scholarly journals Reconstruction and Simulation of Stratospheric Ozone Distributions during the 2002 Austral Winter

2005 ◽  
Vol 62 (3) ◽  
pp. 748-764 ◽  
Author(s):  
C. E. Randall ◽  
G. L. Manney ◽  
D. R. Allen ◽  
R. M. Bevilacqua ◽  
J. Hornstein ◽  
...  

Abstract Satellite-based solar occultation measurements during the 2002 austral winter have been used to reconstruct global, three-dimensional ozone distributions. The reconstruction method uses correlations between potential vorticity and ozone to derive “proxy” distributions from the geographically limited occultation observations. Ozone profiles from the Halogen Occultation Experiment (HALOE), the Polar Ozone and Aerosol Measurement III (POAM III), and the Stratospheric Aerosol and Gas Experiment II and III (SAGE II and III) are incorporated into the analysis. Because this is one of the first uses of SAGE III data in a scientific analysis, preliminary validation results are shown. The reconstruction method is described, with particular emphasis on uncertainties caused by noisy and/or multivalued correlations. The evolution of the solar occultation data and proxy ozone fields throughout the winter is described, and differences with respect to previous winters are characterized. The results support the idea that dynamical forcing early in the 2002 winter influenced the morphology of the stratosphere in a significant and unusual manner, possibly setting the stage for the unprecedented major stratospheric warming in late September. The proxy is compared with ozone from mechanistic, primitive equation model simulations of passive ozone tracer fields during the time of the warming. In regions where chemistry is negligible compared to transport, the model and proxy ozone fields agree well. The agreement between, and changes in, the large-scale ozone fields in the model and proxy indicate that transport processes, particularly enhanced poleward transport and mixing, are the primary cause of ozone changes through most of the stratosphere during this unprecedented event. The analysis culminates with the calculation of globally distributed column ozone during the major warming, showing quantitatively how transport of low-latitude air to the polar region in the middle stratosphere led to the diminished ozone hole in 2002.

2011 ◽  
Vol 11 (1) ◽  
pp. 363-373 ◽  
Author(s):  
H. Bencherif ◽  
L. El Amraoui ◽  
G. Kirgis ◽  
J. Leclair De Bellevue ◽  
A. Hauchecorne ◽  
...  

Abstract. This paper reports on an increase of ozone event observed over Kerguelen (49.4° S, 70.3° E) in relationship with large-scale isentropic transport. This is evidenced by ground-based observations (co-localised radiosonde and SAOZ experiments) together with satellite global observations (Aura/MLS) assimilated into MOCAGE, a Méteo-France model. The study is based on the analyses of the first ozonesonde experiment never recorded at the Kerguelen site within the framework of a French campaign called ROCK that took place from April to August 2008. Comparisons and interpretations of the observed event are supported by co-localised SAOZ observations, by global mapping of tracers (O3, N2O and columns of O3) from Aura/MLS and Aura/OMI experiments, and by model simulations of Ertel Potential Vorticity initialised by the ECMWF (European Centre for Medium-Range Weather Forecasts) data reanalyses. Satellite and ground-based observational data revealed a consistent increase of ozone in the local stratosphere by mid-April 2008. Additionally, Ozone (O3) and nitrous oxide (N2O) profiles obtained during January–May 2008 using the Microwave Limb Sounder (MLS) aboard the Aura satellite are assimilated into MOCAGE (MOdèle de Chimie Atmosphérique à Grande Echelle), a global three-dimensional chemistry transport model of Météo-France. The assimilated total O3 values are consistent with SAOZ ground observations (within ±5%), and isentropic distributions of O3 match well with maps of advected potential vorticity (APV) derived from the MIMOSA model, a high-resolution advection transport model, and from the ECMWF reanalysis. The event studied seems to be related to the isentropic transport of air masses that took place simultaneously in the lower- and middle-stratosphere, respectively from the polar region and from the tropics to the mid-latitudes. In fact, the ozone increase observed by mid April 2008 resulted simultaneously: (1) from an equator-ward departure of polar air masses characterised with a high-ozone layer in the lower stratosphere (near the 475 K isentropic level), and (2) from a reverse isentropic transport from the tropics to mid- and high-latitudes in the upper stratosphere (nearby the 700 K level). The increase of ozone observed over Kerguelen from the 16-April ozonesonde profile is thus attributed to a concomitant isentropic transport of ozone in two stratospheric layers: the tropical air moving southward and reaching over Kerguelen in the upper stratosphere, and the polar air passing over the same area but in the lower stratosphere.


