Quantifying methane emissions in Delaware from field-based mid-IR sensors and satellite observations

2021 ◽  
Author(s):  
Carlos Garcia Diaz ◽  
Zakaria Juracka ◽  
Al R. Alexis ◽  
Mohammad A. Khan
2018 ◽  
Vol 18 (21) ◽  
pp. 15959-15973 ◽  
Author(s):  
Yuzhong Zhang ◽  
Daniel J. Jacob ◽  
Joannes D. Maasakkers ◽  
Melissa P. Sulprizio ◽  
Jian-Xiong Sheng ◽  
...  

Abstract. The hydroxyl radical (OH) is the main tropospheric oxidant and the main sink for atmospheric methane. The global abundance of OH has been monitored for the past decades using atmospheric methyl chloroform (CH3CCl3) as a proxy. This method is becoming ineffective as atmospheric CH3CCl3 concentrations decline. Here we propose that satellite observations of atmospheric methane in the short-wave infrared (SWIR) and thermal infrared (TIR) can provide an alternative method for monitoring global OH concentrations. The premise is that the atmospheric signature of the methane sink from oxidation by OH is distinct from that of methane emissions. We evaluate this method in an observing system simulation experiment (OSSE) framework using synthetic SWIR and TIR satellite observations representative of the TROPOMI and CrIS instruments, respectively. The synthetic observations are interpreted with a Bayesian inverse analysis, optimizing both gridded methane emissions and global OH concentrations. The optimization is done analytically to provide complete error accounting, including error correlations between posterior emissions and OH concentrations. The potential bias caused by prior errors in the 3-D seasonal OH distribution is examined using OH fields from 12 different models in the ACCMIP archive. We find that the satellite observations of methane have the potential to constrain the global tropospheric OH concentration with a precision better than 1 % and an accuracy of about 3 % for SWIR and 7 % for TIR. The inversion can successfully separate the effects of perturbations to methane emissions and to OH concentrations. Interhemispheric differences in OH concentrations can also be successfully retrieved. Error estimates may be overoptimistic because we assume in this OSSE that errors are strictly random and have no systematic component. The availability of TROPOMI and CrIS data will soon provide an opportunity to test the method with actual observations.


2020 ◽  
Author(s):  
David R. Lyon ◽  
Benjamin Hmiel ◽  
Ritesh Gautam ◽  
Mark Omara ◽  
Kate Roberts ◽  
...  

Abstract. Methane emissions associated with the production, transport, and use of oil and natural gas increase the climatic impacts of energy use; however, little is known about how emissions vary temporally and with commodity prices. We present airborne and ground-based data, supported by satellite observations, to measure weekly to monthly changes in total methane emissions in the United States’ Permian Basin during a period of volatile oil prices associated with the COVID-19 pandemic. As oil prices declined from ~$ 60 to $ 20 per barrel, emissions changed concurrently from 3.4 % to 1.5 % of gas production; as prices partially recovered, emissions increased back to near initial values. Concurrently, total oil and natural gas production only declined by a maximum of ~10 % from the peak values seen in the months prior to the crash. Activity data indicate that a rapid decline in well development and subsequent effects on associated gas flaring and midstream infrastructure throughput are the likely drivers of temporary emission reductions. Our results, along with past satellite observations, suggest that under more typical price conditions, the Permian Basin is in a state of overcapacity in which rapidly growing natural gas production exceeds midstream capacity and leads to high methane emissions.


2008 ◽  
Vol 8 (21) ◽  
pp. 6341-6353 ◽  
Author(s):  
J. F. Meirink ◽  
P. Bergamaschi ◽  
M. C. Krol

Abstract. A four-dimensional variational (4D-Var) data assimilation system for inverse modelling of atmospheric methane emissions is presented. The system is based on the TM5 atmospheric transport model. It can be used for assimilating large volumes of measurements, in particular satellite observations and quasi-continuous in-situ observations, and at the same time it enables the optimization of a large number of model parameters, specifically grid-scale emission rates. Furthermore, the variational method allows to estimate uncertainties in posterior emissions. Here, the system is applied to optimize monthly methane emissions over a 1-year time window on the basis of surface observations from the NOAA-ESRL network. The results are rigorously compared with an analogous inversion by Bergamaschi et al. (2007), which was based on the traditional synthesis approach. The posterior emissions as well as their uncertainties obtained in both inversions show a high degree of consistency. At the same time we illustrate the advantage of 4D-Var in reducing aggregation errors by optimizing emissions at the grid scale of the transport model. The full potential of the assimilation system is exploited in Meirink et al. (2008), who use satellite observations of column-averaged methane mixing ratios to optimize emissions at high spatial resolution, taking advantage of the zooming capability of the TM5 model.


2016 ◽  
Vol 16 (22) ◽  
pp. 14371-14396 ◽  
Author(s):  
Daniel J. Jacob ◽  
Alexander J. Turner ◽  
Joannes D. Maasakkers ◽  
Jianxiong Sheng ◽  
Kang Sun ◽  
...  

