MEASUREMENT OF RADIATIVE CAPTURE RESONANCE INTEGRALS IN A THERMAL REACTOR SPECTRUM, AND THE THERMAL CROSS SECTION OF Pu-240

1960 ◽  
Vol 38 (1) ◽  
pp. 57-77 ◽  
Author(s):  
W. H. Walker ◽  
C. H. Westcott ◽  
T. K. Alexander

An apparatus is described which detects γ-rays emitted by a thin target placed in a well-denned neutron beam. It has been used to determine the Cd ratios of Au and Pu-240, from which the ratio of the resonance integral to the 2200 m/s cross section for radiative neutron capture in Pu-240 has been deduced, using Au as a reference standard. Using this ratio and previously measured values of the resonance integral of Pu-240 and its effective cross section in two positions in the NRX reactor, three separate estimates of the 2200 m/s cross section of Pu-240 have been made. The mean value is 270 ± 17 barns.In an auxiliary experiment to indicate the shape of the epithermal spectrum of the neutron beam, the activation Cd ratios of Mn and In were compared with that of Au. These results, combined with the known 2200 m/s capture cross sections of these nuclides, yield new values of the radiative capture resonance integrals for both Mn and In.

1972 ◽  
Vol 50 (17) ◽  
pp. 1978-1986
Author(s):  
M. D. Ricabarra ◽  
R. Turjanski ◽  
G. H. Ricabarra

Values of the reduced activation resonance integral relative to the thermal cross section I′/σ0 of 74Ge and 76Ge were determined relative to gold by measuring cadmium ratios in a reactor spectrum.A lithium-drifted germanium γ-ray spectrometer was used to resolve the activities of the samples.The results for 74Ge are I′/σ0 = 1.514 ± 0.031 and I′ = 0.681 ± 0.123 b with an assumed σ0 = 0.45 ± 0.08 b; for 76GeI′/σ0 = 12.00 ± 0.16 and I′ = 1.992 ± 0.359 with an assumed σ0 = 0.166 ± 0.030 b.The values obtained for I′ are in serious disagreement with the values calculated with neutron resonance parameters and confirm previous results obtained in similar keV average resonance spacing isotopes.Due to this fact a careful evaluation of the keV neutron radiative capture cross section and resonance integral for 74Ge was undertaken.The evaluation and comparison with the experimental value of the resonance integral shows first that for nuclides with an average resonance spacing of keV the unresolved resonance integral has been seriously underestimated in many evaluations, and second that between 10 and 100 keV, resonance integrals calculated with smooth low resolution activation cross sections give a better calculation of neutron captures than that obtained with neutron resonance parameters.


1958 ◽  
Vol 36 (7) ◽  
pp. 863-870 ◽  
Author(s):  
A. P. Baerg ◽  
F. Brown ◽  
M. Lounsbury

The effective cross section for the reaction Cs135 (n, γ) Cs136 with reactor neutrons is 10.4 ± 0.5 barns. The measured reaction rate under cadmium yields a value of 61.7 ± 2.3 barns for the resonance integral of Cs135. The thermal cross section is 8.7 ± 0.5 barns as obtained by combining the reaction rates for uncovered and cadmium-covered samples.


2020 ◽  
Vol 34 (32) ◽  
pp. 2050318
Author(s):  
T. G. Naghiyev

(n, p) transmutations in the silicon nitride (Si3N4) nanoparticles by the neutrons at different energies have been studied by computer simulation. The transmutations by neutrons in the nanomaterial were separately investigated for silicon and nitrogen atoms in the Si3N4 particles. Since the effective cross-section of the possible probability of transmutation is different in the various types of silicon and nitrogen atoms, the modeling was performed separately for each stable isotope. The spectra of the effective cross-sections of the (n, p) transmutations for silicon and nitrogen atoms have been studied in relation to each other.


2019 ◽  
Vol 21 ◽  
pp. 160
Author(s):  
A. Kalamara ◽  
R. Vlastou ◽  
M. Diakaki ◽  
M. Kokkoris ◽  
M. Anastasiou ◽  
...  

