Intercomparison of Bulk Cloud Microphysics Schemes in Mesoscale Simulations of Springtime Arctic Mixed-Phase Stratiform Clouds

2006 ◽  
Vol 134 (7) ◽  
pp. 1880-1900 ◽  
Author(s):  
H. Morrison ◽  
J. O. Pinto

Abstract A persistent, weakly forced, horizontally extensive mixed-phase boundary layer cloud observed on 4–5 May 1998 during the Surface Heat Budget of the Arctic Ocean (SHEBA)/First International Satellite Cloud Climatology Project (ISCCP) Regional Experiment–Arctic Clouds Experiment (FIRE–ACE) is modeled using three different bulk microphysics parameterizations of varying complexity implemented into the polar version of the fifth-generation Pennsylvania State University–National Center for Atmospheric Research Mesoscale Model (MM5). The two simpler schemes predict mostly ice clouds and very little liquid water, while the complex scheme is able to reproduce the observed persistence and horizontal extent of the mixed-phase stratus deck. This mixed-phase cloud results in radiative warming of the surface, the development of a cloud-topped, surface-based mixed layer, and an enhanced precipitation rate. In contrast, the optically thin ice clouds predicted by the simpler schemes lead to radiative cooling of the surface, a strong diurnal cycle in the boundary layer structure, and very weak precipitation. The larger surface precipitation rate using the complex scheme is partly balanced by an increase in the turbulent flux of water vapor from the surface to the atmosphere. This enhanced vapor flux is attributed to changes in the surface and boundary layer characteristics induced by the cloud itself, although cloud–surface interactions appear to be exaggerated in the model compared with reality. The prediction of extensive mixed-phase stratus by the complex scheme is also associated with increased surface pressure and subsidence relative to the other simulations. Sensitivity tests show that the detailed treatment of ice nucleation and prediction of snow particle number concentration in the complex scheme suppresses ice particle concentration relative to the simpler schemes, reducing the vapor deposition rate (for given values of bulk ice mass and ice supersaturation) and leading to much greater amounts of liquid water and mixed-phase cloudiness. These results suggest that the treatments of ice nucleation and the snow intercept parameter in the simpler schemes, which are based upon midlatitude observations, are inadequate for simulating the weakly forced mixed-phase clouds endemic to the Arctic.

2008 ◽  
Vol 8 (4) ◽  
pp. 15901-15939 ◽  
Author(s):  
A. Ehrlich ◽  
E. Bierwirth ◽  
M. Wendisch ◽  
J.-F. Gayet ◽  
G. Mioche ◽  
...  

Abstract. Boundary layer clouds were investigated with a complementary set of remote sensing and in situ instruments during the Arctic Study of Tropospheric Aerosol, Clouds and Radiation (ASTAR) campaign in March and April 2007. The clouds that formed in a cold air outbreak over the open Greenland sea showed a variety in their thermodynamic state. Beside the predominant mixed-phase clouds pure liquid and ice clouds were observed. Utilizing the measurements of solar radiation reflected by the clouds three methods to retrieve the thermodynamic phase of the cloud were defined and compared. Two ice indices IS and IP were obtained by analyzing the spectral pattern of the cloud top reflectance in the near infrared (1500–1800 nm wavelength) characterized by ice and water absorption. A third ice index IA is based on the different side scattering of spherical liquid water particles and nonspherical ice crystals which was recorded in simultaneous measurements of cloud albedo and reflectance. Radiative transfer simulations showed that IS, IP and IA range between 5 to 80, 0 to 20 and 1 to 1.25, respectively, with lowest values indicating pure liquid water clouds and highest values pure ice clouds. IS and IP were found to be strongly sensitive to the effective diameter of the ice crystals present in the cloud. Therefore the identification of mixed-phase clouds requires a priori knowledge of the ice crystal dimension. IA has the disadvantage that this index is mainly dominated by the uppermost cloud layer (τ<1.5). Typical boundary layer mixed-phase clouds with a liquid cloud top layer will be identified as pure liquid water clouds. All three methods were applied to measurements above a cloud field observed during ASTAR 2007. The comparison with independent in situ microphysical measurements showed a good agreement in identifying the dominant mixed-phase clouds and a pure ice cloud at the edge of the cloud field.


