The impact of climate transitions on the radionuclide transport through a sedimentary aquifer

2019 ◽  
pp. 147-163
Author(s):  
Judith Flügge ◽  
Madlen Stockmann ◽  
Anke Schneider ◽  
Ulrich Noseck
Keyword(s):  
Radionuclide Transport ◽  
Sedimentary Aquifer ◽  
The Impact ◽  
Climate Transitions

scholarly journals Impact of the heterogeneity of the sandy Opalinus clay facies at the Mont Terri underground research laboratory on radionuclide migration

2021 ◽  
Vol 1 ◽  
pp. 141-142
Author(s):  
Naila Ait-Mouheb ◽  
Yuankai Yang ◽  
Luc R. Van Loon ◽  
Martin A. Glaus ◽  
Guido Deissmann ◽  
...  
Keyword(s):  
Research Laboratory ◽  
Radioactive Wastes ◽  
Coupled Processes ◽  
Opalinus Clay ◽  
Nuclear Waste Repository ◽  
Radionuclide Transport ◽  
Mont Terri ◽  
Underground Research Laboratory ◽  
Host Rocks ◽  
The Impact

Abstract. The assessment of the safety of a deep geological repository (DGR) for high-level radioactive wastes over assessment time scales of up to 1 million years requires an in-depth understanding of the multi-scale coupled processes that affect the repository system evolution over time, to reduce uncertainties and conservatism in safety analyses. This is in particular required with respect to the challenges of a comparative assessment of different repository concepts in different host rocks within the process of a site selection for a DGR for heat-generating radioactive wastes in Germany. The collaborative project “Integrity of nuclear waste repository systems – Cross-scale system understanding and analysis (iCross)” conducted jointly by five research centres of the Helmholtz Association and co-funded by the Initiative and Networking Fund of the Helmholtz Association and the Federal Ministry of Education and Research (BMBF) has been initiated with the overall objective to improve the understanding of coupled thermal-hydraulic-mechanical-chemical-(micro)biological (THMCB) processes and to develop simulation tools that enable a holistic close to reality description of the long-term evolution of the repository system. Geological formations, such as those foreseen as potential host rocks for DGRs, and their surroundings are heterogeneous on various length scales ranging from nanometers to kilometers. Therefore, the aim of this work in the context of iCross is to evaluate the effects of mineralogical, geochemical and microstructural heterogeneities of repository host rocks on radionuclide transport in the repository far field, using the sandy facies of the Opalinus clay (SF-OPA) from the Mont Terri underground research laboratory (St. Ursanne, Switzerland) as an example. Here, we address in particular the migration behaviour of Ra-226 as an important radionuclide to be considered in safety cases for deep geological disposal of spent nuclear fuel. To assess the impact of the heterogeneities in SF-OPA on radionuclide transport, a complementary approach combining microstructural characterisation methods, experimental techniques for the determination of transport parameters of the rock matrix and the mobility of Ra-226 with innovative developments in reactive transport modelling on the pore and continuum scales was pursued. One of the results was that although the limited clay content in SF-OPA decreases the total amount of Ra bound to the illite phase, the solid solutions of sulphate and carbonate compensate for this and provide a major fixation mechanism.

Influence of distribution co-efficient on radionuclide transport modelling of uranium from a tailings pond in northern Karnataka, India

2020 ◽  
Author(s):  
Bhavya Ravinder ◽  
Elango Lakshmanan
Keyword(s):  
Drinking Water ◽  
Transport Model ◽  
Uranium Mining ◽  
Radionuclide Transport ◽  
Transport Modelling ◽  
Natural Systems ◽  
Tailings Pond ◽  
Surface Method ◽  
Input Source ◽  
The Impact

