scholarly journals Picosecond-resolution phase-sensitive imaging of transparent objects in a single shot

2020 ◽  
Vol 6 (3) ◽  
pp. eaay6200 ◽  
Author(s):  
Taewoo Kim ◽  
Jinyang Liang ◽  
Liren Zhu ◽  
Lihong V. Wang

With the growing interest in the optical imaging of ultrafast phenomena in transparent objects, from shock wave to neuronal action potentials, high contrast imaging at high frame rates has become desirable. While phase sensitivity provides the contrast, the frame rates and sequence depths are highly limited by the detectors. Here, we present phase-sensitive compressed ultrafast photography (pCUP) for single-shot real-time ultrafast imaging of transparent objects by combining the contrast of dark-field imaging with the speed and the sequence depth of CUP. By imaging the optical Kerr effect and shock wave propagation, we demonstrate that pCUP can image light-speed phase signals in a single shot with up to 350 frames captured at up to 1 trillion frames per second. We expect pCUP to be broadly used for a vast range of fundamental and applied sciences.

2009 ◽  
Vol 15 (S2) ◽  
pp. 1082-1083
Author(s):  
D Masiel ◽  
B Reed ◽  
T LaGrange ◽  
ND Browning

Extended abstract of a paper presented at Microscopy and Microanalysis 2009 in Richmond, Virginia, USA, July 26 – July 30, 2009


2021 ◽  
Vol 118 (9) ◽  
pp. e2022319118
Author(s):  
Hongchang Wang ◽  
Kawal Sawhney

Ever since the discovery of X-rays, tremendous efforts have been made to develop new imaging techniques for unlocking the hidden secrets of our world and enriching our understanding of it. X-ray differential phase contrast imaging, which measures the gradient of a sample’s phase shift, can reveal more detail in a weakly absorbing sample than conventional absorption contrast. However, normally only the gradient’s component in two mutually orthogonal directions is measurable. In this article, omnidirectional differential phase images, which record the gradient of phase shifts in all directions of the imaging plane, are efficiently generated by scanning an easily obtainable, randomly structured modulator along a spiral path. The retrieved amplitude and main orientation images for differential phase yield more information than the existing imaging methods. Importantly, the omnidirectional dark-field images can be simultaneously extracted to study strongly ordered scattering structures. The proposed method can open up new possibilities for studying a wide range of complicated samples composed of both heavy, strongly scattering atoms and light, weakly scattering atoms.


Author(s):  
R.A. Herring ◽  
M.E. Twigg

Hollow cone illumination using a large C2 blocked-aperture (bl apt) in the conventional TEM (CTEM) can remove the beams within the zero-order Laue zone (ZOLZ) thereby making lattice images more simply interpretable. Dark-field (DF) hollow cone illumination has the added advantage of enhancing the Z-contrast within the lattice image, since the electrons contributing to the image must be scattered over a large angle (approximately 10 mrad). Both of these imaging methods have been explored, using a 600 um C2 bl apt and objective aperture sizes of 70, 20 and 10 um, and are reported in this paper.Much interest has been generated by the report of Pennycook [1] on STEM Z-contrast imaging using annular dark-field. In earlier work ,it was noted that CTEM hollow cone imaging and STEM annular dark-field imaging are related via reciprocity [2] (Fig. 1). In addition, Zernike has shown the advantages of hollow cone illumination in optical phase-contrast microscopy [3]. The electron-optical analogues to these optical techniques are now possible because of the low Cs values achieved in modern TEMs.


2018 ◽  
Vol 4 (10) ◽  
pp. 113
Author(s):  
Simon Zabler

Very early, in 1896, Wilhelm Conrad Röntgen, the founding father of X-rays, attempted to measure diffraction and refraction by this new kind of radiation, in vain. Only 70 years later, these effects were measured by Ulrich Bonse and Michael Hart who used them to make full-field images of biological specimen, coining the term phase-contrast imaging. Yet, another 30 years passed until the Talbot effect was rediscovered for X-radiation, giving rise to a micrograting based interferometer, replacing the Bonse–Hart interferometer, which relied on a set of four Laue-crystals for beam splitting and interference. By merging the Lau-interferometer with this Talbot-interferometer, another ten years later, measuring X-ray refraction and X-ray scattering full-field and in cm-sized objects (as Röntgen had attempted 110 years earlier) became feasible in every X-ray laboratory around the world. Today, now that another twelve years have passed and we are approaching the 125th jubilee of Röntgen’s discovery, neither Laue-crystals nor microgratings are a necessity for sensing refraction and scattering by X-rays. Cardboard, steel wool, and sandpaper are sufficient for extracting these contrasts from transmission images, using the latest image reconstruction algorithms. This advancement and the ever rising number of applications for phase-contrast and dark-field imaging prove to what degree our understanding of imaging physics as well as signal processing have advanced since the advent of X-ray physics, in particular during the past two decades. The discovery of the electron, as well as the development of electron imaging technology, has accompanied X-ray physics closely along its path, both modalities exploring the applications of new dark-field contrast mechanisms these days. Materials science, life science, archeology, non-destructive testing, and medicine are the key faculties which have already integrated these new imaging devices, using their contrast mechanisms in full. This special issue “Phase-Contrast and Dark-field Imaging” gives us a broad yet very to-the-point glimpse of research and development which are currently taking place in this very active field. We find reviews, applications reports, and methodological papers of very high quality from various groups, most of which operate X-ray scanners which comprise these new imaging modalities.


