scholarly journals Aerosol–Cloud Interactions in a Mesoscale Model. Part II: Sensitivity to Aqueous-Phase Chemistry

2008 ◽  
Vol 65 (2) ◽  
pp. 309-330 ◽  
Author(s):  
Irena T. Ivanova ◽  
Henry G. Leighton
Keyword(s):  
Aqueous Phase ◽  
Mesoscale Model ◽  
Cloud Condensation Nuclei ◽  
Cloud Microphysics ◽  
Size Spectrum ◽  
Chemical Processing ◽  
Strong Constraint ◽  
Cloud Processing ◽  
Sulfate Production ◽  
The Impact

Abstract The feedbacks between aerosols, cloud microphysics, and cloud chemistry are investigated in a mesoscale model. A simple bulk aqueous-phase sulfur chemistry scheme was fully coupled to the existing aerosol and microphysics schemes. The representation of aerosol and microphysics follows the explicit bulk double-moment approach. A case of summertime stratocumulus cloud system is simulated at high resolution (3-km grid spacing), and the evolution of an observed continental aerosol spectrum that changes during the course of the simulation as a result of cloud processing is examined. The results demonstrate that the bulk approach to the aerosol and droplet spectra correctly represents the feedbacks in the coupled system. The simulations capture the characteristic bimodal aerosol size spectrum resulting from cloud processing, with the first mode consisting of particles that did not participate as cloud condensation nuclei and the second mode, in the region of 0.08–0.12-μm radii, comprising the particles that were affected by processing. New information is revealed about the impact of the two main processing pathways and about the spatial distribution of the processed aerosol. One cycle of physical processing produced a relatively modest impact of 3%–5% on the processed particle mean radius of the order that was comparable to the impact of chemical processing, while continuous physical recycling produced a much larger impact as high as 30%–50%. A strong constraint on the chemical processing was found to be the initial chemistry input and the assumption of bulk chemical composition. Simple tests with a more slowly depleting primary oxidant (H2O2) and including the droplet chemical heterogeneity effect favor stronger sulfate production, by, respectively, the H2O2 and O3 oxidation reaction, and both show a larger impact on the processed particle mean radius of similar magnitude, 10%–20%. Spatially, the impact of processing is found initially in the downdraft regions below cloud and at later times at substantial distances downwind. It is shown that cloud processing can either enhance or suppress the number of activated drops in subsequent cycles.

scholarly journals Broadening of Cloud Droplet Spectra through Eddy Hopping: Turbulent Entraining Parcel Simulations

2018 ◽  
Vol 75 (10) ◽  
pp. 3365-3379 ◽  
Author(s):  
Gustavo C. Abade ◽  
Wojciech W. Grabowski ◽  
Hanna Pawlowska
Keyword(s):  
Droplet Size ◽  
Turbulent Mixing ◽  
Cloud Condensation Nuclei ◽  
Cloud Droplet ◽  
Cloud Microphysics ◽  
Droplet Growth ◽  
Size Spectrum ◽  
Entrainment Rate ◽  
The Mean ◽  
The Impact

This paper discusses the effects of cloud turbulence, turbulent entrainment, and entrained cloud condensation nuclei (CCN) activation on the evolution of the cloud droplet size spectrum. We simulate an ensemble of idealized turbulent cloud parcels that are subject to entrainment events modeled as a random process. Entrainment events, subsequent turbulent mixing inside the parcel, supersaturation fluctuations, and the resulting stochastic droplet activation and growth by condensation are simulated using a Monte Carlo scheme. Quantities characterizing the turbulence intensity, entrainment rate, CCN concentration, and the mean fraction of environmental air entrained in an event are all specified as independent external parameters. Cloud microphysics is described by applying Lagrangian particles, the so-called superdroplets. These are either unactivated CCN or cloud droplets that grow from activated CCN. The model accounts for the addition of environmental CCN into the cloud by entraining eddies at the cloud edge. Turbulent mixing of the entrained dry air with cloudy air is described using the classical linear relaxation to the mean model. We show that turbulence plays an important role in aiding entrained CCN to activate, and thus broadening the droplet size distribution. These findings are consistent with previous large-eddy simulations (LESs) that consider the impact of variable droplet growth histories on the droplet size spectra in small cumuli. The scheme developed in this work is ready to be used as a stochastic subgrid-scale scheme in LESs of natural clouds.

scholarly journals Inclusion of biomass burning in WRF-Chem: impact of wildfires on weather forecasts