2016 ◽  
Author(s):  
Klemens Hocke ◽  
Franziska Schranz ◽  
Eliane Maillard Barras ◽  
Lorena Moreira ◽  
Niklaus Kämpfer

Abstract. Observation and simulation of individual ozone streamers are important for the description and understanding of nonlinear transport processes in the middle atmosphere. A sudden increase in mid-stratospheric ozone occurred above Central Europe on December 4, 2015. The GROunbased Millimeter-wave Ozone Spectrometer (GROMOS) and the Stratospheric Ozone MOnitoring RAdiometer (SOMORA) in Switzerland measured an ozone enhancement of about 30 % at 34 km altitude from December 1 to December 4. A similar ozone increase is simulated by the Specified Dynamics-Whole Atmosphere Community Climate (SD-WACCM) model. Further, the global ozone fields at 34 km altitude from SD-WACCM and the satellite experiment Aura/MLS show a remarkable agreement for the location and the timing of an ozone streamer (large-scale tongue like structure) extending from the subtropics in Northern America over the Atlantic to Central Europe. This agreement indicates that SD-WACCM can inform us about the wind inside the Atlantic ozone streamer. SD-WACCM shows an eastward wind of about 100 m/s inside the Atlantic streamer in the mid-stratosphere. SD-WACCM shows that the Atlantic streamer flows along the edge region of the polar vortex. The Atlantic streamer turns southward at an erosion region of the polar vortex located above the Caspian Sea. The spatial distribution of stratospheric water vapour indicates a filament outgoing from this erosion region. The Atlantic streamer, the polar vortex erosion region and the water vapour filament belong to the process of planetary wave breaking in the so-called surf zone of the Northern mid-latitude winter stratosphere.


1993 ◽  
Vol 28 (1) ◽  
pp. 77-86 ◽  
Author(s):  
R. C. Frost ◽  
J. Halliday ◽  
A. S. Dee

Improved design and performance of continuous thickeners should be achieved through a better understanding of the sludge transport processes involved and the variability of sludge thickenability. A software package called PHOENICS was used to model the three-dimensional flow of sludge in the transport zone of a 20m diameter thickener. A mass transport efficiency was evaluated to test the efficacy of the ploughing system, and tracer simulations were performed to study the degree of back-mixing induced. Interpretation of the results suggests that:○Optimum orientation of the ploughs to the radial arm is 60° to 70°.○Transport of sludge to a central outlet occurs principally in the wake of the advancing ploughs, and that ploughs are less efficient than conventional theories dictate.○Sludge in the ploughing zone is mixed, thus potentially impairing thickener performance. The thickenability of mixed raw sludge arising at a large activated sludge works was monitored. Pronounced seasonal variations were observed, with a marked deterioration in thickenability in late summer and autumn. These were confirmed in trials of a 20m diameter continuous thickener. Consequently the proposed thickening strategy for this works has been revised.


Author(s):  
John A. Dykema ◽  
David W. Keith ◽  
James G. Anderson ◽  
Debra Weisenstein

Although solar radiation management (SRM) through stratospheric aerosol methods has the potential to mitigate impacts of climate change, our current knowledge of stratospheric processes suggests that these methods may entail significant risks. In addition to the risks associated with current knowledge, the possibility of ‘unknown unknowns’ exists that could significantly alter the risk assessment relative to our current understanding. While laboratory experimentation can improve the current state of knowledge and atmospheric models can assess large-scale climate response, they cannot capture possible unknown chemistry or represent the full range of interactive atmospheric chemical physics. Small-scale, in situ experimentation under well-regulated circumstances can begin to remove some of these uncertainties. This experiment—provisionally titled the stratospheric controlled perturbation experiment—is under development and will only proceed with transparent and predominantly governmental funding and independent risk assessment. We describe the scientific and technical foundation for performing, under external oversight, small-scale experiments to quantify the risks posed by SRM to activation of halogen species and subsequent erosion of stratospheric ozone. The paper's scope includes selection of the measurement platform, relevant aspects of stratospheric meteorology, operational considerations and instrument design and engineering.


2010 ◽  
Vol 10 (7) ◽  
pp. 17727-17751
Author(s):  
H. Bencherif ◽  
L. El Amraoui ◽  
G. Kirgis ◽  
J. Leclair De Bellevue ◽  
A. Hauchecorne ◽  
...  