<p>A well-designed environmental monitoring plan is essential for safety of uranium mining and processing operations. Evaluating the possible uncertainties in a numerical model helps in enhancing the model output and also increases the reliability over the model results. For a radionuclide transport model, distribution co-efficient is a sensitive parameter and major source of uncertainty in results. In this study, an approach to quantify input source of uncertainty of distribution co-efficient in an engineered tailings pond in Northern Karnataka, India has been carried out. Probabilistic analysis such as Response Surface Method and Monte Carlo Simulation are used to propagate uncertainty. This study considers uncertainty associated with intrinsic heterogeneity of natural systems and estimates the probability that dose rate value through drinking water pathway around the tailings pond exceeds the WHO guidelines for drinking water. The radionuclides considered in this study are <sup>238</sup>U, <sup>234</sup>U, <sup>230</sup>Th and <sup>226</sup>Ra. This study can be used to study the impact of distribution co-efficient on the radionuclide transport model.</p><p>Key words: Numerical modelling, Tailings pond area, Uranium mining, Uncertainty,  Distribution coefficient</p><p> </p>

scholarly journals An interdisciplinary view of the long-term evolution of repository systems across scales: the iCROSS project

2021 ◽  
Vol 1 ◽  
pp. 85-87
Author(s):  
Dirk Bosbach ◽  
Horst Geckeis ◽  
Frank Heberling ◽  
Olaf Kolditz ◽  
Michael Kühn ◽  
...  
Keyword(s):  
Radioactive Waste ◽  
Field Experiments ◽  
Coupled Processes ◽  
Nuclear Waste Repository ◽  
Radionuclide Transport ◽  
Clay Rock ◽  
Rock Characterization ◽  
Mont Terri ◽  
The Impact

Abstract. The interdisciplinary project “Integrity of nuclear waste repository systems – Cross-scale system understanding and analysis (iCROSS)” combines research competencies of Helmholtz scientists related to the topics of nuclear, geosciences, biosciences and environmental simulations in collaborations overarching the research fields energy and earth and environment. The focus is to understand and analyze close-to-real long-term evolutionary pathways of radioactive waste repositories across nanoscales to repository scales. The project is subdivided into work packages dealing with laboratory studies, field experiments in underground research laboratories (URLs), advanced modelling studies and the integration and alignment of data and information using virtual reality methods. In this sense, the project structure aims at a holistic view on relevant processes across scales in order to comprehensively simulate potential repository evolutions. Within the multi-barrier system of a repository for heat-generating radioactive waste, a number of complex reactions proceed, including dissolution, redox processes, biochemical reactions, gas evolution and solid/liquid interface and (co)precipitation reactions. At the same time, thermal and external mechanical stress has an impact on the conditions in a deep geological repository. All those processes are highly coupled, with multiple interdependencies on various scales and have a strong impact on radionuclide mobility and retention. In recent years, substantial progress was achieved in describing coupled thermal-hydro-mechanical-chemical-biological (THM/CB) processes in numerical simulations. A realistic and concise description of these coupled processes on different time and spatial scales is, at present, a largely unresolved scientific and computational challenge. The close interaction of experimental and simulation teams aims at a more accurate quantification and assessment of processes and thus, the reduction of uncertainties and of conservative assumptions and eventually to a close-to-real perception of the repository evolution. One focus of iCROSS is directed to relevant processes in a clay rock repository. In this context, the iCROSS team became a full member of the international Mont Terri consortium and worked in close collaboration with international and German institutions in URL projects. Respective experiments specifically deal with coupled processes at the reactive interfaces in a repository near field (e.g. the steel/bentonite and bentonite/concrete interfaces). Within iCROSS, the impact of secondary phase formation on radionuclide transport is investigated. At Mont Terri, experiments are in preparation to study radionuclide transport phenomena in clay rock formations within temperature gradients and in facies exhibiting significant heterogeneities on different scales (nm to cm). Beside those studies, high resolution exploration methods for rock characterization are developed and tested and the effect of temperature and other boundary conditions on the strength, creep properties and healing of faults within Opalinus clay are quantified. Multiphysics models coupled to reactive transport simulation have been further developed and applied to laboratory and field experiments. Results are digitally analyzed and illustrated in a visualization center, in order to enhance the comprehension of coupled processes in repository systems across scales. The present contribution provides an overview on the project and reports selected results. The impact of considering complex coupled processes in repository subsystems for the assessment of the integrity of a given (generic) repository arrangement is discussed.

scholarly journals Eddy permitting simulations of freshwater injection from major Northern Hemisphere outlets during the last deglacial