2011 ◽  
Vol 11 (11) ◽  
pp. 5289-5303 ◽  
Author(s):  
G. Grell ◽  
S. R. Freitas ◽  
M. Stuefer ◽  
J. Fast
Keyword(s):  
Biomass Burning ◽  
Cloud Model ◽  
Cloud Condensation Nuclei ◽  
Cloud Microphysics ◽  
Fire Season ◽  
Strong Impact ◽  
Emission Rates ◽  
Weather Forecasts ◽  
High Concentrations ◽  
The Impact

Abstract. A plume rise algorithm for wildfires was included in WRF-Chem, and applied to look at the impact of intense wildfires during the 2004 Alaska wildfire season on weather simulations using model resolutions of 10 km and 2 km. Biomass burning emissions were estimated using a biomass burning emissions model. In addition, a 1-D, time-dependent cloud model was used online in WRF-Chem to estimate injection heights as well as the vertical distribution of the emission rates. It was shown that with the inclusion of the intense wildfires of the 2004 fire season in the model simulations, the interaction of the aerosols with the atmospheric radiation led to significant modifications of vertical profiles of temperature and moisture in cloud-free areas. On the other hand, when clouds were present, the high concentrations of fine aerosol (PM2.5) and the resulting large numbers of Cloud Condensation Nuclei (CCN) had a strong impact on clouds and cloud microphysics, with decreased precipitation coverage and precipitation amounts during the first 12 h of the integration. During the afternoon, storms were of convective nature and appeared significantly stronger, probably as a result of both the interaction of aerosols with radiation (through an increase in CAPE) as well as the interaction with cloud microphysics.

scholarly journals Indirect Impact of Atmospheric Aerosols in Idealized Simulations of Convective–Radiative Quasi Equilibrium. Part II: Double-Moment Microphysics

2011 ◽  
Vol 24 (7) ◽  
pp. 1897-1912 ◽  
Author(s):  
Wojciech W. Grabowski ◽  
Hugh Morrison
Keyword(s):  
Atmospheric Aerosols ◽  
Cloud Condensation Nuclei ◽  
Cloud Droplet ◽  
Bowen Ratio ◽  
Cloud Microphysics ◽  
Quasi Equilibrium ◽  
Double Moment ◽  
The Mean ◽  
The Difference ◽  
The Impact

Abstract This paper extends the previous cloud-resolving modeling study concerning the impact of cloud microphysics on convective–radiative quasi equilibrium (CRQE) over a surface with fixed characteristics and prescribed solar input, both mimicking the mean conditions on earth. The current study applies sophisticated double-moment warm-rain and ice microphysics schemes, which allow for a significantly more realistic representation of the impact of aerosols on precipitation processes and on the coupling between clouds and radiative transfer. Two contrasting cloud condensation nuclei (CCN) characteristics are assumed, representing pristine and polluted conditions, as well as contrasting representations of the effects of entrainment and mixing on the mean cloud droplet size. In addition, four sets of sensitivity simulations are also performed with changes that provide a reference for the main simulation set. As in the previous study, the CRQE mimics the estimates of globally and annually averaged water and energy fluxes across the earth’s atmosphere. There are some differences from the previous study, however, consistent with the slightly lower water vapor content in the troposphere and significantly reduced lower-tropospheric cloud fraction in current simulations. There is also a significant reduction of the difference between the pristine and polluted cases, from ∼20 to ∼4 W m−2 at the surface from ∼20 to ∼9 W m−2 at the top of the atmosphere (TOA). The difference between the homogeneous and extremely inhomogeneous mixing scenarios, ∼20 W m−2 in the previous study, is reduced to a mere 2 (1) W m−2 at the surface (TOA). An unexpected difference between the previous and current simulations is the lower Bowen ratio of the surface heat flux, the partitioning of the total flux into sensible and latent components. It is shown that most of the change comes from the difference in the representation of rain evaporation in the subcloud layer in the single- and double-moment microphysics schemes. The difference affects the mean air temperature and humidity near the surface, and thus the Bowen ratio. The differences between the various simulations are discussed, contrasting the process-level approach with the impact of cloud microphysics on the quasi-equilibrium state with a more appropriate system dynamics approach. The key distinction is that the latter includes the interactions among all the processes in the modeled system.

scholarly journals Aerosol activation and cloud processing in the global aerosol-climate model ECHAM5-HAM