2010 ◽  
Vol 10 (2) ◽  
pp. 4027-4077 ◽  
Author(s):  
A. Wiacek ◽  
T. Peter ◽  
U. Lohmann

Abstract. This modelling study explores the availability of mineral dust particles as ice nuclei for interactions with ice, mixed-phase and liquid water clouds, also tracking the particles' history of cloud-processing. We performed 61 320 one-week forward trajectory calculations originating near the surface of major dust emitting regions in Africa and Asia using high-resolution meteorological analysis fields for the year 2007. Without explicitly modelling dust emission and deposition processes, dust-bearing trajectories were assumed to be those coinciding with known dust emission seasons. We found that dust emissions from Asian deserts lead to a higher potential for interactions with high clouds, despite being the climatologically much smaller dust emission source. This is due to Asian regions experiencing significantly more ascent than African regions, with strongest ascent in the Asian Taklimakan desert at ~25%, ~40% and 10% of trajectories ascending to 300 hPa in spring, summer and fall, respectively. The specific humidity at each trajectory's starting point was transported in a Lagrangian manner and relative humidities with respect to water and ice were calculated in 6-h steps downstream, allowing us to estimate the formation of liquid, mixed-phase and ice clouds. Practically none of the simulated air parcels reached regions where homogeneous ice nucleation can take place (T≲−40 °C) along trajectories that have not experienced water saturation first. By far the largest fraction of cloud forming trajectories entered conditions of mixed-phase clouds, where mineral dust will potentially exert the biggest influence. The majority of trajectories also passed through regions supersaturated with respect to ice but subsaturated with respect to water, where "warm" (T≳−40 °C) ice clouds may form prior to supercooled water or mixed-phase clouds. The importance of "warm" ice clouds and the general influence of dust in the mixed-phase cloud region are highly uncertain due to considerable scatter in recent laboratory data from ice nucleation experiments, which we briefly review in this work. For "classical" cirrus-forming temperatures, our results show that only mineral dust IN that underwent mixed-phase cloud-processing previously are likely to be relevant, and, therefore, we recommend further systematic studies of immersion mode ice nucleation on mineral dust suspended in atmospherically relevant coatings.


2010 ◽  
Vol 10 (18) ◽  
pp. 8649-8667 ◽  
Author(s):  
A. Wiacek ◽  
T. Peter ◽  
U. Lohmann

Abstract. This modelling study explores the availability of mineral dust particles as ice nuclei for interactions with ice, mixed-phase and liquid water clouds, also tracking the particles' history of cloud-processing. We performed 61 320 one-week forward trajectory calculations originating near the surface of major dust emitting regions in Africa and Asia using high-resolution meteorological analysis fields for the year 2007. Dust-bearing trajectories were assumed to be those coinciding with known dust emission seasons, without explicitly modelling dust emission and deposition processes. We found that dust emissions from Asian deserts lead to a higher potential for interactions with high ice clouds, despite being the climatologically much smaller dust emission source. This is due to Asian regions experiencing significantly more ascent than African regions, with strongest ascent in the Asian Taklimakan desert at ~25%, ~40% and 10% of trajectories ascending to 300 hPa in spring, summer and fall, respectively. The specific humidity at each trajectory's starting point was transported in a Lagrangian manner and relative humidities with respect to water and ice were calculated in 6-h steps downstream, allowing us to estimate the formation of liquid, mixed-phase and ice clouds. Downstream of the investigated dust sources, practically none of the simulated air parcels reached conditions of homogeneous ice nucleation (T≲−40 °C) along trajectories that have not experienced water saturation first. By far the largest fraction of cloud forming trajectories entered conditions of mixed-phase clouds, where mineral dust will potentially exert the biggest influence. The majority of trajectories also passed through atmospheric regions supersaturated with respect to ice but subsaturated with respect to water, where so-called "warm ice clouds" (T≳−40 °C) theoretically may form prior to supercooled water or mixed-phase clouds. The importance of "warm ice clouds" and the general influence of dust in the mixed-phase cloud region are highly uncertain due to both a considerable scatter in recent laboratory data from ice nucleation experiments, which we briefly review in this work, and due to uncertainties in sub-grid scale vertical transport processes unresolved by the present trajectory analysis. For "classical" cirrus-forming temperatures (T≲−40 °C), our results show that only mineral dust ice nuclei that underwent mixed-phase cloud-processing, most likely acquiring coatings of organic or inorganic material, are likely to be relevant. While the potential paucity of deposition ice nuclei shown in this work dimishes the possibility of deposition nucleation, the absence of liquid water droplets at T≲−40 °C makes the less explored contact freezing mechanism (involving droplet collisions with bare ice nuclei) highly inefficient. These factors together indicate the necessity of further systematic studies of immersion mode ice nucleation on mineral dust suspended in atmospherically relevant coatings.


