One- and two-photon induced change of third order nonlinearity in phenylamine azo-dye polymer thin films

Author(s):  
Chia Chen Hsu ◽  
Victor M. Churikov ◽  
Jiann T'suen Lin ◽  
Hui Hsien Wu ◽  
Jian Hung Lin ◽  
...  
2002 ◽  
Vol 209 (4-6) ◽  
pp. 451-460 ◽  
Author(s):  
Victor M. Churikov ◽  
Jiann T'suen Lin ◽  
Hui Hsien Wu ◽  
Jian Hung Lin ◽  
Tzer-Hsing Huang ◽  
...  

2016 ◽  
Author(s):  
Anil Tumuluri ◽  
Mounika Rapolu ◽  
S. Venugopal Rao ◽  
K. C. James Raju

2013 ◽  
Vol 30 (8) ◽  
pp. 2226 ◽  
Author(s):  
S. Akbar Ali ◽  
P. B. Bisht ◽  
B. S. Kalanoor ◽  
Anuradha Patra ◽  
S. Kasiviswanathan

Author(s):  
HARI SINGH NALWA ◽  
SETSUO KOBAYASHI

Third-order non-linear optical susceptibilities of silicon, germanium, tin, aluminum, manganese and vanadium naphthalocyanine derivatives measured by third-harmonic generation technique from 1.05 μm to 2.1 μm are reported. Our results show the dependence of χ(3)(–3ω;ω,ω,ω) values on the variation of the central metal atom associated to different metal-ligand charge-transfer interactions. Silicon naphthalocyanines ( SiNc ) showed the χ(3)(–3ω;ω,ω,ω) values on the order of 10−10 esu at 1.5 μm, this does not appear to be due to a three-photon resonance, instead the increase in χ(3) could be the two-photon resonance lying just above the one-photon state. Degenerate four-wave mixing measurements on thin films of a SiNc derivative yielded the χ(3)(–3ω;ω,ω,ω) value as high as 5.0 × 10−7 esu at 800 nm, enhanced by one-photon resonance near the Q-band peak region. The figure of merit χ(3)/α at 800 nm is quite large corresponding to 4.2 × 10−12 esu cm. Effect of the metal atoms and plausible resonance contribution accounting for large third-order optical non-linearity of naphthalocyanines are discussed.


2010 ◽  
Vol 39 (45) ◽  
pp. 10967 ◽  
Author(s):  
Li-Wei Han ◽  
Jian Lü ◽  
Tian-Fu Liu ◽  
Shui-Ying Gao ◽  
Rong Cao

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