2006 ◽  
Vol 6 (1) ◽  
pp. 519-548
Author(s):  
G. J. Roelofs ◽  
P. Stier ◽  
J. Feichter ◽  
E. Vignati ◽  
J. Wilson
Keyword(s):  
Climate Model ◽  
Cloud Condensation Nuclei ◽  
Cloud Base ◽  
Cloud Drop ◽  
Direct Role ◽  
Accumulation Mode ◽  
Cloud Processing ◽  
Sulfate Production ◽  
Particle Activation ◽  
Aerosol Activation

Abstract. A parameterization for cloud processing is presented that calculates activation of aerosol particles to cloud drops, cloud drop size, and pH-dependent aqueous phase sulfur chemistry. The parameterization is implemented in the global aerosol-climate model ECHAM5-HAM. The cloud processing parameterization uses updraft speed, temperature, and aerosol size and chemical parameters simulated by ECHAM5-HAM to estimate the maximum supersaturation at the cloud base, and subsequently the cloud drop number concentration (CDNC) due to activation. In-cloud sulfate production occurs through oxidation of dissolved SO2 by ozone and hydrogen peroxide. The model simulates realistic distributions for annually averaged CDNC although it is underestimated especially in remote marine regions. On average, CDNC is dominated by particles from the accumulation mode, with smaller contributions from the Aitken and coarse modes. The simulations indicate that in-cloud sulfate production is a potentially important source of accumulation mode sized cloud condensation nuclei, due to chemical growth of activated Aitken particles and to enhanced coalescence of processed particles. The strength of this source depends on the distribution of produced sulfate over the activated modes. This distribution is affected by uncertainties in many parameters that play a direct role in particle activation, such as the updraft velocity, the aerosol chemical composition and the organic solubility, and the simulated CDNC is found to be relatively sensitive to these uncertainties.

scholarly journals Evidence of mineral dust altering cloud microphysics and precipitation

2008 ◽  
Vol 8 (6) ◽  
pp. 18893-18910 ◽  
Author(s):  
Q.-L. Min ◽  
R. Li ◽  
B. Lin ◽  
E. Joseph ◽  
S. Wang ◽  
...  
Keyword(s):  
Mineral Dust ◽  
Heavy Precipitation ◽  
Cloud Microphysics ◽  
Mesoscale Convective Systems ◽  
Size Spectrum ◽  
Convective Systems ◽  
Mesoscale Convective ◽  
Cloud Ice ◽  
The Impact ◽  
Light Precipitation

Abstract. Multi-platform and multi-sensor observations are employed to investigate the impact of mineral dust on cloud microphysical and precipitation processes in mesoscale convective systems. It is clearly evident that for a given convection strength,small hydrometeors were more prevalent in the stratiform rain regions with dust than in those regions that were dust free. Evidence of abundant cloud ice particles in the dust sector, particularly at altitudes where heterogeneous nucleation process of mineral dust prevails, further supports the observed changes of precipitation. The consequences of the microphysical effects of the dust aerosols were to shift the precipitation size spectrum from heavy precipitation to light precipitation and ultimately suppressing precipitation.

scholarly journals Impact of Aerosol-Cloud Cycling on Aqueous Secondary Organic Aerosol Formation

2019 ◽  
Author(s):  
William G. Tsui ◽  
Joseph L. Woo ◽  
V. Faye McNeill
Keyword(s):  
Organic Acids ◽  
Aqueous Phase ◽  
Atmospheric Aerosols ◽  
Organic Material ◽  
Time Of Day ◽  
Aerosol Formation ◽  
Cloud Processing ◽  
Aerosol Mass ◽  
Phase Chemistry ◽  
The Impact

Chemical processing of organic material in aqueous atmospheric aerosols and cloudwater is known to form secondary organic aerosols (SOA), although the extent to which each of these processes contributes to total aerosol mass is unclear. In this study, we use GAMMA 5.0, a photochemical box model with coupled gas and aqueous-phase chemistry, to consider the impact of aqueous organic reactions in both aqueous aerosols and clouds on isoprene epoxydiol (IEPOX) SOA over a range of pH for both aqueous phases, including cycling between cloud and aerosol within a single simulation. Low-pH aqueous aerosol, in the absence of organic coatings or other morphology which may limit uptake of IEPOX, is found to be an efficient source of IEPOX SOA, consistent with previous work. Cloudwater at pH 4 or lower is also found to be a potentially significant source of IEPOX SOA. This phenomenon is primarily attributed to the relatively high uptake of IEPOX to clouds as a result of higher water content in clouds as compared to aerosol. For more acidic cloudwater, the aqueous organic material is comprised primarily of IEPOX SOA and lower-volatility organic acids. For both cloudwater and aqueous aerosol, pH is the most significant factor considered in this study in determining the mass of aqueous phase organic acids and IEPOX SOA. Other factors, such as the time of day or sequence of aerosol-to-cloud or cloud-to-aerosol transitions, contribute to less than 15% difference in the final aqSOA fractional composition. The potential significance of cloud processing as a contributor to IEPOX SOA production could account for discrepancies between predicted IEPOX SOA mass from atmospheric models and measured ambient IEPOX SOA mass, or observations of IEPOX SOA in locations where mass transfer limitations are expected in aerosol particles.