2020 ◽  
Vol 13 (11) ◽  
pp. 5737-5755
Author(s):  
Setigui Aboubacar Keita ◽  
Eric Girard ◽  
Jean-Christophe Raut ◽  
Maud Leriche ◽  
Jean-Pierre Blanchet ◽  
...  

Abstract. In the Arctic, during polar night and early spring, ice clouds are separated into two leading types of ice clouds (TICs): (1) TIC1 clouds characterized by a large concentration of very small crystals and TIC2 clouds characterized by a low concentration of large ice crystals. Using a suitable parameterization of heterogeneous ice nucleation is essential for properly representing ice clouds in meteorological and climate models and subsequently understanding their interactions with aerosols and radiation. Here, we describe a new parameterization for ice crystal formation by heterogeneous nucleation in water-subsaturated conditions coupled to aerosol chemistry in the Weather Research and Forecasting model coupled with chemistry (WRF-Chem). The parameterization is implemented in the Milbrandt and Yau (2005a, b) two-moment cloud microphysics scheme, and we assess how the WRF-Chem model responds to the run-time interaction between chemistry and the new parameterization. Well-documented reference cases provided us with in situ data from the spring 2008 Indirect and Semi-Direct Aerosol Campaign (ISDAC) over Alaska. Our analysis reveals that the new parameterization clearly improves the representation of the ice water content (IWC) in polluted or unpolluted air masses and shows the poor performance of the reference parameterization in representing ice clouds with low IWC. The new parameterization is able to represent TIC1 and TIC2 microphysical characteristics at the top of the clouds, where heterogenous ice nucleation is most likely occurring, even with the known bias of simulated aerosols by WRF-Chem over the Arctic.


2005 ◽  
Vol 44 (4) ◽  
pp. 427-444 ◽  
Author(s):  
D. D. Turner

Abstract A new approach to retrieve microphysical properties from mixed-phase Arctic clouds is presented. This mixed-phase cloud property retrieval algorithm (MIXCRA) retrieves cloud optical depth, ice fraction, and the effective radius of the water and ice particles from ground-based, high-resolution infrared radiance and lidar cloud boundary observations. The theoretical basis for this technique is that the absorption coefficient of ice is greater than that of liquid water from 10 to 13 μm, whereas liquid water is more absorbing than ice from 16 to 25 μm. MIXCRA retrievals are only valid for optically thin (τvisible &lt; 6) single-layer clouds when the precipitable water vapor is less than 1 cm. MIXCRA was applied to the Atmospheric Emitted Radiance Interferometer (AERI) data that were collected during the Surface Heat Budget of the Arctic Ocean (SHEBA) experiment from November 1997 to May 1998, where 63% of all of the cloudy scenes above the SHEBA site met this specification. The retrieval determined that approximately 48% of these clouds were mixed phase and that a significant number of clouds (during all 7 months) contained liquid water, even for cloud temperatures as low as 240 K. The retrieved distributions of effective radii for water and ice particles in single-phase clouds are shown to be different than the effective radii in mixed-phase clouds.


2009 ◽  
Vol 9 (3) ◽  
pp. 11333-11366 ◽  
Author(s):  
J.-F. Gayet ◽  
G. Mioche ◽  
A. Dörnbrack ◽  
A. Ehrlich ◽  
A. Lampert ◽  
...  