Abstract. This paper reports on an increase of ozone event observed over Kerguelen (49.4° S, 70.3° E) in relationship with large-scale isentropic transport. It is evidenced from ground-based observations, together with satellite global observations and assimilated fields. The study is based on the analyses of the first ozonesonde experiment never recorded at the Kerguelen site in the framework of a French campaign called ROCK that took place from April to August 2008. Comparisons and interpretations of the observed event are supported by co-localised SAOZ observations, by global mapping of tracers (O3, N2O and columns of O3) from Aura/MLS and Aura/OMI experiments, and by model simulations of Ertel Potential Vorticity initialised by ECMWF (European Centre for Medium-Range Weather Forecasts) data reanalyses. Satellite and ground-based observational data revealed a consistent increase of ozone in the local stratosphere by mid-April 2008. Additionally, Ozone (O3) and nitrous oxide (N2O) profiles obtained during January–May 2008 by the Microwave Lamb Sounder (MLS) aboard the Aura satellite are assimilated into MOCAGE (MOdèle de Chimie Atmosphérique à Grande Echelle), a global three-dimensional chemistry transport model of Météo-France. The assimilated total O3 values are consistent with SAOZ ground observations (within ±5%), and isentropic distributions of O3 are matching well with maps of advected potential vorticity (APV) derived from the MIMOSA model, a high-resolution advection transport model, and from ECMWF reanalysis. The studied event seems to be related to isentropic transport of air masses that took place simultaneously in the lower- and middle-stratosphere, respectively from the polar region and from tropics to the mid-latitudes. In fact, the studied ozone increase by mid April 2008 results simultaneously: (1) from an equator-ward departure of polar air masses characterised with a high-ozone layer in the lower stratosphere (nearby the 475 K isentropic level), and (2) from a reverse isentropic transport from tropics to mid- and high-latitudes in the upper stratosphere (nearby the 700 K level). The increase of ozone observed over Kerguelen from the 16-April ozonesonde profile is then attributed to a concomitant isentropic transport of ozone in two stratospheric layers: the tropical air moving southward and reaches over Kerguelen in the upper stratosphere, and the polar air passing over the same area but in the lower stratosphere.


2010 ◽  
Vol 10 (7) ◽  
pp. 17307-17340
Author(s):  
E. Remsberg ◽  
G. Lingenfelser

Abstract. Stratospheric Aerosol and Gas Experiment (SAGE II) Version 6.2 ozone profiles are analyzed for their decadal-scale responses in the middle and upper stratosphere from September 1991 to August 2005, a time span for which the trends in reactive chlorine are relatively small. The profile data are averaged within twelve, 20°-wide latitude bins from 55° S to 55° N and at eleven altitudes from 27.5 to 52.5 km. The separate, 14-yr data time series are analyzed using multiple linear regression (MLR) models that include seasonal, interannual, 11-yr sinusoid, and linear trend terms. Proxies are not used for the interannual, solar uv-flux, or reactive chlorine terms. Instead, the present analysis focuses on the periodic 11-yr terms to see whether they are in-phase with that of a direct, uv-flux forcing or are dominated by some other decadal-scale influence. It is shown that they are in-phase over most of the latitude/altitude domain and that they have max minus min variations between 25° S and 25° N that peak near 4% between 30 and 40 km. Model simulations of the direct effects of uv-flux forcings agree with this finding. Ozone in the middle stratosphere of the northern subtropics is perturbed during 1991–1992, following the eruption of Pinatubo. There are also pronounced decadal-scale variations in the ozone of the upper stratosphere for the middle latitudes of the Northern Hemisphere, presumably due to dynamical forcings. The 11-yr ozone responses of the Southern Hemisphere are relatively free of those extra influences. The associated linear trend terms from the analyses are negative (−2 to −4%/decade) for this 14-yr time period and are nearly constant across latitude in the upper stratosphere. This finding is consistent with the fact that total and reactive chlorine are not changing appreciably from 1991 to 2005. It is concluded that the satellite, solar occultation technique can be used to record the responses of stratospheric ozone to the decadal-scale forcings from the solar uv-flux, as well as those due to the long-term changes from dynamic forcings, reactive chlorine, and the greenhouse gases.


2017 ◽  
Vol 17 (5) ◽  
pp. 3445-3452 ◽  
Author(s):  
Klemens Hocke ◽  
Franziska Schranz ◽  
Eliane Maillard Barras ◽  
Lorena Moreira ◽  
Niklaus Kämpfer

