Exciton-Trion-Polaritons in Two-Dimensional Materials: Correlated Many Body States of Matter and Light

2020 ◽  
Author(s):  
Farhan Rana ◽  
Okan Koksal ◽  
Minwoo Jung ◽  
Gennady Shvets ◽  
Christina Manolatou
Keyword(s):  
Two Dimensional ◽  
Many Body ◽  
Two Dimensional Materials

scholarly journals Phonon-assisted processes in the ultraviolet-transient optical response of graphene

2019 ◽  
Vol 3 (1) ◽  
Author(s):  
Dino Novko ◽  
Marko Kralj
Keyword(s):  
Dominant Role ◽  
Chemical Doping ◽  
Two Dimensional ◽  
Many Body ◽  
Time Resolved ◽  
Electron Phonon Interaction ◽  
Spectral Changes ◽  
Two Dimensional Materials ◽  
Many Body Interactions

AbstractMany recent experiments investigated potential and attractive means of modifying many-body interactions in two-dimensional materials through time-resolved spectroscopy techniques. However, the role of ultrafast phonon-assisted processes in two-dimensional systems is rarely discussed in depth. Here, we investigate the role of electron–phonon interaction in the transient optical absorption of graphene by means of first-principles methods. It is shown at equilibrium that the phonon-assisted transitions renormalize significantly the electronic structure. As a result, absorption peak around the Van-Hove singularity broadens and redshifts by ~100 meV. In addition, temperature increase and chemical doping are shown to notably enhance these phonon-assisted features. In the photoinduced transient response, we obtain spectral changes in close agreement with the experiments, and we associate them to the strong renormalization of occupied and unoccupied $$\pi$$π bands, which predominantly comes from the coupling with the zone-center $${E}_{2g}$$E2g optical phonon. Our estimation of the Coulomb interaction effects shows that the phonon-assisted processes can have a dominant role even in the subpicosecond regime.

Two-dimensional materials: Electronic structure and many-body effects

2014 ◽  
Vol 526 (9-10) ◽  
pp. A81-A82 ◽  
Author(s):  
Francisco Guinea ◽  
Mikhail I. Katsnelson ◽  
Tim O. Wehling
Keyword(s):  
Electronic Structure ◽  
Two Dimensional ◽  
Many Body ◽  
Two Dimensional Materials ◽  
Many Body Effects

First-Principles Evaluation of the Potential of Borophene as a Monolayer Transparent Conductor

2017 ◽  
Author(s):  
Lyudmyla Adamska ◽  
Sridhar Sadasivam ◽  
Jonathan J. Foley ◽  
Pierre Darancet ◽  
Sahar Sharifzadeh
Keyword(s):  
First Principles ◽  
Density Functional ◽  
State Of The Art ◽  
Transparent Electrode ◽  
Visible Range ◽  
Two Dimensional ◽  
Transparent Conductor ◽  
Many Body ◽  
Functional Theory ◽  
Many Body Perturbation Theory

Two-dimensional boron is promising as a tunable monolayer metal for nano-optoelectronics. We study the optoelectronic properties of two likely allotropes of two-dimensional boron using first-principles density functional theory and many-body perturbation theory. We find that both systems are anisotropic metals, with strong energy- and thickness-dependent optical transparency and a weak (<1%) absorbance in the visible range. Additionally, using state-of-the-art methods for the description of the electron-phonon and electron-electron interactions, we show that the electrical conductivity is limited by electron-phonon interactions. Our results indicate that both structures are suitable as a transparent electrode.

Redox-Active Approach Towards New Magnetic And Conductive Two-Dimensional Materials

2018 ◽  
Author(s):  
Penny Perlepe ◽  
Rodolphe Clérac ◽  
Itziar Oyarzabal ◽  
Corine Mathonière
Keyword(s):  
Two Dimensional ◽  
Active Approach ◽  
Redox Active ◽  
Two Dimensional Materials

scholarly journals Polarization-sensitive photodetectors based on three-dimensional molybdenum disulfide (MoS2) field-effect transistors

Nanophotonics ◽  
2020 ◽  
Vol 9 (16) ◽  
pp. 4719-4728
Author(s):  
Tao Deng ◽  
Shasha Li ◽  
Yuning Li ◽  
Yang Zhang ◽  
Jingye Sun ◽  
...  
Keyword(s):  
Molybdenum Disulfide ◽  
Field Effect ◽  
High Performance ◽  
Field Effect Transistors ◽  
Three Dimensional ◽  
Polarized Light ◽  
Optical Field ◽  
Two Dimensional ◽  
Polarization Ratio ◽  
Two Dimensional Materials

AbstractThe molybdenum disulfide (MoS2)-based photodetectors are facing two challenges: the insensitivity to polarized light and the low photoresponsivity. Herein, three-dimensional (3D) field-effect transistors (FETs) based on monolayer MoS2 were fabricated by applying a self–rolled-up technique. The unique microtubular structure makes 3D MoS2 FETs become polarization sensitive. Moreover, the microtubular structure not only offers a natural resonant microcavity to enhance the optical field inside but also increases the light-MoS2 interaction area, resulting in a higher photoresponsivity. Photoresponsivities as high as 23.8 and 2.9 A/W at 395 and 660 nm, respectively, and a comparable polarization ratio of 1.64 were obtained. The fabrication technique of the 3D MoS2 FET could be transferred to other two-dimensional materials, which is very promising for high-performance polarization-sensitive optical and optoelectronic applications.

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