Abstract. Airborne measurements in Arctic boundary-layer stratocumulus were carried out near Spitsbergen on 9 April 2007 during the Arctic Study of Tropospheric Aerosol, Clouds and Radiation (ASTAR) campaign. A unique set of co-located observations is used to describe the cloud properties, including detailed in situ cloud microphysical and radiation measurements along with airborne and co-located spaceborne remote sensing data (Lidar on Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observations [CALIPSO] and radar on CloudSat satellites). The CALIPSO profiles evidence a cloud top temperature which varies between −24°C and −21°C. The in situ cloud observations reveal that the attenuated backscatter signal from lidar along the aircraft trajectory is linked with the presence of liquid water and therefore confirms a cloud top layer dominated by liquid-water, which is a common feature observed in Arctic mixed-phase stratocumulus clouds. A low concentration of quite large ice crystals are also evidenced up to the cloud top and lead to significant CloudSat radar echo. Since the ratio of the extinction of liquid water droplets and ice crystals is high the broadband radiative effects near the cloud top are mostly dominated by water droplets. CloudSat observations as well as in situ measurements reveal high reflectivity factors (up to 15 dBZ) and precipitation rates (1 mm h−1). This feature is due to efficient ice production processes. About 25% of the theoretically available liquid water is converted into ice water with large ice crystals which precipitate. According to an estimation of the mean cloud cover, a considerable value of 106 m3 h−1 of fresh water could be settled over the Greenland sea pool. European Centre for Medium-Range Weather Forecast (ECMWF) operational analyses reproduces the variation of the boundary layer height along the flight track. However, small-scale features in the observed cloud field cannot be resolved by ECMWF analysis. Furthermore, ECMWF's diagnostic partitioning of the condensed water into ice and liquid reveals serious shortcomings for Arctic mixed-phased clouds. Too much ice is modeled.


2020 ◽  
Author(s):  
Setigui Aboubacar Keita ◽  
Eric Girard ◽  
Jean-Christophe Raut ◽  
Maud Leriche ◽  
Jean-Pierre Blanchet ◽  
...  

Abstract. In the Arctic, during polar night and early spring, ice clouds are separated into two leading types: (1) TIC1 clouds characterized by large concentration of very small crystals, and TIC2 clouds characterized by low concentration of large ice crystals. Using suitable parameterization of heterogeneous ice nucleation is essential for properly representing ice cloud in meteorological and climate model and subsequently understanding their interactions with aerosols and radiation. Here, we describe a new parameterization for ice crystals formation by heterogeneous nucleation coupled to aerosols chemistry in WRF-Chem. The parameterization is implemented in the Milbrandt and Yau’s two-moment cloud microphysics scheme and we assess how the WRF-Chem model responds to the real time interaction between chemistry and the new parameterization. Well-documented reference cases provided us in situ data from the spring 2008 Indirect and Semi-Direct Aerosol Campaign (ISDAC) campaign over Alaska. Our analysis reveals that the new parameterization clearly improves the representation of the IWC in polluted or unpolluted air masses and shows the poor performance of the reference parameterization in representing ice clouds with low IWC. The new parameterization is, thus able to represent TIC1 and TIC2 microphysical characteristics at the top of the clouds were heterogeneous ice nucleation is most likely occurring even knowing the bias of simulated aerosols by WRF-Chem over Arctic.


2008 ◽  
Vol 8 (24) ◽  
pp. 7493-7505 ◽  
Author(s):  
A. Ehrlich ◽  
E. Bierwirth ◽  
M. Wendisch ◽  
J.-F. Gayet ◽  
G. Mioche ◽  
...  

Abstract. Arctic boundary-layer clouds were investigated with remote sensing and in situ instruments during the Arctic Study of Tropospheric Aerosol, Clouds and Radiation (ASTAR) campaign in March and April 2007. The clouds formed in a cold air outbreak over the open Greenland Sea. Beside the predominant mixed-phase clouds pure liquid water and ice clouds were observed. Utilizing measurements of solar radiation reflected by the clouds three methods to retrieve the thermodynamic phase of the cloud are introduced and compared. Two ice indices IS and IP were obtained by analyzing the spectral pattern of the cloud top reflectance in the near infrared (1500–1800 nm wavelength) spectral range which is characterized by ice and water absorption. While IS analyzes the spectral slope of the reflectance in this wavelength range, IS utilizes a principle component analysis (PCA) of the spectral reflectance. A third ice index IA is based on the different side scattering of spherical liquid water particles and nonspherical ice crystals which was recorded in simultaneous measurements of spectral cloud albedo and reflectance. Radiative transfer simulations show that IS, IP and IA range between 5 to 80, 0 to 8 and 1 to 1.25 respectively with lowest values indicating pure liquid water clouds and highest values pure ice clouds. The spectral slope ice index IS and the PCA ice index IP are found to be strongly sensitive to the effective diameter of the ice crystals present in the cloud. Therefore, the identification of mixed-phase clouds requires a priori knowledge of the ice crystal dimension. The reflectance-albedo ice index IA is mainly dominated by the uppermost cloud layer (τ<1.5). Therefore, typical boundary-layer mixed-phase clouds with a liquid cloud top layer will be identified as pure liquid water clouds. All three methods were applied to measurements above a cloud field observed during ASTAR 2007. The comparison with independent in situ microphysical measurements shows the ability of the three approaches to identify the ice phase in Arctic boundary-layer clouds.


