scholarly journals The Impact of Warm and Moist Airmass Perturbations on Arctic Mixed-Phase Stratocumulus

2020 ◽  
Vol 33 (22) ◽  
pp. 9615-9628
Author(s):  
Gesa K. Eirund ◽  
Anna Possner ◽  
Ulrike Lohmann
Keyword(s):  
Boundary Layer ◽  
Sea Ice ◽  
Lower Troposphere ◽  
Temperature Inversion ◽  
Open Ocean ◽  
Mixed Phase ◽  
Specific Humidity ◽  
The Arctic ◽  
Free Troposphere ◽  
The Impact

AbstractThe Arctic is known to be particularly sensitive to climate change. This Arctic amplification has partially been attributed to poleward atmospheric heat transport in the form of airmass intrusions. Locally, such airmass intrusions can introduce moisture and temperature perturbations. The effect of airmass perturbations on boundary layer and cloud changes and their impact on the surface radiative balance has received increased attention, especially over sea ice with regard to sea ice melt. Utilizing cloud-resolving model simulations, this study addresses the impact of airmass perturbations occurring at different altitudes on stratocumulus clouds for open-ocean conditions. It is shown that warm and moist airmass perturbations substantially affect the boundary layer and cloud properties, even for the relatively moist environmental conditions over the open ocean. The cloud response is driven by temperature inversion adjustments and strongly depends on the perturbation height. Boundary layer perturbations weaken and raise the inversion, which destabilizes the lower troposphere and involves a transition from stratocumulus to cumulus clouds. In contrast, perturbations occurring in the lower free troposphere lead to a lowering but strengthening of the temperature inversion, with no impact on cloud fraction. In simulations where free-tropospheric specific humidity is further increased, multilayer mixed-phase clouds form. Regarding energy balance changes, substantial surface longwave cooling arises out of the stratocumulus break-up simulated for boundary layer perturbations. Meanwhile, the net surface longwave warming increases resulting from thicker clouds for airmass perturbations occurring in the lower free troposphere.

Pan-Arctic surface ozone seasonality modified by sea-ice-sourced bromine: modelling vs measurements

2021 ◽  
Author(s):  
Xin Yang ◽  
Anne-M Blechschmidt2 ◽  
Kristof Bognar ◽  
Audra McClure–Begley ◽  
Sara Morris ◽  
...  
Keyword(s):  
Boundary Layer ◽  
Sea Ice ◽  
Surface Ozone ◽  
Open Ocean ◽  
Arctic Sea Ice ◽  
The Arctic ◽  
Sea Spray ◽  
Research Station ◽  
Blowing Snow ◽  
Model Control

<p>Within the framework of the International Arctic Systems for Observing the Atmosphere (IASOA), we report a modelling-based study on surface ozone across the Arctic. We use surface ozone from six sites: Summit (Greenland), Pallas (Finland), Barrow (USA), Alert (Canada), Tiksi (Russia), and Villum Research Station (VRS) at Station Nord (North Greenland, Danish Realm), and ozonesonde data from three Canadian sites: Resolute, Eureka, and Alert. Two global chemistry models: a global chemistry transport model (p-TOMCAT) and a global chemistry climate model (UKCA), are used for model-data comparisons. Remotely sensed data of BrO from the GOME-2 satellite instrument at Eureka, Canada are used for model validation.</p><p>The observed climatology data show that spring surface ozone at coastal Arctic is heavily depleted, making ozone seasonality at Arctic coastal sites distinctly different from that at inland sites. Model simulations show that surface ozone can be greatly reduced by bromine chemistry. In April, bromine chemistry can cause a net ozone loss (monthly mean) of 10-20 ppbv, with almost half attributable to open-ocean-sourced bromine and the rest to sea-ice-sourced bromine. However, the open-ocean-sourced bromine, via sea spray bromide depletion, cannot by itself produce ozone depletion events (ODEs) (defined as ozone volume mixing ratios VMRs < 10 ppbv). In contrast, sea-ice-sourced bromine, via sea salt aerosol (SSA) production from blowing snow, can produce ODEs even without bromine from sea spray, highlighting the importance of sea ice surface in polar boundary layer chemistry.</p><p>Modelled total inorganic bromine (Br<sub>Y</sub>) over the Arctic sea ice  is sensitive to model configuration, e.g., under the same bromine loading, Br<sub>Y</sub> in the Arctic spring boundary layer in the p-TOMCAT control run (i.e., with all bromine emissions) can be 2 times that in the UKCA control run. Despite the model differences, both model control runs can successfully reproduce large bromine explosion events (BEEs) and ODEs in polar spring. Model-integrated tropospheric column BrO generally matches GOME-2 tropospheric columns within ~50% in UKCA and a factor of 2 in p-TOMCAT. The success of the models in reproducing both ODEs and BEEs in the Arctic indicates that the relevant parameterizations implemented in the models work reasonably well, which supports the proposed mechanism of SSA production and bromide release on sea ice. Given that sea ice is a large source of SSA and halogens, changes in sea ice type and extent in a warming climate will influence Arctic boundary layer chemistry, including the oxidation of atmospheric elemental mercury. Note that this work dose not necessary rule out other possibilities that may act as a source of reactive bromine from sea ice zone.</p>

