Transverse Noise of Hot Electrons in n-Type Germanium

1971 ◽  
Vol 49 (11) ◽  
pp. 1469-1481 ◽  
Author(s):  
L. G. Hart

This work is an extension of previous analysis of high-field, hot-electron noise in n-type germanium. The previous analysis, developed to explain the author's observations of field-direction (longitudinal) noise, is extended here in an attempt to explain the hot-electron, transverse noise observations of Erlbach and Gunn.In the model adopted, the transverse current fluctuations, resulting from intravalley and intervalley scattering, within the interelectrode volume (electrode area × separation), yield both thermal and intervalley contributions to the noise temperature. For two of the three crystal orientations considered, the intervalley noise is negligible, but in the third case, the two contributions are of the same order.Individual valley currents, populations, and relative intervalley transition rates are calculated from Nathan's analysis, and the Barrie–Burgess theory of high-field transport provides the valley electron temperatures. The intervalley scattering data of Weinreich, Sanders, and White yield absolute values of the intervalley scattering probabilities.Poor agreement is found with the Erlbach–Gunn observations of transverse noise temperature, which may be due to the shunting effect of the portion of the sample exterior to the interelectrode volume.

2020 ◽  
Author(s):  
Hailu Wang ◽  
Fang Wang ◽  
Hui Xia ◽  
Peng Wang ◽  
Tianxin Li ◽  
...  

Abstract In modern electronics and optoelectronics, hot electron behaviors are highly concerned since they determine the performance limit of a device or system, like the associated thermal or power constraint of chips, the Shockley-Queisser limit for solar cell efficiency. Up-to-date, however, the manipulation of hot electrons is mostly based on conceptual interpretations rather than a direct observation. The problem arises from a fundamental fact that energy-differential electrons are mixed up in real-space, making it hard to distinguish them from each other by standard measurements. Here we demonstrate a distinct approach to artificially (spatially) separate hot electrons from cold ones in semiconductor nanowire transistors, which thus offers a unique opportunity to observe and modulate electron occupied state, energy, mobility, and even its path. Such a process is accomplished through the scanning-photocurrent-microscopy (SPCM) measurements by activating the intervalley-scattering events and one-dimensional charge-neutrality rule. Findings discovered here may provide a new degree of freedom in manipulating nonequilibrium electrons for both electronic and optoelectronic applications.


Nanophotonics ◽  
2021 ◽  
Vol 0 (0) ◽  
Author(s):  
Wenhao Wang ◽  
Lucas V. Besteiro ◽  
Peng Yu ◽  
Feng Lin ◽  
Alexander O. Govorov ◽  
...  

Abstract Hot electrons generated in metallic nanostructures have shown promising perspectives for photodetection. This has prompted efforts to enhance the absorption of photons by metals. However, most strategies require fine-tuning of the geometric parameters to achieve perfect absorption, accompanied by the demanding fabrications. Here, we theoretically propose a Ag grating/TiO2 cladding hybrid structure for hot electron photodetection (HEPD) by combining quasi-bound states in the continuum (BIC) and plasmonic hot electrons. Enabled by quasi-BIC, perfect absorption can be readily achieved and it is robust against the change of several structural parameters due to the topological nature of BIC. Also, we show that the guided mode can be folded into the light cone by introducing a disturbance to become a guided resonance, which then gives rise to a narrow-band HEPD that is difficult to be achieved in the high loss gold plasmonics. Combining the quasi-BIC and the guided resonance, we also realize a multiband HEPD with near-perfect absorption. Our work suggests new routes to enhance the light-harvesting in plasmonic nanosystems.


2020 ◽  
Vol 29 (5) ◽  
pp. 058505
Author(s):  
Kang-Min Zhou ◽  
Wei Miao ◽  
Yue Geng ◽  
Yan Delorme ◽  
Wen Zhang ◽  
...  

2021 ◽  
Author(s):  
Sergio Kogikoski Junior ◽  
Anushree Dutta ◽  
Ilko Bald

<p>Using hot charge carriers far from a plasmonic nanoparticle surface is very attractive for many applications in catalysis and nanomedicine, and will lead to a better understanding of plasmon-induced processes, such as hot charge carrier or heat driven chemical reactions. Herein we show that DNA is able to transfer hot electrons generated by a silver nanoparticle over several nanometers to drive a chemical reaction in a molecule non-adsorbed on the surface. For this we use 8-bromo-adenosine introduced in different positions within a double stranded DNA oligonucleotide. The DNA is also used to assemble the nanoparticles into superlattices enabling the use of surface enhanced Raman scattering to track the decomposition reaction. To prove the DNA mediated transfer, the probe molecule was insulated from the charge carriers source, which hindered the reaction. The results indicate that DNA can provide an attractive platform to study the transfer of hot electrons, leading to the future development of more advanced plasmonic catalysts. </p>


2019 ◽  
Vol 10 (1) ◽  
Author(s):  
Lifeng Wang ◽  
Zongwei Chen ◽  
Guijie Liang ◽  
Yulu Li ◽  
Runchen Lai ◽  
...  

Abstract Hot electrons can dramatically improve the efficiency of solar cells and sensitize energetically-demanding photochemical reactions. Efficient hot electron devices have been hindered by sub-picosecond intraband cooling of hot electrons in typical semiconductors via electron-phonon scattering. Semiconductor quantum dots were predicted to exhibit a “phonon bottleneck” for hot electron relaxation as their quantum-confined electrons would couple very inefficiently to phonons. However, typical cadmium selenide dots still exhibit sub-picosecond hot electron cooling, bypassing the phonon bottleneck possibly via an Auger-like process whereby the excessive energy of the hot electron is transferred to the hole. Here we demonstrate this cooling mechanism can be suppressed in copper-doped cadmium selenide colloidal quantum dots due to femtosecond hole capturing by copper-dopants. As a result, we observe a lifetime of ~8.6 picosecond for 1Pe hot electrons which is more than 30-fold longer than that in same-sized, undoped dots (~0.25 picosecond).


1960 ◽  
Vol 15 (1) ◽  
pp. 207-208 ◽  
Author(s):  
Motoichi Shibuya ◽  
Wataru Sasaki

Author(s):  
D. R. Rusby ◽  
C. D. Armstrong ◽  
G. G. Scott ◽  
M. King ◽  
P. McKenna ◽  
...  

After a population of laser-driven hot electrons traverses a limited thickness solid target, these electrons will encounter the rear surface, creating TV/m fields that heavily influence the subsequent hot-electron propagation. Electrons that fail to overcome the electrostatic potential reflux back into the target. Those electrons that do overcome the field will escape the target. Here, using the particle-in-cell (PIC) code EPOCH and particle tracking of a large population of macro-particles, we investigate the refluxing and escaping electron populations, as well as the magnitude, spatial and temporal evolution of the rear surface electrostatic fields. The temperature of both the escaping and refluxing electrons is reduced by 30%–50% when compared to the initial hot-electron temperature as a function of intensity between $10^{19}$ and $10^{21}~~\text{W}/\text{cm}^{2}$ . Using particle tracking we conclude that the highest energy internal hot electrons are guaranteed to escape up to a threshold energy, below which only a small fraction are able to escape the target. We also examine the temporal characteristic of energy changes of the refluxing and escaping electrons and show that the majority of the energy change is as a result of the temporally evolving electric field that forms on the rear surface.


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