scholarly journals Reducing the aerosol forcing uncertainty using observational constraints on warm rain processes

2020 ◽  
Vol 6 (22) ◽  
pp. eaaz6433 ◽  
Author(s):  
Johannes Mülmenstädt ◽  
Christine Nam ◽  
Marc Salzmann ◽  
Jan Kretzschmar ◽  
Tristan S. L’Ecuyer ◽  
...  

Global climate models (GCMs) disagree with other lines of evidence on the rapid adjustments of cloud cover and liquid water path to anthropogenic aerosols. Attempts to use observations to constrain the parameterizations of cloud processes in GCMs have failed to reduce the disagreement. We propose using observations sensitive to the relevant cloud processes rather than only to the atmospheric state and focusing on process realism in the absence of aerosol perturbations in addition to the process susceptibility to aerosols. We show that process-sensitive observations of precipitation can reduce the uncertainty on GCM estimates of rapid cloud adjustments to aerosols. The feasibility of an observational constraint depends on understanding the precipitation intensity spectrum in both observations and models and also on improving methods to compare the two.

2021 ◽  
Author(s):  
Hao Wang ◽  
Minghuai Wang ◽  
Daniel Rosenfeld ◽  
Yannian Zhu ◽  
Zhibo Zhang

<p>Representing subgrid variability of cloud properties has always been a challenge in global climate models (GCMs). In microphysics schemes, the effects of subgrid cloud variability on warm rain process rates calculated based on mean cloud properties are usually accounted for by scaling process rates by an enhancement factor (EF) that is derived from the subgrid variance of cloud water. In our study, we find that the EF derived from Cloud Layers Unified by Binormals (CLUBB) in Community Earth System Model Version 2 (CESM2) is severely overestimated in most of the oceanic areas, which leads to the strong overestimation in the autoconversion rate. Through an EF formula based on empirical fitting of MODIS, we improve the EF in the liquid phase clouds. Results show that the model has a more reasonable relationship between autoconversion rate, cloud liquid water content (LWC), and droplet number concentration (CDNC) in warm rain simulation. The annual mean liquid cloud fraction (LCF), liquid water path (LWP), and CDNC show obvious increases for marine stratocumulus, where the probability of precipitation (POP) shows an obvious decrease. The annual mean LCF, cloud optical thickness (COT), and shortwave cloud forcing (SWCF) match better with observation. The sensitivity of LWP to aerosol decreases obviously. The sensitivities of LCF, LWP, cloud top droplet effective radius (CER), and COT to aerosol are in better agreement with MODIS, but the model still underestimates the response of cloud albedo to aerosol. These results indicate the importance of representing reasonable subgrid cloud variabilities in the simulation of cloud properties and aerosol-cloud interaction in climate models.</p>


2017 ◽  
Vol 17 (7) ◽  
pp. 4451-4475 ◽  
Author(s):  
Ilissa B. Ocko ◽  
Paul A. Ginoux

Abstract. Anthropogenic aerosols are a key factor governing Earth's climate and play a central role in human-caused climate change. However, because of aerosols' complex physical, optical, and dynamical properties, aerosols are one of the most uncertain aspects of climate modeling. Fortunately, aerosol measurement networks over the past few decades have led to the establishment of long-term observations for numerous locations worldwide. Further, the availability of datasets from several different measurement techniques (such as ground-based and satellite instruments) can help scientists increasingly improve modeling efforts. This study explores the value of evaluating several model-simulated aerosol properties with data from spatially collocated instruments. We compare aerosol optical depth (AOD; total, scattering, and absorption), single-scattering albedo (SSA), Ångström exponent (α), and extinction vertical profiles in two prominent global climate models (Geophysical Fluid Dynamics Laboratory, GFDL, CM2.1 and CM3) to seasonal observations from collocated instruments (AErosol RObotic NETwork, AERONET, and Cloud–Aerosol Lidar with Orthogonal Polarization, CALIOP) at seven polluted and biomass burning regions worldwide. We find that a multi-parameter evaluation provides key insights on model biases, data from collocated instruments can reveal underlying aerosol-governing physics, column properties wash out important vertical distinctions, and improved models does not mean all aspects are improved. We conclude that it is important to make use of all available data (parameters and instruments) when evaluating aerosol properties derived by models.


