scholarly journals Manipulating surface magnetic order in iron telluride

2019 ◽  
Vol 5 (3) ◽  
pp. eaav3478 ◽  
Author(s):  
Christopher Trainer ◽  
Chi M. Yim ◽  
Christoph Heil ◽  
Feliciano Giustino ◽  
Dorina Croitori ◽  
...  

Control of emergent magnetic orders in correlated electron materials promises new opportunities for applications in spintronics. For their technological exploitation, it is important to understand the role of surfaces and interfaces to other materials and their impact on the emergent magnetic orders. Here, we demonstrate for iron telluride, the nonsuperconducting parent compound of the iron chalcogenide superconductors, determination and manipulation of the surface magnetic structure by low-temperature spin-polarized scanning tunneling microscopy. Iron telluride exhibits a complex structural and magnetic phase diagram as a function of interstitial iron concentration. Several theories have been put forward to explain the different magnetic orders observed in the phase diagram, which ascribe a dominant role either to interactions mediated by itinerant electrons or to local moment interactions. Through the controlled removal of surface excess iron, we can separate the influence of the excess iron from that of the change in the lattice structure.

Science ◽  
2014 ◽  
Vol 345 (6197) ◽  
pp. 653-656 ◽  
Author(s):  
Mostafa Enayat ◽  
Zhixiang Sun ◽  
Udai Raj Singh ◽  
Ramakrishna Aluru ◽  
Stefan Schmaus ◽  
...  

Spin-polarized scanning tunneling microscopy (SP-STM) has been used extensively to study magnetic properties of nanostructures. Using SP-STM to visualize magnetic order in strongly correlated materials on an atomic scale is highly desirable, but challenging. We achieved this goal in iron tellurium (Fe1+yTe), the nonsuperconducting parent compound of the iron chalcogenides, by using a STM tip with a magnetic cluster at its apex. Our images of the magnetic structure reveal that the magnetic order in the monoclinic phase is a unidirectional stripe order; in the orthorhombic phase at higher excess iron concentration (y > 0.12), a transition to a phase with coexisting magnetic orders in both directions is observed. It may be possible to generalize the technique to other high-temperature superconductor families, such as the cuprates.


1988 ◽  
Vol 49 (C8) ◽  
pp. C8-479-C8-480 ◽  
Author(s):  
M. Kuznietz ◽  
P. Burlet ◽  
J. Rossat-Mignod ◽  
O. Vogt ◽  
K. Mattenberger ◽  
...  

1993 ◽  
Vol 07 (01n03) ◽  
pp. 867-870 ◽  
Author(s):  
H. SHIRAISHI ◽  
T. HORI ◽  
Y. YAMAGUCHI ◽  
S. FUNAHASHI ◽  
K. KANEMATSU

The magnetic susceptibility measurements have been made on antiferromagnetic compounds Mn1–xFexSn2 and the magnetic phase diagram was illustrated. The high temperature magnetic phases I and III, major phases, were analyzed on the basis of molecular field theory and explained the change of magnetic structure I⇌III occured at x≈0.8.


2021 ◽  
Vol 132 ◽  
pp. 107134
Author(s):  
Piotr Konieczny ◽  
Stanisław M. Dubiel

2021 ◽  
Vol 12 (1) ◽  
Author(s):  
Jan Ravnik ◽  
Michele Diego ◽  
Yaroslav Gerasimenko ◽  
Yevhenii Vaskivskyi ◽  
Igor Vaskivskyi ◽  
...  

AbstractMetastable self-organized electronic states in quantum materials are of fundamental importance, displaying emergent dynamical properties that may be used in new generations of sensors and memory devices. Such states are typically formed through phase transitions under non-equilibrium conditions and the final state is reached through processes that span a large range of timescales. Conventionally, phase diagrams of materials are thought of as static, without temporal evolution. However, many functional properties of materials arise as a result of complex temporal changes in the material occurring on different timescales. Hitherto, such properties were not considered within the context of a temporally-evolving phase diagram, even though, under non-equilibrium conditions, different phases typically evolve on different timescales. Here, by using time-resolved optical techniques and femtosecond-pulse-excited scanning tunneling microscopy (STM), we track the evolution of the metastable states in a material that has been of wide recent interest, the quasi-two-dimensional dichalcogenide 1T-TaS2. We map out its temporal phase diagram using the photon density and temperature as control parameters on timescales ranging from 10−12 to 103 s. The introduction of a time-domain axis in the phase diagram enables us to follow the evolution of metastable emergent states created by different phase transition mechanisms on different timescales, thus enabling comparison with theoretical predictions of the phase diagram, and opening the way to understanding of the complex ordering processes in metastable materials.


1990 ◽  
Vol 83 (1-3) ◽  
pp. 313-314 ◽  
Author(s):  
M. Bacmann ◽  
D. Fruchart ◽  
B. Chenevier ◽  
R. Fruchart ◽  
J.A. Puertolas ◽  
...  

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