scholarly journals Self-Assembly of Ternary Particles for Tough Colloidal Crystals with Vivid Structure Colors

2013 ◽  
Vol 2013 ◽  
pp. 1-14 ◽  
Author(s):  
Binfu Bao ◽  
Duo Liu ◽  
Youyou Yang ◽  
Zhehong Shen ◽  
Bo You

Self-assembly of colloidal spheres is the most frequently used method for structural colors, but the chroma of the structural colors is usually so low that people cannot observe it under natural conditions. This paper presents a facile method for fabrications of vivid structural colors by doping carbon black into the self-assembly of colloidal polymer spheres and nanosilica particles. This approach can generate very gorgeous structural colors which can be very easily seen under natural conditions. The fabrication conditions for the self-assembly of composite dispersions of polymer/silica/carbon black were optimized to obtain colloidal crystals with vivid colors. Thus, robust mechanical properties, large-scale, and brilliant structural colors can guarantee the obtained crystal films to find practical applications, which are demonstrated by the fact that the successful applications of structural colors beautify the original simple and tedious surface of bamboo strand board (BSB).

2019 ◽  
Vol 4 (1) ◽  
pp. 68-74
Author(s):  
Aleš Dakskobler ◽  
Matjaz Valant

Background: Studies on the formation of colloidal crystals in concentrated suspensions have mainly been based on dispersed suspensions with a repulsive inter-particle potential of hard or nearly hard spheres. The self-assembly in weakly-flocculated suspensions has still been unrealized. Here, we report on the formation of ordered structures in concentrated suspensions of nearly-hard spherical particles with weakly-attractive inter-particle interactions that are an order of magnitude higher than the particles’ thermal energy. Methods: In our case, the self-assembly in such suspensions is not thermodynamically driven, but an external shear force must be applied. The driving force for the particles’ ordering is an increase in the inter-particle interactions. This manifests itself in a decrease in the average angle between the interparticle interaction direction and the applied shear stress direction. Results: For a successful ordering into a large-scale closed packed assembly, the external shear force must not exceed the inter-particle attractive interaction for the minimum possible average angle (as in the closed packed structures) but be high enough to enable the particles to move in the highly loaded suspension. Conclusion: The developed method for the self-assembly of the weakly flocculated systems can be applied very generally e.g. a control over a composition of heterogeneous colloidal crystals, manufacturing of the large-scale photonic crystals or preparation of very densely packed compacts of particles needed for the production of sintered ceramics.


Author(s):  
Zhengting Zhang ◽  
Guiyun Yi ◽  
Xiaodong Wang ◽  
Peng Li ◽  
Zhuoyan Wan ◽  
...  

Micromachines ◽  
2020 ◽  
Vol 11 (5) ◽  
pp. 473 ◽  
Author(s):  
Pengcheng Zhang ◽  
Xi Chen ◽  
Hui Yang

A large-scale homogenized photonic nanojet array with defined pattern and spacing facilitates practical applications in super-resolution imaging, subwavelength-resolution nanopatterning, nano objects trapping and detection technology. In this paper, we present the fabrication of a large-scale photonic nanojet array via the template-assisted self-assembly (TASA) approach. Templates of two-dimensional (2D) large-scale microwell array with defined pattern and spacing are fabricated. Melamine microspheres with excellent size uniformity are utilized to pattern on the template. It is found that microwells can be filled at a yield up to 95%. These arrayed microspheres on the template serve as microlenses and can be excited to generate large-scale photonic nanojets. The uniformly-sized melamine spheres are beneficial for the generation of a homogenized photonic nanojet array. The intensity of the photonic nanojets in water is as high as ~2 fold the background light signal. Our work shows a simple, robust, and fast means for the fabrication of a large-scale homogenized photonic nanojet array.


2020 ◽  
Vol 4 (8) ◽  
pp. 2409-2417
Author(s):  
Mengfan Wu ◽  
Chuyan Zhang ◽  
Fujing Wei ◽  
Huifang An ◽  
Xiaqing Wang ◽  
...  