2005 ◽  
Vol 5 (3) ◽  
pp. 715-737 ◽  
Author(s):  
U. Lohmann ◽  
J. Feichter

Abstract. Aerosols affect the climate system by changing cloud characteristics in many ways. They act as cloud condensation and ice nuclei, they may inhibit freezing and they could have an influence on the hydrological cycle. While the cloud albedo enhancement (Twomey effect) of warm clouds received most attention so far and traditionally is the only indirect aerosol forcing considered in transient climate simulations, here we discuss the multitude of effects. Different approaches how the climatic implications of these aerosol effects can be estimated globally as well as improvements that are needed in global climate models in order to better represent indirect aerosol effects are discussed in this paper.


2020 ◽  
Author(s):  
Zhibo Zhang ◽  
Qianqian Song ◽  
David Mechem ◽  
Vincent Larson ◽  
Jian Wang ◽  
...  

Abstract. In the current global climate models (GCM), the nonlinearity effect of subgrid cloud variations on the parameterization of warm rain process, e.g., the autoconversion rate, is often treated by multiplying the resolved-scale warm ran process rates by a so-called enhancement factor (EF). In this study, we investigate the subgrid-scale horizontal variations and covariation of cloud water content (qc) and cloud droplet number concentration (Nc) in marine boundary layer (MBL) clouds based on the in-situ measurements from a recent field campaign, and study the implications for the autoconversion rate EF in GCMs. Based on a few carefully selected cases from the field campaign, we found that in contrast to the enhancing effect of qc and Nc variations that tends to make EF > 1, the strong positive correlation between qc and Nc results in a suppressing effect that makes tends to make EF 


2011 ◽  
Vol 11 (1) ◽  
pp. 3399-3459 ◽  
Author(s):  
M. Wang ◽  
S. Ghan ◽  
M. Ovchinnikov ◽  
X. Liu ◽  
R. Easter ◽  
...  

Abstract. Much of the large uncertainty in estimates of anthropogenic aerosol effects on climate arises from the multi-scale nature of the interactions between aerosols, clouds and large-scale dynamics, which are difficult to represent in conventional global climate models (GCMs). In this study, we use a multi-scale aerosol-climate model that treats aerosols and clouds across multiple scales to study aerosol indirect effects. This multi-scale aerosol-climate model is an extension of a multi-scale modeling framework (MMF) model that embeds a cloud-resolving model (CRM) within each grid cell of a GCM. The extension allows the explicit simulation of aerosol/cloud interactions in both stratiform and convective clouds on the global scale in a computationally feasible way. Simulated model fields, including liquid water path (LWP), ice water path, cloud fraction, shortwave and longwave cloud forcing, precipitation, water vapor, and cloud droplet number concentration are in agreement with observations. The new model performs quantitatively similar to the previous version of the MMF model in terms of simulated cloud fraction and precipitation. The simulated change in shortwave cloud forcing from anthropogenic aerosols is −0.77 W m−2, which is less than half of that in the host GCM (NCAR CAM5) (−1.79 W m−2) and is also at the low end of the estimates of most other conventional global aerosol-climate models. The smaller forcing in the MMF model is attributed to its smaller increase in LWP from preindustrial conditions (PI) to present day (PD): 3.9% in the MMF, compared with 15.6% increase in LWP in large-scale clouds in CAM5. The much smaller increase in LWP in the MMF is caused by a much smaller response in LWP to a given perturbation in cloud condensation nuclei (CCN) concentrations from PI to PD in the MMF (about one-third of that in CAM5), and, to a lesser extent, by a smaller relative increase in CCN concentrations from PI to PD in the MMF (about 26% smaller than that in CAM5). The smaller relative increase in CCN concentrations in the MMF is caused in part by a smaller increase in aerosol lifetime from PI to PD in the MMF, a positive feedback in aerosol indirect effects induced by cloud lifetime effects. The smaller response in LWP to anthropogenic aerosols in the MMF model is consistent with observations and with high resolution model studies, which may indicate that aerosol indirect effects simulated in conventional global climate models are overestimated and point to the need to use global high resolution models, such as MMF models or global CRMs, to study aerosol indirect effects. The simulated total anthropogenic aerosol effect in the MMF is −1.05 W m−2, which is close to the Murphy et al. (2009) inverse estimate of −1.1 ± 0.4 W m−2 (1σ) based on the examination of the Earth's energy balance. Further improvements in the representation of ice nucleation and low clouds are needed.