scholarly journals Influence of Rain-Rate Initialization, Cloud Microphysics, and Cloud Torques on Hurricane Intensity

2011 ◽  
Vol 139 (2) ◽  
pp. 627-649 ◽  
Author(s):  
S. Pattnaik ◽  
C. Inglish ◽  
T. N. Krishnamurti
Keyword(s):  
Angular Momentum ◽  
Rain Rate ◽  
Velocity Structure ◽  
Mesoscale Model ◽  
Initial Conditions ◽  
Cloud Microphysics ◽  
Hurricane Intensity ◽  
Storm Intensity ◽  
Intensity Changes ◽  
The Impact

Abstract This study examines the impact of rain-rate initialization (RINIT), microphysical modifications, and cloud torques (in the context of angular momentum) on hurricane intensity forecasts using a mesoscale model [the Advanced Research Weather Research and Forecasting model (ARW-WRF)] at a cloud-resolving resolution of 2.7 km. The numerical simulations are performed in a triple-nested manner (25, 8.3, and 2.7 km) for Hurricane Dennis of 2005. Unless mentioned otherwise, all the results discussed are from the innermost grid with finest resolution (2.7 km). It is found that the model results obtained from the RINIT technique demonstrated robust improvement in hurricane structure, track, and intensity forecasts compared to the control experiment (CTRL; i.e., without RINIT). Thereafter, using RINIT initial conditions datasets three sensitive experiments are designed by modifying specific ice microphysical parameters (i.e., temperature-independent snow intercept parameter, doubling number of concentrations of ice, and ice crystal diameter) within the explicit parameterization scheme [i.e., the WRF Single-Moment 6-class (WSM6)]. It is shown that the experiment with enhanced ice mass concentration and temperature-independent snow intercept parameter produces the strongest and weakest storms, respectively. The results suggest that the distributions of hydrometeors are also impacted by the limited changes introduced in the microphysical scheme (e.g., the quantitative amount of snow drastically reduced to 0.1–0.2 g kg−1 when the intercept parameter of snow is made independent of temperature). It is noted that the model holds ice at a warmer temperature for a longer time with a temperature-independent intercept parameter. These variations in hydrometeor distribution in the eyewall region of the storm affect diabatic heating and vertical velocity structure and modulated the storm intensity. However, irrespective of the microphysical changes the quantitative amount of graupel hydrometeors remained nearly unaffected. Finally, the indirect effect of microphysical modifications on storm intensity through angular momentum and cloud torques is examined. A formulation to predict the short-term changes in the storm intensity using a parcel segment angular momentum budget method is developed. These results serve to elucidate the indirect impact of microphysical modifications on tropical cyclone intensity changes through modulation in cloud torque magnitude.

scholarly journals Increase of the aerosol hygroscopicity by cloud processing in a mesoscale convective system: a case study from the AMMA campaign

2008 ◽  
Vol 8 (23) ◽  
pp. 6907-6924 ◽  
Author(s):  
S. Crumeyrolle ◽  
L. Gomes ◽  
P. Tulet ◽  
A. Matsuki ◽  
A. Schwarzenboeck ◽  
...  
Keyword(s):  
Cloud Condensation Nuclei ◽  
Mesoscale Convective System ◽  
Atmospheric Model ◽  
Dust Particles ◽  
Convective System ◽  
Cloud Processing ◽  
Before And After ◽  
Mesoscale Convective ◽  
The Impact ◽  
Aerosol Properties