Abstract. Observation and simulation of individual ozone streamers are important for the description and understanding of non-linear transport processes in the middle atmosphere. A sudden increase in mid-stratospheric ozone occurred above central Europe on 4 December 2015. The GROund-based Millimeter-wave Ozone Spectrometer (GROMOS) and the Stratospheric Ozone MOnitoring RAdiometer (SOMORA) in Switzerland measured an ozone enhancement of about 30 % at 34 km altitude (8.3 hPa) from 1 to 4 December. A similar ozone increase is simulated by the Specified Dynamics Whole Atmosphere Community Climate (SD-WACCM) model. Further, the global ozone fields at 34 km altitude (8.3 hPa) from SD-WACCM and the satellite experiment Aura/MLS show a remarkable agreement for the location and timing of an ozone streamer (large-scale tongue-like structure) extending from the subtropics in northern America over the Atlantic to central Europe. This agreement indicates that SD-WACCM can inform us about the wind inside the Atlantic ozone streamer. SD-WACCM shows an eastward wind of about 100 m s−1 inside the Atlantic streamer in the mid-stratosphere. SD-WACCM shows that the Atlantic streamer flows along the edge of the polar vortex. The Atlantic streamer turns southward at an erosion region of the polar vortex located above the Caspian Sea. The spatial distribution of stratospheric water vapour indicates a filament outgoing from this erosion region. The Atlantic streamer, the polar vortex erosion region and the water vapour filament belong to the process of planetary wave breaking in the so-called surf zone of the northern midlatitude winter stratosphere.


2010 ◽  
Vol 10 (1) ◽  
pp. 1-8 ◽  
Author(s):  
S. P. Burton ◽  
L. W. Thomason ◽  
J. M. Zawodny

Abstract. Solar occultation has proven to be a reliable technique for the measurement of atmospheric constituents in the stratosphere. NASA's Stratospheric Aerosol and Gas Experiments (SAGE, SAGE II, and SAGE III) together have provided over 25 years of quality solar occultation data, a data record which has been an important resource for the scientific exploration of atmospheric composition and climate change. Herein, we describe an improvement to the processing of SAGE data that corrects for a previously uncorrected short-term time-dependence in the calibration function. The variability relates to the apparent rotation of the scanning track with respect to the face of the sun due to the motion of the satellite. Correcting for this effect results in a decrease in the measurement noise in the Level 1 line-of-sight optical depth measurements of approximately 40% in the middle and upper stratospheric SAGE II and III observations where it has been applied. The technique is potentially useful for any scanning solar occultation instrument and suggests further improvement for future occultation measurements if a full disk imaging system can be included.


2009 ◽  
Vol 9 (5) ◽  
pp. 20259-20282 ◽  
Author(s):  
S. P. Burton ◽  
L. W. Thomason ◽  
J. M. Zawodny

Abstract. Solar occultation has proven to be a reliable technique for the measurement of atmospheric constituents in the stratosphere. NASA's Stratospheric Aerosol and Gas Experiments (SAGE, SAGE II, and SAGE III) together have provided over 25 years of quality solar occultation data, a data record which has been an important resource for the scientific exploration of atmospheric composition and climate change. Herein, we describe an improvement to the processing of SAGE data that corrects for a previously uncorrected short-term time-dependence in the calibration function. The variability relates to the apparent rotation of the scanning track with respect to the face of the sun due to the motion of the satellite. Correcting for this effect results in a decrease in the measurement noise in the Level 1 line-of-sight optical depth measurements of approximately 40% in the middle and upper stratospheric SAGE II and III observations where it has been applied. The technique is potentially useful for any scanning solar occultation instrument, and suggests further improvement for future occultation measurements if a full disk imaging system can be included.


2014 ◽  
Vol 2014 ◽  
pp. 1-10
Author(s):  
Bo Dong ◽  
Feng Xu ◽  
Xiao-fang Hu ◽  
Hong-yan Qu ◽  
Dan Kang ◽  
...  

To investigate the local micro-/nanoscale region in a large scale sample, an image reconstruction method for nanometer computed tomography (nano-CT) was proposed in this paper. In the algorithm, wavelets were used to localize the filtered-backprojection (FBP) algorithm because of its space-frequency localization property. After the implementation of the algorithm, two simulation local reconstruction experiments were performed to confirm its effectiveness. Three evaluation criteria were used in the experiments to judge the quality of the reconstructed images. The experimental results showed that the algorithm proposed in this paper performed best because (1) the quality of its results had improved 20%–30% compared to the results of FBP and 10%–30% compared to the results of another wavelet algorithm; (2) the new algorithm was stable under different circumstances. Besides, an actual reconstruction experiment was performed using real projection data that had been collected in a CT experiment. Two-dimensional (2D) and three-dimensional (3D) images of the sample were reconstructed. The microstructure of the sample could be clearly observed in the reconstructed images. Since much attention has been directed towards the nano-CT technique to investigate the microstructure of materials, this new wavelet-based local tomography algorithm could be considered as a meaningful effort.


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