2021 ◽  
Author(s):  
Isabel L. McCoy ◽  
Daniel T. McCoy ◽  
Robert Wood ◽  
Paquita Zuidema ◽  
Frida A.-M. Bender

<p>Mesoscale cellular convective (MCC) clouds occur in large-scale patterns over the ocean, are prevalent in sub-tropical cloud regions and mid-latitudes, and have important radiative impacts on the climate system. On average, closed MCC clouds have higher albedos than open or disorganized MCC clouds for the same cloud fraction which suggests differences in micro- and macro-physical characteristics between MCC morphologies. Marine cold air outbreaks (MCAOs) influence the development of open MCC clouds and the transition from closed to open MCC clouds in the mid-latitudes. A MCAO index, M, combines atmospheric surface forcing and static stability and can be used to examine global MCC morphology dependencies. MCC cloud morphology occurrence is also expected to shift with sea surface temperature (SST) changes as the climate warms. Analysis of MCC identifications (derived from a neural network classifier applied to MODIS satellite collection 6 liquid water path retrievals) and ECMWF ERA5 reanalysis data shows that closed MCC cloud occurrence shifts to open or disorganized MCC within an M-SST space. Global climate models (GCMs) predict that M will change regionally in strength as SSTs increase. Based on our derived MCC-M-SST relationship in the current climate, closed MCC occurrence frequency is expected to increase with a weakening of M but decrease with an increase in SSTs. This results in a shift to cloud morphologies with lower albedos. Cloud controlling factor analysis is used to estimate the resulting low cloud morphology feedback which is found to be spatially varied and between ±0.15 W m<sup>-2</sup> K<sup>-1</sup>. Because the morphology feedback is estimated to be positive in the extra-tropics and is not currently represented in GCMs, this implies a higher climate sensitivity than GCMs currently estimate.</p>


2021 ◽  
Author(s):  
xiao li ◽  
minghuai wang ◽  
yawen liu ◽  
yiquan jiang ◽  
xinyi dong

<h3>Knowledge of aerosol concentration, type, and physical and chemical properties is necessary to understand their role in Earth’s climate system. However, CMIP6 models’ performance of AOD simulation in China lacks a comprehensive evaluation and the potential improvement for CMIP6 models is still unclear. Here, we assess the performance of CMIP6 models in simulating annual mean AOD climatology and its seasonality over China from 2000 to 2014 and explore the underlying reasons for its performance. Compared with CMIP5, CMIP6 models can better capture the annual mean AOD climatology magnitude over Eastern Central China (ECC) with a notable enhancement of 52.98% due to a significant increase in the dominate sulfate aerosol. However, the majority of CMIP6 models fail to capture the observed inverted “V-like” pattern that depicts two centers of maximum AOD in spring over northeast China (NEC) and in summer over southeast China (SEC), respectively. The deficiency of two maximums by CMIP6 models is separately due to the negative bias in the simulation of organic aerosol (OA) AOD and sulfate AOD. Our analysis suggests that the deviation of simulated precipitation, relative humidity (RH), and liquid water path (LWP) in CMIP6 models contributes to the deviation of simulated sulfate AOD through affecting sulfate aerosol concentration by wet deposition and aqueous-phase production. Therefore, this study illustrates the urgent need to improve AOD simulation in global climate models.</h3>