The Impact of Mixed-Phase Microphysical Processes on the Turbulence in Low-level Clouds in the Arctic

2021 ◽  
Author(s):  
Jan Chylik ◽  
Roel Neggers
Keyword(s):  
Boundary Layer ◽  
Climate Models ◽  
Weather Forecast ◽  
Mixed Phase ◽  
The Arctic ◽  
Contributing Factors ◽  
Microphysics Scheme ◽  
Low Level ◽  
Microphysical Processes ◽  
The Impact

<p>The proper representation of Arctic mixed-phased clouds remains a challenge in both weather forecast and climate models. Amongst the contributing factors is the complexity of turbulent properties of clouds. While the effect of evaporating hydrometeors on turbulent properties of the boundary layer has been identified in other latitudes, the extent of similar studies in the Arctic has been so far limited.</p><p>Our study focus on the impact of heat release from mixed-phase microphysical processes on the turbulent properties of the convective low-level clouds in the Arctic. We  employ high-resolution simulations, properly constrained by relevant measurements.<br>Semi-idealised model cases are based on convective clouds observed during the recent campaign in the Arctic: ACLOUD, which took place May--June 2017 over Fram Strait. The simulations are performed in Dutch Atmospheric Large Eddy Simulation (DALES) with double-moment mixed-phase microphysics scheme of Seifert & Beheng.</p><p>The results indicate an enhancement of boundary layer turbulence is some convective regimes.<br>Furthermore, results are sensitive to aerosols concentrations. Additional implications for the role of mixed-phase clouds in the Arctic Amplification will be discussed.</p>

scholarly journals Aircraft observations of enhancement and depletion of black carbon mass in the springtime Arctic

2010 ◽  
Vol 10 (6) ◽  
pp. 15167-15196
Author(s):  
J. R. Spackman ◽  
R. S. Gao ◽  
W. D. Neff ◽  
J. P. Schwarz ◽  
L. A. Watts ◽  
...  
Keyword(s):  
Boundary Layer ◽  
Black Carbon ◽  
Biomass Burning ◽  
Boundary Layer Transition ◽  
Arctic Climate ◽  
The Arctic ◽  
Vertical Profiles ◽  
Free Troposphere ◽  
Air Mass ◽  
The Impact