2021 ◽  
Author(s):  
Ryan Love ◽  
Heather Andres ◽  
Alan Condron ◽  
Lev Tarasov
Keyword(s):  
North Atlantic ◽  
Large Scale ◽  
Critical Role ◽  
The Arctic ◽  
Bering Strait ◽  
The North ◽  
Glacial Runoff ◽  
The North Atlantic ◽  
The Impact ◽  
Climate Transitions

Abstract. Freshwater, in the form of glacial runoff, is hypothesized to play a critical role in centennial to millennial scale climate variability such as the Younger Dryas and Dansgaard-Oeschger Events. Indeed, freshwater injection/hosing experiments with climate models have long shown that freshwater has the capability of generating such abrupt climate transitions. However, the relationship between freshwater and abrupt climate transitions is not straightforward. Large-scale glacial runoff events, such as Meltwater Pulse 1A, are not always temporally proximal to subsequent large-scale cooling. As well, the typical design of hosing experiments tends to artificially amplify the climate response. This study explores the impact that limitations in the representation of runoff in conventional hosing simulations has on our understanding of this relationship and addresses the more fundamental question of where coastally released freshwater is transported when it reaches the ocean. We focus particularly on the prior use of excessive freshwater volumes (often by a factor of 5) and present-day (rather than paleo) ocean gateways, as well as the injection of freshwater directly over sites of deep-water formation (DWF) rather than at runoff locations. We track the routing of glaciologically-constrained freshwater volumes from four different plausible injection locations in a suite of eddy-permitting glacial ocean simulations using MITGCM under both open and closed Bering Strait conditions. Restricting freshwater forcing values to realistic ranges results in less spreading of freshwater across the North Atlantic and indicates that the response of DWF depends strongly on the geographical location of meltwater input. In particular, freshwater released into the Gulf of Mexico has little impact on DWF regions as a result of turbulent mixing by the Gulf Stream. In contrast, freshwater released from the Eurasian Ice sheet or initially into the Arctic is found to have the largest impact on DWF in the North Atlantic and GIN seas. Additional experiments show that when the Bering Strait is open, much like present-day, the Mackenzie River source exhibits twice as much freshening of the Labrador sea as a closed Bering Strait. Finally, our results illustrate that applying a freshwater hosing directly into the North Atlantic with even realistic freshwater amounts still over-estimates the effect of terrestrial runoff on ocean circulation.

scholarly journals NUMERICAL SIMULATION OF THE IMPACT OF WATER-AIR FRONTS ON RADIONUCLIDE PLUMES IN HETEROGENEOUS MEDIA

2006 ◽  
Vol 5 (1) ◽  
pp. 46
Author(s):  
J. Aquino ◽  
A. S. Francisco ◽  
F. Pereira ◽  
H. P. Amaral Souto
Keyword(s):  
Heterogeneous Media ◽  
Flow Problem ◽  
Mixed Finite Element ◽  
Air Flow ◽  
Heterogeneous Porous Media ◽  
Radionuclide Transport ◽  
Central Difference ◽  
Modified Method ◽  
Modified Method Of Characteristics ◽  
The Impact

The goal of this paper is to investigate the interaction of water-air fronts with radionuclide plumes in unsaturated heterogeneous porous media. This problem is modeled by a system of equations that describes both water-air flow and radionuclide transport. The water-air flow problem is solved numerically by a mixed finite element combined with a non-oscillatory central difference scheme. For the radionuclide transport equation we use the Modified Method of Characteristics (MMOC).We present results of numerical simulations for heterogeneous permeability fields taking into account sorption effects.

Radionuclide Transport Calculations in the Safety Assessment SR 97

2000 ◽  
Vol 663 ◽  
Author(s):  
M. Lindgren ◽  
F. Lindström
Keyword(s):  
Input Data ◽  
Safety Assessment ◽  
Spent Nuclear Fuel ◽  
Near Field ◽  
Radionuclide Transport ◽  
Spent Fuel ◽  
Release Rates ◽  
Dose Limits ◽  
The Impact ◽  
Different Parts