2020 ◽  
Author(s):  
Kevin Grise ◽  
Sean Davis

<p><strong>            </strong>One of the most robust aspects of the atmospheric circulation response to increasing greenhouse gases is the poleward shift in the subsiding branches of the Hadley circulation, potentially pushing subtropical dry zones poleward toward midlatitudes.  Numerous lines of observational evidence suggest that this tropical expansion may have already begun.  Yet, the degree to which the observed tropical widening is anthropogenically forced has remained a topic of great debate, as previous studies have attributed the recent circulation trends to some combination of increasing greenhouse gases, stratospheric ozone depletion, anthropogenic aerosols, and natural variability.  During the past few years, two international working groups have synthesized recent findings about the magnitude and causes of the observed tropical widening, primarily using output from global climate models that participated in phase 5 of the Coupled Model Intercomparison Project (CMIP5).  In this presentation, we update those findings using the recently released CMIP6 global climate models.</p><p>            Over recent decades, the poleward expansion of the Hadley circulation estimated from modern reanalyses is relatively modest (< 0.5 degrees latitude per decade).  The reanalysis trends have similar magnitudes in the annual mean in the Northern Hemisphere (NH) and Southern Hemisphere (SH), but both CMIP5 and CMIP6 models suggest that increasing greenhouse gases should drive 2–3 times larger circulation shifts in the SH.  The reanalysis trends fall within the bounds of the models’ simulations of the late 20<sup>th</sup> century and early 21<sup>st</sup> century, although prescribing observed coupled atmosphere-ocean variability allows the models to better capture the observed trends in the NH.  We find two notable differences between CMIP5 and CMIP6 models.  First, both CMIP5 and CMIP6 models contract the NH summertime Hadley circulation equatorward (particularly over the Pacific sector) in response to increasing greenhouse gases, but this contraction is larger in CMIP6 models due to their higher average climate sensitivity.  Second, in recent decades, the poleward shift of the NH annual-mean Hadley cell edge is slightly larger in the historical runs of CMIP6 models.  Increasing greenhouse gases drive similar trends in CMIP5 and CMIP6 models, so CMIP6 models imply a stronger role for other forcings (such as aerosols) in recent circulation trends than CMIP5 models.</p>


2004 ◽  
Vol 4 (6) ◽  
pp. 7561-7614 ◽  
Author(s):  
U. Lohmann ◽  
J. Feichter

Abstract. Aerosols affect the climate system by changing cloud characteristics in many ways. They act as cloud condensation and ice nuclei, they may inhibit freezing and they could have an influence on the hydrological cycle. While the cloud albedo enhancement (Twomey effect) of warm clouds received most attention so far and traditionally is the only indirect aerosol forcing considered in transient climate simulations, here we discuss the multitude of effects. Different approaches how the climatic implications of these aerosol effects can be estimated globally as well as improvements that are needed in global climate models in order to better represent indirect aerosol effects are discussed in this paper.


2021 ◽  
Vol 21 (4) ◽  
pp. 3103-3121
Author(s):  
Zhibo Zhang ◽  
Qianqian Song ◽  
David B. Mechem ◽  
Vincent E. Larson ◽  
Jian Wang ◽  
...  

Abstract. In the current global climate models (GCMs), the nonlinearity effect of subgrid cloud variations on the parameterization of warm-rain process, e.g., the autoconversion rate, is often treated by multiplying the resolved-scale warm-rain process rates by a so-called enhancement factor (EF). In this study, we investigate the subgrid-scale horizontal variations and covariation of cloud water content (qc) and cloud droplet number concentration (Nc) in marine boundary layer (MBL) clouds based on the in situ measurements from a recent field campaign and study the implications for the autoconversion rate EF in GCMs. Based on a few carefully selected cases from the field campaign, we found that in contrast to the enhancing effect of qc and Nc variations that tends to make EF > 1, the strong positive correlation between qc and Nc results in a suppressing effect that tends to make EF < 1. This effect is especially strong at cloud top, where the qc and Nc correlation can be as high as 0.95. We also found that the physically complete EF that accounts for the covariation of qc and Nc is significantly smaller than its counterpart that accounts only for the subgrid variation of qc, especially at cloud top. Although this study is based on limited cases, it suggests that the subgrid variations of Nc and its correlation with qc both need to be considered for an accurate simulation of the autoconversion process in GCMs.


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