Abstract. Understanding the processes controlling black carbon (BC) in the Arctic is crucial for evaluating the impact of anthropogenic and natural sources of BC on Arctic climate. Vertical profiles of BC mass were observed from the surface to near 7-km altitude in April 2008 using a Single-Particle Soot Photometer (SP2) during flights on the NOAA WP-3D research aircraft from Fairbanks, Alaska. These measurements were conducted during the NOAA-sponsored Aerosol, Radiation, and Cloud Processes affecting Arctic Climate (ARCPAC) project as part of POLARCAT, an International Polar Year (IPY) activity. In the free troposphere, the Arctic air mass was influenced by long-range transport from biomass-burning and anthropogenic source regions at lower latitudes especially during the latter part of the campaign. Maximum average BC mass loadings of 150 ng kg−1 were observed near 5.5-km altitude in the aged Arctic air mass. In biomass-burning plumes, BC was enhanced from near the top of the Arctic boundary layer (ABL) to 5.5 km compared to the aged Arctic air mass. At the bottom of some of the profiles, positive vertical gradients in BC were observed in the vicinity of open leads in the sea-ice. BC mass loadings increased by about a factor of two across the boundary layer transition in the ABL in these cases while carbon monoxide (CO) remained constant, evidence for depletion of BC in the ABL. BC mass loadings were positively correlated with O3 in ozone depletion events (ODEs) for all the observations in the ABL suggesting that BC was removed by dry deposition of BC on the snow or ice because molecular bromine, Br2, which photolyzes and catalytically destroys O3, is thought to be released near the open leads in regions of ice formation. We estimate the deposition flux of BC mass to the snow using a box model constrained by the vertical profiles of BC in the ABL. The open leads may increase vertical mixing in the ABL and entrainment of pollution from the free troposphere possibly enhancing the deposition of BC to the snow.

Measurements of bromine monoxide over four halogen activation seasons in the Canadian high Arctic

2020 ◽  
Author(s):  
Kristof Bognar ◽  
Xiaoyi Zhao ◽  
Kimberly Strong ◽  
Rachel Y.-W. Chang ◽  
Udo Frieß ◽  
...  
Keyword(s):  
Boundary Layer ◽  
Sea Ice ◽  
Vertical Mixing ◽  
Temperature Inversion ◽  
The Arctic ◽  
Optical Absorption Spectroscopy ◽  
Blowing Snow ◽  
Atmospheric Conditions ◽  
Coarse Mode ◽  
Arctic Haze

<p><span>Bromine explosions and corresponding ozone depletion events (ODEs) are common in the Arctic spring. The snowpack on sea ice and sea salt aerosols (SSA) are both thought to release bromine, but the relative contribution of each source is not yet known. Furthermore, the role of atmospheric conditions is not fully understood. Long-term measurements of bromine monoxide (BrO) provide useful insight into the underlying processes of bromine activation. Here we present a four-year dataset (2016-2019) of springtime BrO partial columns retrieved from Multi-AXis Differential Optical Absorption Spectroscopy (MAX-DOAS) measurements in Eureka, Canada (80.1° N, 86.4° W). Due to the altitude of the measurement site (610 m), the measurements often represent BrO above the shallow boundary layer, and the strength of the temperature inversion has limited impact on the BrO partial columns. When the boundary layer is deep, however, the effects of the enhanced vertical mixing manifest as an increase in the minimum BrO values (and reduced ODE frequency) for wind speeds of ~8 m/s or greater. We find that BrO events show two modes differentiated by local wind direction and air mass history. Longer time spent in first-year sea ice areas corresponds to increased BrO for one of these modes only. We argue that snow on multi-year ice (salted and acidified by Arctic haze) might also contribute to bromine release. The MAX-DOAS measurements show that high aerosol optical depth is required to maintain lofted BrO. In situ measurements indicate that accumulation mode aerosols (mostly Arctic haze) have no direct correlation with BrO. The presence of coarse mode aerosols, however, is a necessary and sufficient condition for observing enhanced BrO at Eureka. The measurements of coarse mode aerosols are consistent with SSA generated from blowing snow. The good correlation between BrO and coarse mode aerosols (R<sup>2</sup> up to 0.57) supports the view that SSA is a direct source of bromine to the polar troposphere.</span></p>

Impact of Aerosol Intrusions on Arctic Boundary Layer Clouds. Part I: 4 May 1998 Case

2005 ◽  
Vol 62 (9) ◽  
pp. 3082-3093 ◽  
Author(s):  
G. G. Carrió ◽  
H. Jiang ◽  
W. R. Cotton
Keyword(s):  
Boundary Layer ◽  
Sea Ice ◽  
National Laboratory ◽  
Atmospheric Modeling ◽  
Mixed Phase ◽  
Radiative Properties ◽  
Arctic Boundary Layer ◽  
Water Fraction ◽  
Boundary Layer Clouds ◽  
The Impact