ABSTRACTThis study treats radionuclide transport calculations for a canister defect scenario in the safety assessment SR 97, which concerns a deep repository for spent nuclear fuel of the KBS-3 type in Sweden. The aims of the calculations are to:Quantitatively describe the radionuclide transport.Show the impact of uncertainty in input data and show which parameters govern the calculated release rates.Compare three different real sites in Sweden (Aberg, Beberg and Ceberg) with each other and with dose limits given in Swedish regulations (none of the sites is considered in the on-going localization process). Only briefly described in this paper.Illustrate the impact of the different barriers in the system.Deterministic calculations illustrate the radionuclide transport for reasonable conditions. Uncertainty cases show the influence of the uncertainty for data related to different parts of the repository system by systematically giving them pessimistic values while all others are reasonable. Simplified probabilistic calculations have also been performed.The analysis shows that the most important parameters in the near field are the number of defective canisters and the instant release fraction. In the far field the most important uncertainties affecting release and retention are connected to permeability and connectivity of the fractures in the rock. The dose rate in the biosphere is essentially controlled by the possibilities of dilution.The calculated maximum doses for the hypothetical repositories are well below the dose limits, and hence they meet the acceptance criteria for a deep repository for spent fuel.

Formation of Lunar Craters and Bright Rays as a Result of Meteorite Impacts

1962 ◽  
Vol 14 ◽  
pp. 415-418
Author(s):  
K. P. Stanyukovich ◽  
V. A. Bronshten
Keyword(s):  
Explosive Charge ◽  
The Moon ◽  
Meteorite Impacts ◽  
The Earth ◽  
Lunar Craters ◽  
The Impact

The phenomena accompanying the impact of large meteorites on the surface of the Moon or of the Earth can be examined on the basis of the theory of explosive phenomena if we assume that, instead of an exploding meteorite moving inside the rock, we have an explosive charge (equivalent in energy), situated at a certain distance under the surface.

The Geosciences Applied to Lunar Exploration

1962 ◽  
Vol 14 ◽  
pp. 169-257 ◽  
Author(s):  
J. Green
Keyword(s):  
Lunar Surface ◽  
Probable Mechanism ◽  
Point Of View ◽  
Lunar Exploration ◽  
Geological Model ◽  
Apply Geophysics ◽  
Surface Features ◽  
The Impact

The term geo-sciences has been used here to include the disciplines geology, geophysics and geochemistry. However, in order to apply geophysics and geochemistry effectively one must begin with a geological model. Therefore, the science of geology should be used as the basis for lunar exploration. From an astronomical point of view, a lunar terrain heavily impacted with meteors appears the more reasonable; although from a geological standpoint, volcanism seems the more probable mechanism. A surface liberally marked with volcanic features has been advocated by such geologists as Bülow, Dana, Suess, von Wolff, Shaler, Spurr, and Kuno. In this paper, both the impact and volcanic hypotheses are considered in the application of the geo-sciences to manned lunar exploration. However, more emphasis is placed on the volcanic, or more correctly the defluidization, hypothesis to account for lunar surface features.

Asteroid and Comet Impact Speeds upon Mars: Significance for Panspermia and the Supply of Organics

1997 ◽  
Vol 161 ◽  
pp. 197-201 ◽  
Author(s):  
Duncan Steel
Keyword(s):  
Probability Distributions ◽  
Regions Of Interest ◽  
Significant Fraction ◽  
Organic Chemicals ◽  
Impact Speed ◽  
The Mean ◽  
The Impact

AbstractWhilst lithopanspermia depends upon massive impacts occurring at a speed above some limit, the intact delivery of organic chemicals or other volatiles to a planet requires the impact speed to be below some other limit such that a significant fraction of that material escapes destruction. Thus the two opposite ends of the impact speed distributions are the regions of interest in the bioastronomical context, whereas much modelling work on impacts delivers, or makes use of, only the mean speed. Here the probability distributions of impact speeds upon Mars are calculated for (i) the orbital distribution of known asteroids; and (ii) the expected distribution of near-parabolic cometary orbits. It is found that cometary impacts are far more likely to eject rocks from Mars (over 99 percent of the cometary impacts are at speeds above 20 km/sec, but at most 5 percent of the asteroidal impacts); paradoxically, the objects impacting at speeds low enough to make organic/volatile survival possible (the asteroids) are those which are depleted in such species.

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