Kinetics of flowing dispersions. X. Oscillations in optical properties of streaming suspensions of spheroids

1977 ◽  
Vol 55 (24) ◽  
pp. 4243-4256 ◽  
Author(s):  
A. Okagawa ◽  
S. G. Mason

Transients in angular light scattering and turbidity of dilute suspensions of nearly monodisperse spheroidal particles undergoing simple shear flow have been investigated by combining Rayleigh–Debye light scattering theory for single dielectric particles with fluid mechanical theory for the orientation distributions of particle assemblies in shear flow. Applying shear to an initially isotropic suspension causes the orientation distributions and thus the angular scattering coefficients to oscillate. Various geometrical arrangements are considered with a view to selecting those that will maximize such rheo-optical effects.By calculating the optical scattering cross section of a single particle, the turbidity of a suspension is obtained; like the scattering coefficient, it undergoes oscillations that are damped by (1) the inevitable spread in particle shape and volume in real systems, (2) shear-induced particle interactions, and (3) rotary Brownian motion. The rates of damping, expressed as relaxation times, are considered for the three mechanisms acting alone or in concert.Preliminary measurements of the turbidity of dilute suspensions of hardened human red blood cells confirm this general pattern of behavior. Apart from their intrinsic interest, such rheo-optical effects can be used to determine a number of useful properties of dispersions.

1992 ◽  
Vol 238 ◽  
pp. 277-296 ◽  
Author(s):  
Carl A. Stover ◽  
Donald L. Koch ◽  
Claude Cohen

The orientations of fibres in a semi-dilute, index-of-refraction-matched suspension in a Newtonian fluid were observed in a cylindrical Couette device. Even at the highest concentration (nL3 = 45), the particles rotated around the vorticity axis, spending most of their time nearly aligned in the flow direction as they would do in a Jeffery orbit. The measured orbit-constant distributions were quite different from the dilute orbit-constant distributions measured by Anczurowski & Mason (1967b) and were described well by an anisotropic, weak rotary diffusion. The measured ϕ-distributions were found to be similar to Jeffery's solution. Here, ϕ is the meridian angle in the flow-gradient plane. The shear viscosities measured by Bibbo (1987) compared well with the values predicted by Shaqfeh & Fredrickson's theory (1990) using moments of the orientation distribution measured here.


1998 ◽  
Vol 366 ◽  
pp. 289-310 ◽  
Author(s):  
Y. ALMOG ◽  
I. FRANKEL

We study the respective effects of shear rate and of external field intensity and direction on the contribution to the bulk stress of Brownian dipolar axisymmetric particles suspended in a steady macroscopically homogeneous shear flow of an incompressible Newtonian fluid. Towards this end we obtain the steady orientational distribution and make use of existing general dynamic theories of dilute suspensions. The calculation focuses on the limit of weak rotary diffusion. Thus, unlike previous analyses, the present contribution is not restricted to weak shear effects.Explicit results are presented for the bulk stress when the external field acts in the plane of the simple shear flow. In cases when the deterministic rotary motion possesses a single sufficiently stable node a simple unified description of the respective effects of both the intensity and azimuthal direction of the external field is provided by the boundary-layer approximation. This approximation enables a qualitative explanation of existing numerical results as well as furnishing quantitatively accurate analytical results at relatively moderate values of the rotary Peclét number and the Langevin parameter (∼10). Furthermore, at still larger values of these parameters use of the present asymptotic approximation is clearly preferable since the numerical schemes rapidly deteriorate when steep orientational gradients appear.Singularities of the bulk stress are rationalized in terms of the corresponding deterministic rotary motion. This is particularly interesting because some of these singular phenomena (e.g. those associated with an ‘intermediate regime’ of the field intensity and direction, for which more than one stable attractor exists in the deterministic problem) have no counterparts in suspensions of dipolar spheres or torque-free axisymmetric particles.Finally, the present results obtained for the orientational distribution are also applicable to the study of other aspects of the macroscale description of suspensions of dipolar axisymmetric particles. In this context we mention the extension of continuum modelling of suspensions of swimming micro-organisms so as to enable the analysis of fully developed bioconvection.


Author(s):  
Tobias Merkel ◽  
Julius Henne ◽  
Lena Hecht ◽  
Volker Gräf ◽  
Elke Walz ◽  
...  

2006 ◽  
Vol 91 (9) ◽  
pp. 3415-3424 ◽  
Author(s):  
Juan Jaspe ◽  
Stephen J. Hagen

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