Abstract The objective of this paper is to assess the impact of the entrainment of aerosol from above the inversion on the microphysical structure and radiative properties of boundary layer clouds. For that purpose, the Los Alamos National Laboratory sea ice model was implemented into the research and real-time versions of the Regional Atmospheric Modeling System at Colorado State University. A series of cloud-resolving simulations have been performed for a mixed-phase Arctic boundary layer cloud using a new microphysical module that considers the explicit nucleation of cloud droplets. Different aerosol profiles based on observations were used for initialization. When more polluted initial ice-forming nuclei (IFN) profiles are assumed, the liquid water fraction of the cloud decreases while the total condensate path, the residence time of the ice particles, and the downwelling infrared radiation monotonically increase. Results suggest that increasing the aerosol concentrations above the boundary layer may increase sea ice melting rates when mixed-phase clouds are present.

scholarly journals Lidar characterization of the Arctic atmosphere during ASTAR 2007: four cases studies of boundary layer, mixed-phase and multi-layer clouds

2010 ◽  
Vol 10 (6) ◽  
pp. 2847-2866 ◽  
Author(s):  
A. Lampert ◽  
C. Ritter ◽  
A. Hoffmann ◽  
J.-F. Gayet ◽  
G. Mioche ◽  
...  
Keyword(s):  
Boundary Layer ◽  
Case Studies ◽  
Airborne Lidar ◽  
Mixed Phase ◽  
Spherical Particles ◽  
The Arctic ◽  
Free Troposphere ◽  
Atmospheric Conditions ◽  
Raman Lidar ◽  
Tropospheric Aerosol

Abstract. During the Arctic Study of Tropospheric Aerosol, Clouds and Radiation (ASTAR), which was conducted in Svalbard in March and April 2007, tropospheric Arctic clouds were observed with two ground-based backscatter lidar systems (micro pulse lidar and Raman lidar) and with an airborne elastic lidar. In the time period of the ASTAR 2007 campaign, an increase in low-level cloud cover (cloud tops below 2.5 km) from 51% to 65% was observed above Ny-Ålesund. Four different case studies of lidar cloud observations are analyzed: With the ground-based Raman lidar, a layer of spherical particles was observed at an altitude of 2 km after the dissolution of a cloud. The layer probably consisted of small hydrated aerosol (radius of 280 nm) with a high number concentration (around 300 cm−3) at low temperatures (−30 °C). Observations of a boundary layer mixed-phase cloud by airborne lidar and concurrent airborne in situ and spectral solar radiation sensors revealed the localized process of total glaciation at the boundary of different air masses. In the free troposphere, a cloud composed of various ice layers with very different optical properties was detected by the Raman lidar, suggesting large differences of ice crystal size, shape and habit. Further, a mixed-phase double layer cloud was observed by airborne lidar in the free troposphere. Local orography influenced the evolution of this cloud. The four case studies revealed relations of cloud properties and specific atmospheric conditions, which we plan to use as the base for numerical simulations of these clouds.

scholarly journals Radiative energy budget and cloud radiative forcing in the daytime marginal sea ice zone during Arctic spring and summer

2021 ◽  
Author(s):  
Johannes Stapf ◽  
André Ehrlich ◽  
Christof Lüpkes ◽  
Manfred Wendisch
Keyword(s):  
Boundary Layer ◽  
Sea Ice ◽  
Energy Budget ◽  
Radiative Forcing ◽  
The Arctic ◽  
Radiative Energy ◽  
Cloud Radiative Forcing ◽  
Airborne Measurements ◽  
Marginal Sea ◽  
The Impact

