scholarly journals Time-resolved terahertz time-domain near-field microscopy

2018 ◽  
Vol 26 (24) ◽  
pp. 32118 ◽  
Author(s):  
N. J. J. van Hoof ◽  
S. E. T. ter Huurne ◽  
J. Gómez Rivas ◽  
A. Halpin
Keyword(s):  
Time Domain ◽  
Near Field ◽  
Time Resolved

scholarly journals A time-domain phase diagram of metastable states in a charge ordered quantum material

2021 ◽  
Vol 12 (1) ◽  
Author(s):  
Jan Ravnik ◽  
Michele Diego ◽  
Yaroslav Gerasimenko ◽  
Yevhenii Vaskivskyi ◽  
Igor Vaskivskyi ◽  
...  
Keyword(s):  
Phase Diagram ◽  
Time Domain ◽  
Metastable States ◽  
Scanning Tunneling ◽  
Photon Density ◽  
Tunneling Microscopy ◽  
Equilibrium Conditions ◽  
Time Resolved ◽  
A Charge ◽  
Non Equilibrium

AbstractMetastable self-organized electronic states in quantum materials are of fundamental importance, displaying emergent dynamical properties that may be used in new generations of sensors and memory devices. Such states are typically formed through phase transitions under non-equilibrium conditions and the final state is reached through processes that span a large range of timescales. Conventionally, phase diagrams of materials are thought of as static, without temporal evolution. However, many functional properties of materials arise as a result of complex temporal changes in the material occurring on different timescales. Hitherto, such properties were not considered within the context of a temporally-evolving phase diagram, even though, under non-equilibrium conditions, different phases typically evolve on different timescales. Here, by using time-resolved optical techniques and femtosecond-pulse-excited scanning tunneling microscopy (STM), we track the evolution of the metastable states in a material that has been of wide recent interest, the quasi-two-dimensional dichalcogenide 1T-TaS2. We map out its temporal phase diagram using the photon density and temperature as control parameters on timescales ranging from 10−12 to 103 s. The introduction of a time-domain axis in the phase diagram enables us to follow the evolution of metastable emergent states created by different phase transition mechanisms on different timescales, thus enabling comparison with theoretical predictions of the phase diagram, and opening the way to understanding of the complex ordering processes in metastable materials.

Three-Dimensional Finite-Difference Time-Domain Method Modeling of Nanowire Optical Probe

2014 ◽  
Vol 602-605 ◽  
pp. 3359-3362
Author(s):  
Chun Li Zhu ◽  
Jing Li
Keyword(s):  
Finite Difference ◽  
Time Domain ◽  
Finite Difference Time Domain ◽  
Incident Light ◽  
Near Field ◽  
Three Dimensional ◽  
Polarization Direction ◽  
Near Field Imaging ◽  
Difference Time ◽  
Field Imaging

In this paper, output near fields of nanowires with different optical and structure configurations are calculated by using the three-dimensional finite-difference time-domain (3D FDTD) method. Then a nanowire with suitable near field distribution is chosen as the probe for scanning dielectric and metal nanogratings. Scanning results show that the resolution in near-field imaging of dielectric nanogratings can be as low as 80nm, and the imaging results are greatly influenced by the polarization direction of the incident light. Compared with dielectric nanogratings, metal nanogratings have significantly enhanced resolutions when the arrangement of gratings is perpendicular to the polarization direction of the incident light due to the enhancement effect of the localized surface plasmons (SPs). Results presented here could offer valuable references for practical applications in near-field imaging with nanowires as optical probes.

scholarly journals An Iterative Interpolated DFT to Remove Spectral Leakage in Time-Domain Near-Field Scanning

2018 ◽  
Vol 60 (1) ◽  
pp. 202-210 ◽  
Author(s):  
Tim Claeys ◽  
Dries Vanoost ◽  
Joan Peuteman ◽  
Guy A. E. Vandenbosch ◽  
Davy Pissoort
Keyword(s):  
Time Domain ◽  
Near Field ◽  
Spectral Leakage ◽  
Near Field Scanning
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