The 241Am(n,2n)240Am reaction cross section has been measured at neutron beam energy 17.5 MeV, relative to the 27Al(n,α)24Na, 197Au(n,2n)196Au and 93Nb(n,2n)92mNb reference reaction cross sections, using the activation technique. The irradiation was carried out at the Van der Graaff 5.5 MV Tandem accelerator laboratory of NCSR “Demokritos” with monoenergetic neutron beam provided by means of the 3H(d,n)4He reaction, implementing a new Ti-tritiated target. The high purity Am target has been constructed at IRMM, Geel, Belgium and consisted of 40 mg 241Am in the form of AmO2 pressed into pellet with Al2O3 and encapsulated into Al container. Due to this high radioactivity (5 GBq), the Am target was enclosed in a Pb container for safety reasons. After the end of the irradiation, the activity induced by the neutron beam at the target and reference foils, was measured off-line by two 100%, a 50% and a 16% relative efficiency, HPGe detectors.


1993 ◽  
Vol 46 (1) ◽  
pp. 13 ◽  
Author(s):  
LF Phillips

Quasi-classical trajectory calculations have been used to calculate effective collision cross-sections for polar and non-polar molecules with charged and neutral conducting spheres of radius 0.001-0.1 μm over the temperature range 10-400 K. In general the effective cross-section is much larger than the geometrical cross-section, especially for small, highly charged, particles colliding with highly polar molecules at low temperatures. The results may have a bearing on the growth of atmospheric aerosols and of interstellar dust grains.


1968 ◽  
Vol 9 (2-3) ◽  
Author(s):  
J. I. Kim ◽  
F. Adams

SummaryBy neutron activation measurement with a cadmium filter, using gold as a standard monitor, the thermal neutron cross sections and the resonance integrals of


1961 ◽  
Vol 39 (8) ◽  
pp. 1184-1192 ◽  
Author(s):  
W. H. Walker ◽  
R. E. Green

Cadmium ratio measurements have been made in similar lattice positions in ZEEP with thin foils of Sm152 and gold. From a comparison of these cadmium ratios we find[Formula: see text]If gσ0 is assumed to be 212 ± 12 barns, then I′ = 3100 ± 200 barns. On the assumption that only one resonance in Sm152, at 8 ev, contributes appreciably to both the resonance integral and the thermal cross section, it follows that g = 1 and that Γ, the width at half-maximum of the total cross section resonance, is 193 ± 5 milli-ev. Because of the appreciable disagreement between this value and one reported earlier, a new time-of-flight measurement of the resonance parameters has been made, and it is reported in the next paper (Chrien 1961).


1987 ◽  
Vol 65 (6) ◽  
pp. 687-690 ◽  
Author(s):  
D. Počanić ◽  
K. Wang ◽  
C. J. Martoff ◽  
S. S. Hanna ◽  
R. C. Byrd ◽  
...  

A new monochromatic neutron-beam facility has been set up at the Indiana University Cyclotron Facility, primarily for (n, p) reaction measurements at intermediate energies (100–200 MeV). Reported are the experimental layout of the facility and preliminary results of the first measurements: 6Li(n,p)6He cross sections at six angles ranging from Θcm = 0–22°, with En = 118 MeV (laboratory). Good agreement is found between the measured σ(0°) and the cross sections measured for the mirror reaction 6Li(p, n) at 120 and 144 MeV. Results of a distorted wave calculation, while slightly lower, are consistent with the preliminary experimental 0° cross section.


1988 ◽  
Vol 66 (4) ◽  
pp. 330-333 ◽  
Author(s):  
R. K. Y. Singh ◽  
M. Afzal Ansari ◽  
R. P. Gautam ◽  
I. A. Rizvi ◽  
S. Kailas

Radiative neutron capture cross sections for 160Gd have been measured at eight different neutron energies: 0.46 ± 0.04, 0.57 ± 0.04, 0.75 ± 0.04, 0.97 ± 0.20, 1.22 ± 0.19, 1.52 ± 0.17, 2.22 ± 0.17, and 3.05 ± 0.18 MeV. The activation technique has been employed in the present measurement. Our experimental values are compared with the theoretical values calculated using the FISPRO II code, using the most recent set of parameters available in the published literatures.


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