2018 ◽  
Vol 63 (18) ◽  
pp. 185010 ◽  
Author(s):  
Maria Seifert ◽  
Veronika Ludwig ◽  
Michael Gallersdörfer ◽  
Christian Hauke ◽  
Katharina Hellbach ◽  
...  

1996 ◽  
Vol 4 (9) ◽  
pp. 14-15
Author(s):  
Michael Kersker

High Angle Dark Field Imaging, or Z contrast imaging, is an Imaging method. It takes advantage of the useful fact that if one uses the high angle scattering intensities and eliminates the elastic scattered (diffracted) beams from the image (by using a Howie type angular dark field detector), the remaining image will be characterized by, if the probe used is on the order of the atomic dimensions, intensity modulations that reveal atom positions and relative atomic number. In simple terms, the image will display Z-contrast at the atomic level and can differentiate columns of heavy atoms from columns of lighter ones.


2001 ◽  
Vol 7 (S2) ◽  
pp. 214-215
Author(s):  
R.F. Klie ◽  
N.D. Browning

Mixed conductors have been the focus of many studies in the last decade, leading to a detailed understanding of many of the macroscopic bulk properties of these materials. in particular, although the reduced low temperature phase in rare earth perovskite oxides is commonly explained in terms of ordered brownmillerite structured micro domains, its transition to the high temperature phase remains elusive. in this presentation an investigation of (La, Sr)FeO3, prepared under different reducing conditions through correlated atomic resolution annular dark field imaging and electron energy loss spectroscopy will be shown.We investigate the (La, Sr)FeO3 material by atomic resolution Z-contrast imaging and EELS using a 200 keV STEM/TEM JEOL2010F with a post column GIF. The combination of these techniques allows us to obtain direct images from the atomic structure of the bulk sample and to correlate this with the atomically resolved EELS information. In-situ heating of the material in a heating double tilt holder in the microscope columns allows us to simulate the highly reducing operating conditions for this oxygen conducting membrane material.


2021 ◽  
Vol 7 (12) ◽  
pp. 249
Author(s):  
Zhi Qiao ◽  
Xianbo Shi ◽  
Michael Wojcik ◽  
Lahsen Assoufid

Near-field X-ray speckle tracking has been used in phase-contrast imaging and tomography as an emerging technique, providing higher contrast images than traditional absorption radiography. Most reported methods use sandpaper or membrane filters as speckle generators and digital image cross-correlation for phase reconstruction, which has either limited resolution or requires a large number of position scanning steps. Recently, we have proposed a novel coded-mask-based multi-contrast imaging (CMMI) technique for single-shot measurement with superior performance in efficiency and resolution compared with other single-shot methods. We present here a scanning CMMI method for the ultimate imaging resolution and phase sensitivity by using a coded mask as a high-contrast speckle generator, the flexible scanning mode, the adaption of advanced maximum-likelihood optimization to scanning data, and the multi-resolution analysis. Scanning CMMI can outperform other speckle-based imaging methods, such as X-ray speckle vector tracking, providing higher quality absorption, phase, and dark-field images with fewer scanning steps. Scanning CMMI is also successfully demonstrated in multi-contrast tomography, showing great potentials in high-resolution full-field imaging applications, such as in vivo biomedical imaging.


2019 ◽  
Vol 9 (1) ◽  
Author(s):  
Youngju Kim ◽  
Jacopo Valsecchi ◽  
Jongyul Kim ◽  
Seung Wook Lee ◽  
Markus Strobl

AbstractWe introduce the application of a symmetric Talbot-Lau neutron grating interferometer which provides a significantly extended autocorrelation length range essential for quantitative dark-field contrast imaging. The highly efficient set-up overcomes the limitation of the conventional Talbot-Lau technique to a severely limited micrometer range as well as the limitation of the other advanced dark-field imaging techniques in the nanometer regime. The novel set-up enables efficient and continuous dark-field contrast imaging providing quantitative small-angle neutron scattering information for structures in a regime from some tens of nanometers to several tens of micrometers. The quantitative analysis enabled in and by such an extended range is demonstrated through application to reference sample systems of the diluted polystyrene particle in aqueous solutions. Here we additionally demonstrate and successfully discuss the correction for incoherent scattering. This correction results to be necessary to achieve meaningful quantitative structural results. Furthermore, we present the measurements, data modelling and analysis of the two distinct kinds of cohesive powders enabled by the novel approach, revealing the significant structural differences of their fractal nature.


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