Anisotropy of Nonlinear Change of Refractive Index in Cr4+:YAG at Continuous-Wave Resonant Excitation

Author(s):  
Alexander V. Kir'yanov ◽  
Juan Carlos Bermudez G.
2020 ◽  
pp. 131-138

The nonlinear optical properties of pepper oil are studied by diffraction ring patterns and Z-scan techniques with continuous wave beam from solid state laser at 473 nm wavelength. The nonlinear refractive index of the sample is calculated by both techniques. The sample show high nonlinear refractive index. Based on Fresnel-Kirchhoff diffraction integral, the far-field intensity distributions of ring patterns have been calculated. It is found that the experimental results are in good agreement with the theoretical results. Also the optical limiting property of pepper oil is reported. The results obtained in this study prove that the pepper oil has applications in nonlinear optical devices.


PLoS ONE ◽  
2021 ◽  
Vol 16 (9) ◽  
pp. e0257808
Author(s):  
Dian Alwani Zainuri ◽  
Mundzir Abdullah ◽  
Muhamad Fikri Zaini ◽  
Hazri Bakhtiar ◽  
Suhana Arshad ◽  
...  

The Ultraviolet-visible (UV-Vis) spectra indicate that anthracenyl chalcones (ACs) have high maximum wavelengths and good transparency windows for optical applications and are suitable for optoelectronic applications owing to their HOMO–LUMO energy gaps (2.93 and 2.76 eV). Different donor substituents on the AC affect their dipole moments and nonlinear optical (NLO) responses. The positive, negative, and neutral electrostatic potential regions of the molecules were identified using molecular electrostatic potential (MEP). The stability of the molecule on account of hyperconjugative interactions and accompanying charge delocalization was analyzed using natural bond orbital (NBO) analysis. Open and closed aperture Z-scans were performed using a continuous-wave frequency-doubled diode-pumped solid-state (DPSS) laser to measure the nonlinear absorption and nonlinear refractive index coefficients, respectively. The valley-to-peak profile of AC indicated a negative nonlinear refractive index coefficient. The obtained single crystals possess reverse saturation absorption due to excited-state absorption. The structural and nonlinear optical properties of the molecules have been discussed, along with the role of anthracene substitution for enhancing the nonlinear optical properties. The calculated third-order susceptibility value was 1.10 x10-4 esu at an intensity of 4.1 kW/cm2, higher than the reported values for related chalcone derivatives. The NLO response for both ACs offers excellent potential in optical switching and limiting applications.


2011 ◽  
Vol 20 (02) ◽  
pp. 183-191 ◽  
Author(s):  
FRYAD Z. HENARI ◽  
ABDULLAH M. ASIRI

We report results from investigations of the nonlinear refractive index and nonlinear absorption coefficient of (2E)-3-[4-(Dimethylamino)phenyl]-1-(2,5-dimethylthiophen-3-yl)prop-2-en-1-one and (2E)-3-(3,4-Dimethoxyphenyl)-1-(2,5-dimethylthiophen-3-yl) prop-2-en-1-one using Z-scan technique with a continuous wave (cw) laser at wavelengths 488 nm and 514 nm. The nonlinear refractive index and nonlinear absorption coefficient of both samples were evaluated. The origin of the nonlinear effects was discussed. Optical limiting based on light induced nonlinear refractive index variation is demonstrated. The limiting thresholds were estimated for both samples. The results suggested that these materials offer promise as candidates for optical limiting and optical devices in the low power regime.


1998 ◽  
Vol 23 (16) ◽  
pp. 1274 ◽  
Author(s):  
D. Monzón-Hernández ◽  
A. N. Starodumov ◽  
Yu. O. Barmenkov ◽  
I. Torres-Gómez ◽  
F. Mendoza-Santoyo

2005 ◽  
Vol 81 (1) ◽  
pp. 83-91 ◽  
Author(s):  
N. N. Il’ichev ◽  
A. V. Kir’yanov ◽  
V. P. Shapkin ◽  
S. A. Nasibov ◽  
S. Ye. Mosaleva

2021 ◽  
Vol 11 (1) ◽  
Author(s):  
Stefan Reich ◽  
Sebastian Schäffer ◽  
Martin Lueck ◽  
Matthias Wickert ◽  
Jens Osterholz

AbstractWhen laser beams propagate through media with non-vanishing absorption, the media is heated resulting in a change of the refractive index, which can lead to thermal lensing and thermal blooming. However, experimental details about both phenomena for propagations in water are lacking, especially for high-power lasers in the kilowatt range. We show that significant thermal lensing occurs only for high input powers before the onset of convective flow, while for low input powers, no strong thermal lens arises. After the onset of water flow, thermal blooming occurs at low input powers comparable to that known for propagations over kilometres in the air. However, for high input powers a thermal blooming on a qualitatively higher level is shown. By wavefront sensing, the change of refractive index distribution in water is investigated. This clearly shows the fast development of a strong thermal lens for high input powers and the onset of convection. Furthermore, a qualitatively good agreement of the accompanying simulations is observed. It is found that the absorption coefficient is linear with a value of $$\mu ={13.7}\,{\mathrm{m}^{-1}}$$ μ = 13.7 m - 1 at least up to 7.5 kW, i.e. 8 $$\mathrm{kW/cm}^2$$ kW / cm 2 . However, the directed transmission into an aperture is only constant before any thermal lensing of blooming occurs.


We discuss the origin and characteristics of the very large intensity-dependent changes in the refractive index of the semiconductor cadmium mercury telluride at 10.6 m. With continuous wave (c.w.) radiation and sample temperatures of 77 K nonlinear Fabry-Perot effects can be observed at powers as low as 1 mW. The Auger dominated recombination process and the thermal contributions to the refractive index make observations of optical bistability difficult with c.w. radiation. However, the use of a pulsed CO 2 laser and two-photon absorption of the radiation does lead to the observation of bistability at room temperature. We compare these results with the reported work on InSb.


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