Abstract. Methane is a greenhouse gas emitted by a range of natural and anthropogenic sources. Atmospheric methane has been measured continuously from space since 2003, and new instruments are planned for launch in the near future that will greatly expand the capabilities of space-based observations. We review the value of current, future, and proposed satellite observations to better quantify and understand methane emissions through inverse analyses, from the global scale down to the scale of point sources and in combination with suborbital (surface and aircraft) data. Current global observations from Greenhouse Gases Observing Satellite (GOSAT) are of high quality but have sparse spatial coverage. They can quantify methane emissions on a regional scale (100–1000 km) through multiyear averaging. The Tropospheric Monitoring Instrument (TROPOMI), to be launched in 2017, is expected to quantify daily emissions on the regional scale and will also effectively detect large point sources. A different observing strategy by GHGSat (launched in June 2016) is to target limited viewing domains with very fine pixel resolution in order to detect a wide range of methane point sources. Geostationary observation of methane, still in the proposal stage, will have the unique capability of mapping source regions with high resolution, detecting transient "super-emitter" point sources and resolving diurnal variation of emissions from sources such as wetlands and manure. Exploiting these rapidly expanding satellite measurement capabilities to quantify methane emissions requires a parallel effort to construct high-quality spatially and sectorally resolved emission inventories. Partnership between top-down inverse analyses of atmospheric data and bottom-up construction of emission inventories is crucial to better understanding methane emission processes and subsequently informing climate policy.


2016 ◽  
Author(s):  
Daniel J. Jacob ◽  
Alexander J. Turner ◽  
Joannes D. Maasakkers ◽  
Jianxiong Sheng ◽  
Kang Sun ◽  
...  

Abstract. Methane is a greenhouse gas emitted by a range of natural and anthropogenic sources. Atmospheric methane has been measured continuously from space since 2003, and new instruments are planned for launch in the near future that will greatly expand the capabilities of space-based observations. We review the value of current, future, and proposed satellite observations to better quantify and understand methane emissions through inverse analyses, down to the scale of point sources and in combination with suborbital (surface and aircraft) data. Current observations from GOSAT are of high quality but have sparse spatial coverage. They provide limited information to quantify methane emissions on a regional (100–1000 km) scale. TROPOMI to be launched in late 2016 is expected to quantify daily emissions on the regional scale and will also effectively detect large point sources. Future satellite instruments with much higher spatial resolution, such as the recently launched GHGSat with 50 × 50 m2 resolution over targeted viewing domains, have the potential to detect a wide range of methane point sources. Geostationary observation of methane, still in the proposal stage, will have unique capability for mapping source regions with high resolution while also detecting transient "super-emitter" point sources. Exploiting the rapidly expanding satellite measurement capabilities to quantify methane emissions requires a parallel effort to construct high-quality spatially and sectorally resolved emission inventories. Partnership between top-down inverse analyses of atmospheric data and bottom-up construction of emission inventories is crucial to better understand methane emission processes and from there to inform climate policy.


Author(s):  
Pankaj Sadavarte ◽  
Sudhanshu Pandey ◽  
Joannes D. Maasakkers ◽  
Alba Lorente ◽  
Tobias Borsdorff ◽  
...  

2018 ◽  
Author(s):  
Yuzhong Zhang ◽  
Daniel J. Jacob ◽  
Joannes D. Maasakkers ◽  
Melissa P. Sulprizio ◽  
Jian-Xiong Sheng ◽  
...  

Abstract. The hydroxyl radical (OH) is the main tropospheric oxidant and is the largest sink for atmospheric methane. The global abundance of OH has been monitored for the past decades with the methyl chloroform (CH3CCl3) proxy. This approach is becoming ineffective as atmospheric CH3CCl3 concentrations decline. Here we propose that satellite observations of atmospheric methane in the shortwave infrared (SWIR) and thermal infrared (TIR) can provide an effective replacement method. The premise is that the atmospheric signature of the methane sink from oxidation by OH is distinct from that of methane emissions. We evaluate this method in an observing system simulation experiment (OSSE) framework using synthetic SWIR and TIR satellite observations representative of the TROPOMI and CrIS instruments, respectively. The synthetic observations are interpreted with a Bayesian inverse analysis optimizing both gridded methane emissions and global OH concentrations with detailed error accounting, including errors in meteorological fields and in OH distributions. We find that the satellite observations can constrain the global tropospheric OH concentrations with a precision better than 1 % and an accuracy of about 3 % for SWIR and 7 % for TIR. The inversion can successfully separate contributions from methane emissions and OH concentrations to the methane budget and its trend. We also show that satellite methane observations can constrain the interhemispheric difference in OH. The main limitation to the accuracy is uncertainty in the spatial and seasonal distribution of OH.


2020 ◽  
Vol 54 (16) ◽  
pp. 10246-10253 ◽  
Author(s):  
Daniel J. Varon ◽  
Daniel J. Jacob ◽  
Dylan Jervis ◽  
Jason McKeever

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