Abstract. Aerosol properties were measured during an airborne campaign experiment that took place in July 2006 in West Africa within the framework of the African Monsoon Multidisciplinary Analyses (AMMA). The goal of the present study was to determine the main microphysical processes that affect the aerosols during the passage of a mesoscale convective system (MCS) over the region of Niamey in Niger. A significant change in the aerosol profiles measured before and after the passage of the MCS was found in a layer located between 1300 and 3000 m, where the aerosol concentration drastically decreased after the passage of the MCS. Concurrently, a significant increase in the cloud condensation nuclei (CCN) fraction was also observed during the post-MCS period in the same layer. Moreover, the results of the elemental composition analyses of individual particles collected in this layer after the MCS passage have shown higher contributions of sulfate, nitrate and chloride to the total aerosol mass. A mesoscale atmospheric model with on-line dust parameterization and Lagrangian backtrajectories was used to interpret the impact of the MCS on the aerosol properties. The results of the simulation show that the MCS 1) generates dust particles at the surface in the gust front of the system and washout of particles during the system precipitation, 2) modifies the aerosol mixing state (intensive aerosol property) through cloud processing, and 3) enhances CCN activity of particles through coating by soluble material.

scholarly journals Aerosol effects on deep convection: the propagation of aerosol perturbations through convective cloud microphysics

2019 ◽  
Vol 19 (4) ◽  
pp. 2601-2627 ◽  
Author(s):  
Max Heikenfeld ◽  
Bethan White ◽  
Laurent Labbouz ◽  
Philip Stier
Keyword(s):  
Latent Heat ◽  
Cloud Condensation Nuclei ◽  
Cloud Microphysics ◽  
Latent Heating ◽  
Microphysics Scheme ◽  
Convective Clouds ◽  
Wide Range ◽  
Microphysical Processes ◽  
Aerosol Effects ◽  
The Impact

Abstract. The impact of aerosols on ice- and mixed-phase processes in deep convective clouds remains highly uncertain, and the wide range of interacting microphysical processes is still poorly understood. To understand these processes, we analyse diagnostic output of all individual microphysical process rates for two bulk microphysics schemes in the Weather and Research Forecasting model (WRF). We investigate the response of individual processes to changes in aerosol conditions and the propagation of perturbations through the microphysics all the way to the macrophysical development of the convective clouds. We perform simulations for two different cases of idealised supercells using two double-moment bulk microphysics schemes and a bin microphysics scheme. The simulations cover a comprehensive range of values for cloud droplet number concentration (CDNC) and cloud condensation nuclei (CCN) concentration as a proxy for aerosol effects on convective clouds. We have developed a new cloud tracking algorithm to analyse the morphology and time evolution of individually tracked convective cells in the simulations and their response to the aerosol perturbations. This analysis confirms an expected decrease in warm rain formation processes due to autoconversion and accretion for more polluted conditions. There is no evidence of a significant increase in the total amount of latent heat, as changes to the individual components of the integrated latent heating in the cloud compensate each other. The latent heating from freezing and riming processes is shifted to a higher altitude in the cloud, but there is no significant change to the integrated latent heat from freezing. Different choices in the treatment of deposition and sublimation processes between the microphysics schemes lead to strong differences including feedbacks onto condensation and evaporation. These changes in the microphysical processes explain some of the response in cloud mass and the altitude of the cloud centre of gravity. However, there remain some contrasts in the development of the bulk cloud parameters between the microphysics schemes and the two simulated cases.

scholarly journals Evidence of mineral dust altering cloud microphysics and precipitation

2009 ◽  
Vol 9 (9) ◽  
pp. 3223-3231 ◽  
Author(s):  
Q.-L. Min ◽  
R. Li ◽  
B. Lin ◽  
E. Joseph ◽  
S. Wang ◽  
...  
Keyword(s):  
Mineral Dust ◽  
Heavy Precipitation ◽  
Cloud Microphysics ◽  
Mesoscale Convective Systems ◽  
Size Spectrum ◽  
Convective Systems ◽  
Mesoscale Convective ◽  
Cloud Ice ◽  
The Impact ◽  
Light Precipitation

Abstract. Multi-platform and multi-sensor observations are employed to investigate the impact of mineral dust on cloud microphysical and precipitation processes in mesoscale convective systems. For a given convective strength, small hydrometeors were more prevalent in the stratiform rain regions with dust than in those regions that were dust free. Evidence of abundant cloud ice particles in the dust sector, particularly at altitudes where heterogeneous nucleation of mineral dust prevails, further supports the observed changes of precipitation. The consequences of the microphysical effects of the dust aerosols were to shift the precipitation size spectrum from heavy precipitation to light precipitation and ultimately suppressing precipitation.

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