This is the first time that a hydrogel interface has been used as an assembly interface for the self-assembly of photonic crystals with excellent performances.


Soft Matter ◽  
2020 ◽  
Vol 16 (26) ◽  
pp. 6056-6062 ◽  
Author(s):  
Xianggui Ye ◽  
Bamin Khomami

Large-scale dissipative particle dynamics (DPD) simulations have been performed to investigate the self-assembly of over 20 000 linear diblock copolymer chains in a selective solvent.


Biology Open ◽  
2021 ◽  
Vol 10 (3) ◽  
pp. bio056432 ◽  
Author(s):  
Shohei Yamamoto ◽  
Ryoichi Yabuki ◽  
Daiju Kitagawa

ABSTRACTThe deuterosome is a non-membranous organelle involved in large-scale centriole amplification during multiciliogenesis. Deuterosomes are specifically assembled during the process of multiciliogenesis. However, the molecular mechanisms underlying deuterosome formation are poorly understood. In this study, we investigated the molecular properties of deuterosome protein 1 (Deup1), an essential protein involved in deuterosome assembly. We found that Deup1 has the ability to self-assemble into macromolecular condensates both in vitro and in cells. The Deup1-containing structures formed in multiciliogenesis and the Deup1 condensates self-assembled in vitro showed low turnover of Deup1, suggesting that Deup1 forms highly stable structures. Our biochemical analyses revealed that an increase of the concentration of Deup1 and a crowded molecular environment both facilitate Deup1 self-assembly. The self-assembly of Deup1 relies on its N-terminal region, which contains multiple coiled coil domains. Using an optogenetic approach, we demonstrated that self-assembly and the C-terminal half of Deup1 were sufficient to spatially compartmentalize centrosomal protein 152 (Cep152) and polo like kinase 4 (Plk4), master components for centriole biogenesis, in the cytoplasm. Collectively, the present data suggest that Deup1 forms the structural core of the deuterosome through self-assembly into stable macromolecular condensates.This article has an associated First Person interview with the first author of the paper.


2013 ◽  
Vol 850-851 ◽  
pp. 92-95
Author(s):  
Yong Wan ◽  
Zhong Yu Cai ◽  
Ming Hui Jia ◽  
Chao Li ◽  
Wan Qin Yang

Silica and polystyrene (PS) microspheres assembled on two quite different patterned silicon substrates, cross-like pillar pattern and eye-like pattern, respectively. The results indicated that the surface pattern imposes a predetermined lattice orientation in colloidal crystals (CCs). Other influent factors, such as microsphere size, the altitude of pattern and the concentration of colloidal suspension, may also play an important role on the self-assembly process.


2018 ◽  
Vol 2018 ◽  
pp. 1-13 ◽  
Author(s):  
Ingrid Saba ◽  
Weronika Jakubowska ◽  
Stéphane Bolduc ◽  
Stéphane Chabaud

Twenty years ago, Dr. François A. Auger, the founder of the Laboratory of Experimental Organogenesis (LOEX), introduced the self-assembly technique. This innovative technique relies on the ability of dermal fibroblasts to produce and assemble their own extracellular matrix, differing from all other tissue-engineering techniques that use preformed synthetic scaffolds. Nevertheless, the use of the self-assembly technique was limited for a long time due to its main drawbacks: time and cost. Recent scientific breakthroughs have addressed these limitations. New protocol modifications that aim at increasing the rate of extracellular matrix formation have been proposed to reduce the production costs and laboratory handling time of engineered tissues. Moreover, the introduction of vascularization strategies in vitro permits the formation of capillary-like networks within reconstructed tissues. These optimization strategies enable the large-scale production of inexpensive native-like substitutes using the self-assembly technique. These substitutes can be used to reconstruct three-dimensional models free of exogenous materials for clinical and fundamental applications.


Nanoscale ◽  
2019 ◽  
Vol 11 (12) ◽  
pp. 5450-5459 ◽  
Author(s):  
Pritam Kumar Jana ◽  
Bortolo Matteo Mognetti

Functionalized surfaces direct colloidal layer deposition by enhancing particle–particle interactions.


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