Abstract. Airborne measurements of the surface radiative energy budget (REB) collected in the area of the marginal sea ice zone (MIZ) close to Svalbard (Norway) during two campaigns conducted in early spring and and early summer are presented. From the data, the cloud radiative forcing was derived. The analysis is focussed on the impact of changing atmospheric thermodynamic conditions on the REB and on the linkage of sea ice properties and cloud radiative forcing (CRF). The observed two-mode longwave net irradiance frequency distributions above sea ice are compared with measurements from previous studies. The transition of both states (cloudy and cloud-free) from winter towards summer and the associated broadening of the modes is discussed as a function of the seasonal thermodynamic profiles and the surface type. The influence of cold air outbreaks (CAO) and warm air intrusions on the REB is illustrated for several case studies, whereby the source and sink terms of REB in the evolving CAO boundary layer are quantified. Furthermore, the role of thermodynamic profiles and the vertical location of clouds during on-ice flow is illustrated. The sea ice concentration was identified as the main driver of the shortwave cooling by the clouds. The longwave warming of clouds, estimated to about 75 W m−2, seems to be representative for this region, as compared to other studies. Simplified radiative transfer simulations of the frequently observed low-level boundary layer clouds and average thermodynamic profiles represent the observed radiative quantities fairly well. The simulations illustrate the delicate interplay of surface and cloud properties that modify the REB and CRF, and the challenges in quantifying trends in the Arctic REB induced by potential changes of the cloud optical thickness.

scholarly journals The NO<sub><i>x</i></sub> dependence of bromine chemistry in the Arctic atmospheric boundary layer

2015 ◽  
Vol 15 (18) ◽  
pp. 10799-10809 ◽  
Author(s):  
K. D. Custard ◽  
C. R. Thompson ◽  
K. A. Pratt ◽  
P B. Shepson ◽  
J. Liao ◽  
...  
Keyword(s):  
Climate Change ◽  
Boundary Layer ◽  
Nitrogen Oxides ◽  
Sea Ice ◽  
Gas Phase ◽  
Atmospheric Chemistry ◽  
The Arctic ◽  
Arctic Boundary Layer ◽  
Large Variability ◽  
The Impact

Abstract. Arctic boundary layer nitrogen oxides (NOx = NO2 + NO) are naturally produced in and released from the sunlit snowpack and range between 10 to 100 pptv in the remote background surface layer air. These nitrogen oxides have significant effects on the partitioning and cycling of reactive radicals such as halogens and HOx (OH + HO2). However, little is known about the impacts of local anthropogenic NOx emission sources on gas-phase halogen chemistry in the Arctic, and this is important because these emissions can induce large variability in ambient NOx and thus local chemistry. In this study, a zero-dimensional photochemical kinetics model was used to investigate the influence of NOx on the unique springtime halogen and HOx chemistry in the Arctic. Trace gas measurements obtained during the 2009 OASIS (Ocean – Atmosphere – Sea Ice – Snowpack) field campaign at Barrow, AK were used to constrain many model inputs. We find that elevated NOx significantly impedes gas-phase halogen radical-based depletion of ozone, through the production of a variety of reservoir species, including HNO3, HO2NO2, peroxyacetyl nitrate (PAN), BrNO2, ClNO2 and reductions in BrO and HOBr. The effective removal of BrO by anthropogenic NOx was directly observed from measurements conducted near Prudhoe Bay, AK during the 2012 Bromine, Ozone, and Mercury Experiment (BROMEX). Thus, while changes in snow-covered sea ice attributable to climate change may alter the availability of molecular halogens for ozone and Hg depletion, predicting the impact of climate change on polar atmospheric chemistry is complex and must take into account the simultaneous impact of changes in the distribution and intensity of anthropogenic combustion sources. This is especially true for the Arctic, where NOx emissions are expected to increase because of increasing oil and gas extraction and shipping activities.

scholarly journals Aircraft observations of enhancement and depletion of black carbon mass in the springtime Arctic

2010 ◽  
Vol 10 (19) ◽  
pp. 9667-9680 ◽  
Author(s):  
J. R. Spackman ◽  
R. S. Gao ◽  
W. D. Neff ◽  
J. P. Schwarz ◽  
L. A. Watts ◽  
...  
Keyword(s):  
Sea Ice ◽  
Black Carbon ◽  
Biomass Burning ◽  
Dry Deposition ◽  
Arctic Climate ◽  
The Arctic ◽  
Vertical Profiles ◽  
Free Troposphere ◽  
Air Mass ◽  
The Impact

