driver is analyzed and set in perspective to other aerosol and ozone forcings under pre-industrial, present day and future conditions. In the near future, year 2030, ammonium nitrate radiative forcing is about −0.14 W/m² and contributes roughly 10% of the net aerosol and ozone forcing. The present day nitrate and pre-industrial nitrate forcings are −0.11 and −0.05 W/m², respectively. The steady increase of nitrate aerosols since industrialization increases its role as a non greenhouse gas forcing agent. However, this impact is still small compared to greenhouse gas forcings, therefore the main role nitrate will play in the future atmosphere is as an air pollutant, with annual mean near surface air concentrations, in the fine particle mode, rising above 3 μg/m³ in China and therefore reaching pollution levels, like sulphate aerosols.


2013 ◽  
Vol 13 (1) ◽  
pp. 177-199 ◽  
Author(s):  
A. Devasthale ◽  
T. Koenigk ◽  
J. Sedlar ◽  
E. J. Fetzer

Abstract. The record sea-ice minimum (SIM) extents observed during the summers of 2007 and 2012 in the Arctic are stark evidence of accelerated sea ice loss during the last decade. Improving our understanding of the Arctic atmosphere and accurate quantification of its characteristics becomes ever more crucial, not least to improve predictions of such extreme events in the future. In this context, the Atmospheric Infrared Sounder (AIRS) instrument onboard NASA's Aqua satellite provides crucial insights due to its ability to provide 3-D information on atmospheric thermodynamics. Here, we facilitate comparisons in the evolution of the thermodynamic state of the Arctic atmosphere during these two SIM events using a decade long AIRS observational record (2003–2012). It is shown that the meteorological conditions during 2012 were not extreme but three factors in preconditioning from winter through early summer probably played an important role in accelerating sea-ice melt. First, the marginal sea-ice zones along the central Eurasian and North Atlantic sectors remained warm throughout winter and early spring in 2012 preventing thicker ice build-up. Second, the circulation pattern favoured efficient sea-ice transport out of the Arctic in the Atlantic sector during late spring and early summer in 2012 compared to 2007. Third, additional warming over the Canadian Archipelago and southeast Beaufort Sea from May onward further contributed to accelerated sea-ice melt. All these factors may have lead already thin and declining sea-ice cover to pass below the previous sea-ice extent minimum of 2007. In sharp contrast to 2007, negative surface temperature anomalies and increased cloudiness were observed over the East Siberian and Chukchi Seas in the summer of 2012. The results suggest that satellite-based monitoring of atmospheric preconditioning could be a critical source of information in predicting extreme sea-ice melting events in the Arctic.


2021 ◽  
Author(s):  
Janosch Michaelis ◽  
Christof Lüpkes ◽  
Amelie Schmitt ◽  
Jörg Hartmann

<p><span><span>The polar ocean regions are characterised by a large variety of interactions between sea ice surfaces</span><span>, open water</span><span>, and the atmosphere. Especially between late autumn and spring, leads (open-water channels in sea ice) may play a crucial role within this system: Due to large temperature differences between the surface of leads and the near-surface atmosphere, strong turbulent convective plumes are generated with an enhanced turbulent transport of heat, moisture, and momentum. In consequence, lead-generated convection has a strong impact on the characteristics of the polar atmospheric boundary layer (ABL). </span></span></p><p><span><span>We apply a plume- but non-eddy-resolving, microscale model to study the convection over three different leads, which had been observed during the aircraft campaign STABLE over the Arctic Marginal Sea Ice Zone in March 2013. Model simulations are performed using a local and a non-local turbulence closure. The latter represents a lead-width-dependent approach for </span><span>the </span><span>turbulent fluxes </span><span>based on large eddy simulation </span><span>and it is</span><span> designed for an idealised, </span><span>lead-perpendicular</span><span>, and near-neutral inflow in an ABL of 300m </span><span>thickness</span><span>. </span><span>The observed cases from STABLE are also characterised by lead-perpendicular inflow conditions</span><span>, but the ABL is much shallower than in the ideali</span><span>s</span><span>ed cases and the inflow stratification is </span><span>partly</span><span> (slightly) stable. </span><span>Our main goal is to study the quality of both parametrizations and to evaluate, if the non-local parametrization shows advantages as compared to the local closure.</span></span></p><p><span><span>We show that the basic</span><span> observed features of the lead-generated convection are represented with both closures </span><span>despite some minor differences that will be explained</span><span>. However, the advantages of the non-local closure become clearly obvious by the physically more realistic representation of regions with observed vertical entrainment or where the observations hint at counter-gradient transport. Moreover, we also show that some weaknesses of the simulations can be </span><span>almost </span><span>overcome by introducing two further modifications </span><span>of</span><span> the non-local closure. We consider our results as another important step in the development of atmospheric turbulence parametrizations </span><span>for </span><span>non-eddy-resolving, microscale simulations of</span><span> strongly inhomogeneous convective </span><span>boundary layers</span><span>.</span></span></p>


Sign in / Sign up

Export Citation Format

Share Document