2005 ◽  
Vol 44 (10) ◽  
pp. 1544-1562 ◽  
Author(s):  
Matthew D. Shupe ◽  
Taneil Uttal ◽  
Sergey Y. Matrosov

Abstract An operational suite of ground-based, remote sensing retrievals for producing cloud microphysical properties is described, assessed, and applied to 1 yr of observations in the Arctic. All measurements were made in support of the Surface Heat Budget of the Arctic (SHEBA) program and First International Satellite Cloud Climatology Project Regional Experiment (FIRE) Arctic Clouds Experiment (ACE) in 1997–98. Retrieval techniques and cloud-type classifications are based on measurements from a vertically pointing 35-GHz Doppler radar, microwave and infrared radiometers, and radiosondes. The retrieval methods are assessed using aircraft in situ measurements from a limited set of case studies and by intercomparison of multiple retrievals for the same parameters. In all-liquid clouds, retrieved droplet effective radii Re have an uncertainty of up to 32% and liquid water contents (LWC) have an uncertainty of 49%–72%. In all-ice clouds, ice particle mean sizes Dmean can be retrieved with an uncertainty of 26%–46% while retrieved ice water contents (IWC) have an uncertainty of 62%–100%. In general, radar-only, regionally tuned empirical power-law retrievals were best suited among the tested retrieval algorithms for operational cloud monitoring at SHEBA because of their wide applicability, ease of use, and reasonable statistical accuracy. More complex multisensor techniques provided a moderate improvement in accuracy for specific case studies and were useful for deriving location-specific coefficients for the empirical retrievals but were not as frequently applicable as the single sensor methods because of various limitations. During the yearlong SHEBA program, all-liquid clouds were identified 19% of the time and were characterized by an annual average droplet Re of 6.5 μm, LWC of 0.10 g m−3, and liquid water path of 45 g m−2. All-ice clouds were identified 38% of the time with an annual average particle Dmean of 73 μm, IWC of 0.014 g m−3, and ice water path of 30 g m−2.


2009 ◽  
Vol 9 (17) ◽  
pp. 6581-6595 ◽  
Author(s):  
J.-F. Gayet ◽  
G. Mioche ◽  
A. Dörnbrack ◽  
A. Ehrlich ◽  
A. Lampert ◽  
...  

Abstract. Airborne measurements in Arctic boundary-layer stratocumulus were carried out near Spitsbergen on 9 April 2007 during the Arctic Study of Tropospheric Aerosol, Clouds and Radiation (ASTAR) campaign. A unique set of co-located observations is used to describe the cloud properties, including detailed in situ cloud microphysical and radiation measurements along with airborne and co-located spaceborne remote sensing data (CALIPSO lidar and CloudSat radar). CALIPSO profiles indicate cloud top levels at temperature between −24°C and −21°C. In situ measurements confirm that the cloud-top lidar attenuated backscatter signal along the aircraft trajectory is linked with the presence of liquid water, a common feature observed in Arctic mixed-phase stratocumulus clouds. A low concentration of large ice crystals is also observed up to the cloud top resulting in significant CloudSat radar echoes. Since the ratio of the extinction of liquid water droplets to ice crystals is high, broadband radiative effects near the cloud top are mostly dominated by water droplets. CloudSat observations and in situ measurements reveal high reflectivity factors (up to 15 dBZ) and precipitation rates (1 mm h−1). This feature results from efficient ice growth processes. About 25% of the theoretically available liquid water is converted into ice water with large precipitating ice crystals. Using an estimate of mean cloud cover, a considerable value of 106 m3 h−1 of fresh water could be settled over the Greenland sea pool. European Centre for Medium-Range Weather Forecast (ECMWF) operational analyses reproduces the boundary layer height variation along the flight track. However, small-scale features in the observed cloud field cannot be resolved by ECMWF analysis. Furthermore, ECMWF's diagnostic partitioning of the condensed water into ice and liquid reveals serious shortcomings for Arctic mixed-phased clouds. Too much ice is modelled.


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