Abstract. Understanding the processes controlling black carbon (BC) in the Arctic is crucial for evaluating the impact of anthropogenic and natural sources of BC on Arctic climate. Vertical profiles of BC mass loadings were observed from the surface to near 7-km altitude in April 2008 using a Single-Particle Soot Photometer (SP2) during flights on the NOAA WP-3D research aircraft from Fairbanks, Alaska. These measurements were conducted during the NOAA-sponsored Aerosol, Radiation, and Cloud Processes affecting Arctic Climate (ARCPAC) project. In the free troposphere, the Arctic air mass was influenced by long-range transport from biomass-burning and anthropogenic source regions at lower latitudes especially during the latter part of the campaign. Average BC mass mixing ratios peaked at about 150 ng BC (kg dry air )−1 near 5.5 km altitude in the aged Arctic air mass and 250 ng kg−1 at 4.5 km in biomass-burning influenced air. BC mass loadings were enhanced by up to a factor of 5 in biomass-burning influenced air compared to the aged Arctic air mass. At the bottom of some of the profiles, positive vertical gradients in BC were observed over the sea-ice. The vertical profiles generally occurred in the vicinity of open leads in the sea-ice. In the aged Arctic air mass, BC mass loadings more than doubled with increasing altitude within the ABL and across the boundary layer transition while carbon monoxide (CO) remained constant. This is evidence for depletion of BC mass in the ABL. BC mass loadings were positively correlated with O3 in ozone depletion events (ODEs) for all the observations in the ABL. Since bromine catalytically destroys ozone in the ABL after being released as molecular bromine in regions of new sea-ice formation at the surface, the BC–O3 correlation suggests that BC particles were removed by a surface process such as dry deposition. We develop a box model to estimate the dry deposition flux of BC mass to the snow constrained by the vertical profiles of BC mass in the ABL. Open leads in the sea-ice may increase vertical mixing and entrainment of pollution from the free troposphere possibly enhancing the deposition of BC aerosol to the snow.

scholarly journals The NO<sub>x</sub> dependence of bromine chemistry in the Arctic atmospheric boundary layer

2015 ◽  
Vol 15 (6) ◽  
pp. 8329-8360 ◽  
Author(s):  
K. D. Custard ◽  
C. R. Thompson ◽  
K. A. Pratt ◽  
P. B. Shepson ◽  
J. Liao ◽  
...  
Keyword(s):  
Climate Change ◽  
Boundary Layer ◽  
Nitrogen Oxides ◽  
Sea Ice ◽  
Gas Phase ◽  
Atmospheric Chemistry ◽  
The Arctic ◽  
Arctic Boundary Layer ◽  
Large Variability ◽  
The Impact

Abstract. Arctic boundary layer nitrogen oxides (NOx = NO2 + NO) are naturally produced in and released from the sunlit snowpack and range between 10 to 100 pptv in the remote background surface layer air. These nitrogen oxides have significant effects on the partitioning and cycling of reactive radicals such as halogens and HOx (OH + HO2). However, little is known about the impacts of local anthropogenic NOx emission sources on gas-phase halogen chemistry in the Arctic, and this is important because these emissions can induce large variability in ambient NOx and thus local chemistry. In this study, a zero-dimensional photochemical kinetics model was used to investigate the influence of NOx on the unique springtime halogen and HOx chemistry in the Arctic. Trace gas measurements obtained during the 2009 OASIS (Ocean–Atmosphere–Sea Ice–Snowpack) field campaign at Barrow, AK were used to constrain many model inputs. We find that elevated NOx significantly impedes gas-phase radical chemistry, through the production of a variety of reservoir species, including HNO3, HO2NO2, peroxyacetyl nitrate (PAN), BrNO2, ClNO2 and reductions in BrO and HOBr, with a concomitant, decreased net O3 loss rate. The effective removal of BrO by anthropogenic NOx was directly observed from measurements conducted near Prudhoe Bay, AK during the 2012 Bromine, Ozone, and Mercury Experiment (BROMEX). Thus, while changes in snow-covered sea ice attributable to climate change may alter the availability of molecular halogens for ozone and Hg depletion, predicting the impact of climate change on polar atmospheric chemistry is complex and must take into account the simultaneous impact of changes in the distribution and intensity of anthropogenic combustion sources. This is especially true for the Arctic, where NOx emissions are expected to increase because of increasing oil and gas extraction and shipping activities.

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