Effects of a finite spectral bandwidth light source in time-resolved diffuse spectroscopy

2009 ◽  
Author(s):  
Andrea Farina ◽  
Andrea Bassi ◽  
Paola Taroni ◽  
Daniela Comelli ◽  
Lorenzo Spinelli ◽  
...  
Author(s):  
Andrea Farina ◽  
Andrea Bassi ◽  
Paola Taroni ◽  
Daniela Comelli ◽  
Lorenzo Spinelli ◽  
...  

Author(s):  
Andrea Farina ◽  
Andrea Bassi ◽  
Paola Taroni ◽  
Daniela Comelli ◽  
Lorenzo Spinelli ◽  
...  

2019 ◽  
Author(s):  
Haoke Zhang ◽  
Lili Du ◽  
Lin Wang ◽  
Junkai Liu ◽  
Qing Wan ◽  
...  

<p>Building molecular machine has long been a dream of scientists as it is expected to revolutionize many aspects of technology and medicine. Implementing the solid-state molecular motion is the prerequisite for a practical molecular machine. However, few works on solid-state molecular motion have been reported and it is almost impossible to “see” the motion even if it happens. Here the light-driven molecular motion in solid state is discovered in two non-conjugated molecules <i>s</i>-DPE and <i>s</i>-DPE-TM, resulting in the formation of excited-state though-space complex (ESTSC). Meanwhile, the newly formed ESTSC generates an abnormal visible emission which is termed as clusteroluminescence. Notably, the original packing structure can recover from ESTSC when the light source is removed. These processes have been confirmed by time-resolved spectroscopy and quantum mechanics calculation. This work provides a new strategy to manipulate and “see” solid-state molecular motion and gains new insights into the mechanistic picture of clusteroluminescence.<br></p>


2015 ◽  
Vol 51 (5) ◽  
pp. 408-409
Author(s):  
Yu. Kostin ◽  
A. Chamorovskiy ◽  
S.D. Yakubovich

2007 ◽  
Author(s):  
C. Martel ◽  
S. Fourmaux ◽  
C. Y. Côté ◽  
S. Magnan ◽  
L. Lecherbourg ◽  
...  

2021 ◽  
Vol 11 (24) ◽  
pp. 11850
Author(s):  
Kaiqing Zhang ◽  
Yin Kang ◽  
Tao Liu ◽  
Zhen Wang ◽  
Chao Feng ◽  
...  

Terahertz (THz) radiation sources are increasingly significant for many scientific frontiers, while the generation of THz radiation with high-power at wide-tunable frequencies is still a limitation for most existing methods. In this paper, a compact accelerator-based light source is proposed to produce coherent THz radiation with high pulse energy and tunable frequency from 0.1 THz to 60 THz. By using a frequency beating laser-modulated electron beam and undulator taper, intense coherent THz radiation can be generated through undulators. Theoretical analysis and numerical simulations demonstrate that the proposed technique can generate narrow-bandwidth THz radiation with a pulse energy up to 6.3 millijoule (mJ) and the three-dimensional effects of beam has limited influence on its performance. The proposed technique will open up new opportunities for THz spectroscopic and time-resolved experiments.


2001 ◽  
Vol 480 (3) ◽  
pp. 173-179 ◽  
Author(s):  
C Quitmann ◽  
U Flechsig ◽  
L Patthey ◽  
T Schmidt ◽  
G Ingold ◽  
...  

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