Reduction of Radioactive Cesium in Contaminated Soil Through Heat Treatment

2017 ◽  
Vol 9 (12) ◽  
pp. 2161-2165
Author(s):  
Byoung-Jik Kim ◽  
Min-Wook Oh
2015 ◽  
Vol 84 (1) ◽  
pp. 9-16 ◽  
Author(s):  
Naoki Ogata ◽  
Toshirou Fujita ◽  
Masako Kato

2013 ◽  
Vol 8 (2) ◽  
pp. 297-310
Author(s):  
Hideto HORAI ◽  
Masahiro KAMIO ◽  
Takeshi KAMEI

Author(s):  
Guilhermina Torrao ◽  
Robert Carlino ◽  
Steve L. Hoeffner ◽  
James D. Navratil

Plutonium (239/240Pu) contamination in soils is an environmental concern at many U.S. Department of Energy (DOE) sites. Remediation actions have been attempted using different technologies, and clean-up plans have been implemented at several sites, such as the Nevada Test Site (NTS). During the 1950’s and early 1960’s, nuclear weapons testing at and near the NTS resulted in soil contaminated with plutonium particles. Clean-up efforts are continuing using conventional remediation techniques. However, the DOE desires to obtain technologies that can further reduce risks, reduce clean-up costs, and reduce the volume of contaminated soil for disposal. Low levels of plutonium contamination are distributed somewhat uniformly throughout the NTS soils and, as a result, it is difficult to obtain volume reductions above 70%. The subject of this research was to characterize the plutonium-contaminated soil from the Tonopah Test Range (TTR) north of the NTS. In order to select remediation methods, it is important to gain a better understanding of how plutonium is bound to the contaminated soil; thus, size separation, magnetic separation, and the sequential extraction (SE) methods were used for this purpose. The SE method consisted of targeting five operationally defined geochemical phases: ion exchangeable, bound to carbonates, bound to iron and manganese oxides (reducible), bound to organic matter, and resistant. Radiometric measurements were used to determine plutonium in each of these defined phases in the soil. Selected stable elements were also determined, to compare the operation of the SE method to other investigators. The SE experiments were performed with two types of samples: soil without heat treatment and soil with heat treatment. The MF treatment was used to destroy the organic content in the soil so as to further evaluate the SE procedure. Particle size analysis indicated that approximately 37% of the TTR soil by weight was larger than 300 micrometers and this fraction contained little plutonium, < 100 pCi/g. Thus, size separation may be useful as part of a remediation process. Magnetic separation tests showed that the magnetic fraction of the TTR soils is very small, and the non-magnetic fraction still contained the majority of the plutonium. Thus, a magnetic separation step in a treatment process would not be useful. Following SE, analysis results of the stable elements agreed with reported values. The SE results also indicated an association of plutonium with the organic and resistant defined phases. The main change in 239/240Pu distribution following heat treatment was an increase of plutonium recovery in the reducible phase. The SE results showed that fairly aggressive chemical treatment would be required if leaching were part of a remediation process.


2013 ◽  
Vol 1 ◽  
pp. 08003
Author(s):  
S. R. Mallampati ◽  
Y. Mitoma ◽  
T. Okuda ◽  
S. Sakita ◽  
M. Kakeda

Electronics ◽  
2021 ◽  
Vol 10 (22) ◽  
pp. 2833
Author(s):  
Sujung Min ◽  
Kwang-Hoon Ko ◽  
Bumkyung Seo ◽  
JaeHak Cheong ◽  
Changhyun Roh ◽  
...  

The miniaturization and usability of radiation detectors make it increasingly possible to use mobile instruments to detect and monitor gamma radiations. Here, a Bluetooth-based mobile detection system for integrated interaction in a backpack was designed and implemented to smart equipment for the detection of radioactive cesium on contaminated soil. The radiation measurement system was demonstrated in the form of a backpack using a quantum dot (QD)-loaded plastic scintillator manufactured and prepared directly in this study, and it can be measured by a person in the wireless framework of integrated interaction. The QD-loaded plastic scintillator was measured after setting the distance from the contaminated soil to 20, 50, and 100 mm. As a result, the detection efficiency of the commercial plastic scintillator (EJ-200) was calculated to be 11.81% and that of the QD-loaded plastic scintillator was 15.22%, which proved the higher detection efficiency performance than the commercial plastic scintillator. The measurement result was transmitted to a personal computer using Bluetooth as a portable system. In the future, this wireless system design could be expanded as a wireless communication system equipped with a global positioning system to detect and measure radioactively contaminated environments.


2012 ◽  
Vol 22 (01n02) ◽  
pp. 13-19 ◽  
Author(s):  
K. ISHII ◽  
A. TERAKAWA ◽  
S. MATSUYAMA ◽  
A. HASEGAWA ◽  
K. NAGAKUBO ◽  
...  

We studied the structure of radioactive cesium distribution in soil and found the exponential dependence. This behavior could be explained theoretically. We developed a useful method to decontaminate the soil contaminated with radioactive cesium atoms. We applied our method to the contaminated school yards of elementary schools of Marumori town and decontaminated total area of about 7000 m2.


2002 ◽  
Vol 2002.12 (0) ◽  
pp. 288-290
Author(s):  
Mamoru ARAOKA ◽  
Satoshi OKUNO ◽  
Reiji TAHARA ◽  
Hiroki HONDA ◽  
Takeshi AMARI ◽  
...  

2020 ◽  
Vol 10 (18) ◽  
pp. 6471
Author(s):  
Ai Van Tran ◽  
Makoto Yanaga

Radiocontaminated soil in a paddy field in the Iitate village in Fukushima was treated with an industrial paper sludge carbon (PSC) prior to growing rice in May 2011. The results showed that the sum of the activity concentrations of 134Cs and 137Cs in the polished rice harvested in October 2011 was 30 Bq·kg−1, a level much lower than the Japanese governmental safeguard value of 100 Bq·kg−1. Upon contacting with the contaminated soil, the contents of calcium, magnesium, copper, potassium, and barium in the PSC were decreased. Among the PSCs impregnated with various chlorides and sulfates of the previously mentioned minerals, potassium chloride, copper sulfate, magnesium sulfate, and potassium sulfate yielded higher decontamination degrees compared to the original PSC. The results imply that radioactive cesium in the soil exchanges cations with these minerals.


2018 ◽  
Vol 316 (3) ◽  
pp. 1213-1219
Author(s):  
Il Park ◽  
Jin O Lee ◽  
Tae Gwan Do ◽  
Min Jun Kim ◽  
A Ra Go ◽  
...  

Sign in / Sign up

Export Citation Format

Share Document