scholarly journals Femtosecond excited-state absorption dynamics and optical limiting in fullerene solutions, sol-gel glasses, and thin films

Author(s):  
Duncan W. McBranch ◽  
Victor I. Klimov ◽  
Laura B. Smilowitz ◽  
M. Grigorova ◽  
Jeanne M. Robinson ◽  
...  
1997 ◽  
Vol 488 ◽  
Author(s):  
R. Kohlman ◽  
V. Klimov ◽  
X. Shi ◽  
M. Grigorova ◽  
B. R. Mattes ◽  
...  

AbstractWe review our results from spectral studies of the ultrafast excited-state absorption in fullerenes and derivatized fullerenes. These results allow determination of both the spectral response of reverse saturable absorption (RSA) nonlinearities such as optical limiting (OL) in fullerenes, and the dynamical response for different morphologies. We have investigated the effects of thin film and various sol-gel glass environments on the nanosecond OL and femtosecond dynamics of derivatized fullerenes. These data provide evidence of decay pathways which compete with the intersystem crossing to a triplet from the initial singlet states. With appropriate processing, however, the OL response of derivatized-fullerene sol-gel glasses can be enhanced to approach that of the same molecule in solution, while significantly enhancing the optical damage threshold. The optical limiting of these derivatized fullerenes is compared with that of various porphyrin and phthalocyanine molecules.


2021 ◽  
Vol 24 (3) ◽  
pp. 38-42
Author(s):  
Marwa Mudfer Alqaisi ◽  
◽  
Alla J. Ghazai ◽  

In this work, pure Zinc oxide and tin doped Zinc oxide thin films nanoparticles with various volume concentrations of 2, 4, 6, and 8V/V% were prepared by using the sol-gel method. The optical properties were investigated by using UV-Visible spectroscope, and the value exhibits the direct allowed transition. The average of transmittance was around ~(17-23) %in visible region. The optical energy band gap was calculated with wavelength (300-900) nm for pure ZnO and Sn doped ZnO thin films which decreases with increasing concentration from 3.4 eV to 3.1 eV respectively and red shift. The real dielectric(εr) and the imaginary dielectric εiare the same behavior of the refractive index(n) the extinction coefficient (k) respectively. The optical limiting properties were studied by using an SDL laser with a wavelength of 235 nm. ZnO and doping thin films an found efficient as optic limiting and depend on the concentration of the all samples.


2019 ◽  
Vol 237 ◽  
pp. 121827 ◽  
Author(s):  
C. Babeela ◽  
N.K. Siji Narendran ◽  
Mehboobali Pannipara ◽  
Abdullah G. Al-Sehemi ◽  
T.C. Sabari Girisun

2000 ◽  
Vol 319 (5-6) ◽  
pp. 494-500 ◽  
Author(s):  
Carlos Silva ◽  
David M Russell ◽  
Mark A Stevens ◽  
J.Devin Mackenzie ◽  
Sepas Setayesh ◽  
...  

2005 ◽  
Vol 87 (6) ◽  
pp. 063104 ◽  
Author(s):  
Parinda Vasa ◽  
Pushan Ayyub ◽  
B. P. Singh

2000 ◽  
Vol 88 (4) ◽  
pp. 1726-1732 ◽  
Author(s):  
J. Staromlynska ◽  
T. J. McKay ◽  
P. Wilson

2016 ◽  
Vol 62 ◽  
pp. 110-118 ◽  
Author(s):  
Kamal P. Mani ◽  
Perumbilavil Sreekanth ◽  
G. Vimal ◽  
P.R. Biju ◽  
N.V. Unnikrishnan ◽  
...  

1996 ◽  
Vol 10 (01n02) ◽  
pp. 61-67 ◽  
Author(s):  
RIJU C. ISSAC ◽  
C.V. BINDHU ◽  
S.S. HARILAL ◽  
GEETHA K. VARIER ◽  
V.P.N. NAMPOORI ◽  
...  

Pulsed photoacoustic studies in solution of C 60 in toluene have been made using the 532 nm radiation from a frequency doubled Nd:YAG laser. Though C 60 is found to exhibit the phenomenon of optical limiting, the results on photoacoustic measurements do not give any indication of multiphoton transitions as suggested in some of the earlier works. Results of photoacoustic measurements show that excited state absorption is the dominant process responsible for optical limiting while phenomena like nonlinear scattering may contribute to a lesser extent.


Author(s):  
J. W. Perry ◽  
L. R. Khundkar ◽  
D. R. Coulter ◽  
D. Alvarez ◽  
S. R. Marder ◽  
...  

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