Custom high-sensitivity CCD and sCMOS detectors for high-harmonic generation, x-ray absorption spectroscopy, soft x-ray microscopy/tomography, and hard x-ray detection

2020 ◽  
Author(s):  
Justin T. Cooper ◽  
Adam J. Wise ◽  
Thomas Woodward ◽  
Antoine Varagnat
Keyword(s):  
Harmonic Generation ◽  
Absorption Spectroscopy ◽  
Generation X ◽  
High Harmonic ◽  
High Harmonic Generation ◽  
High Sensitivity ◽  
X Ray ◽  
X Ray Absorption

scholarly journals Transient absorption spectroscopy using high harmonic generation: a review of ultrafast X-ray dynamics in molecules and solids

2019 ◽  
Vol 377 (2145) ◽  
pp. 20170463 ◽  
Author(s):  
Romain Geneaux ◽  
Hugo J. B. Marroux ◽  
Alexander Guggenmos ◽  
Daniel M. Neumark ◽  
Stephen R. Leone
Keyword(s):  
Time Scales ◽  
Harmonic Generation ◽  
Absorption Spectroscopy ◽  
Transient Absorption ◽  
High Harmonic ◽  
High Harmonic Generation ◽  
Transient Absorption Spectroscopy ◽  
Spectroscopic Techniques ◽  
X Rays ◽  
X Ray

Attosecond science opened the door to observing nuclear and electronic dynamics in real time and has begun to expand beyond its traditional grounds. Among several spectroscopic techniques, X-ray transient absorption spectroscopy has become key in understanding matter on ultrafast time scales. In this review, we illustrate the capabilities of this unique tool through a number of iconic experiments. We outline how coherent broadband X-ray radiation, emitted in high-harmonic generation, can be used to follow dynamics in increasingly complex systems. Experiments performed in both molecules and solids are discussed at length, on time scales ranging from attoseconds to picoseconds, and in perturbative or strong-field excitation regimes. This article is part of the theme issue ‘Measurement of ultrafast electronic and structural dynamics with X-rays’.

scholarly journals Few-Cycle Infrared Pulse Evolving in FEL Oscillators and Its Application to High-Harmonic Generation for Attosecond Ultraviolet and X-ray Pulses

Atoms ◽  
2021 ◽  
Vol 9 (1) ◽  
pp. 15
Author(s):  
Ryoichi Hajima
Keyword(s):  
Harmonic Generation ◽  
Short Pulse ◽  
High Harmonic ◽  
High Harmonic Generation ◽  
Pulse Generation ◽  
Solid State Lasers ◽  
Linear Accelerators ◽  
X Ray ◽  
Ultrafast Science ◽  
Historical Remarks

Generation of few-cycle optical pulses in free-electron laser (FEL) oscillators has been experimentally demonstrated in FEL facilities based on normal-conducting and superconducting linear accelerators. Analytical and numerical studies have revealed that the few-cycle FEL lasing can be explained in the frame of superradiance, cooperative emission from self-bunched systems. In the present paper, we review historical remarks of superradiance FEL experiments in short-pulse FEL oscillators with emphasis on the few-cycle pulse generation and discuss the application of the few-cycle FEL pulses to the scheme of FEL-HHG, utilization of infrared FEL pulses to drive high-harmonic generation (HHG) from gas and solid targets. The FEL-HHG enables one to explore ultrafast science with attosecond ultraviolet and X-ray pulses with a MHz repetition rate, which is difficult with HHG driven by solid-state lasers. A research program has been launched to develop technologies for the FEL-HHG and to conduct a proof-of-concept experiment of FEL-HHG.

scholarly journals Attosecond soft X-ray high harmonic generation

2019 ◽  
Vol 377 (2145) ◽  
pp. 20170468 ◽  
Author(s):  
Allan S. Johnson ◽  
Timur Avni ◽  
Esben W. Larsen ◽  
Dane R. Austin ◽  
Jon P. Marangos
Keyword(s):  
Harmonic Generation ◽  
Spectral Range ◽  
High Harmonic ◽  
High Harmonic Generation ◽  
Intense Laser ◽  
X Rays ◽  
X Ray ◽  
Optical Phenomenon ◽  
Highly Nonlinear ◽  
Attosecond Pulses

High harmonic generation (HHG) of an intense laser pulse is a highly nonlinear optical phenomenon that provides the only proven source of tabletop attosecond pulses, and it is the key technology in attosecond science. Recent developments in high-intensity infrared lasers have extended HHG beyond its traditional domain of the XUV spectral range (10–150 eV) into the soft X-ray regime (150 eV to 3 keV), allowing the compactness, stability and sub-femtosecond duration of HHG to be combined with the atomic site specificity and electronic/structural sensitivity of X-ray spectroscopy. HHG in the soft X-ray spectral region has significant differences from HHG in the XUV, which necessitate new approaches to generating and characterizing attosecond pulses. Here, we examine the challenges and opportunities of soft X-ray HHG, and we use simulations to examine the optimal generating conditions for the development of high-flux, attosecond-duration pulses in the soft X-ray spectral range. This article is part of the theme issue ‘Measurement of ultrafast electronic and structural dynamics with X-rays’.

Apparatus for soft x-ray table-top high harmonic generation

2018 ◽  
Vol 89 (8) ◽  
pp. 083110 ◽  
Author(s):  
Allan S. Johnson ◽  
David Wood ◽  
Dane R. Austin ◽  
Christian Brahms ◽  
Andrew Gregory ◽  
...  
Keyword(s):  
Harmonic Generation ◽  
High Harmonic ◽  
High Harmonic Generation ◽  
X Ray

High-Order X-Ray Raman Scattering Using Coherent Electrons from High Harmonic Generation

2006 ◽  
Vol 17 (12) ◽  
pp. 43 ◽  
Author(s):  
Nicholas L. Wagner ◽  
Andrea Wüest ◽  
Ivan P. Christov ◽  
Tenio Popmintchev ◽  
Xibin Zhou ◽  
...  
Keyword(s):  
Raman Scattering ◽  
Harmonic Generation ◽  
High Harmonic ◽  
High Harmonic Generation ◽  
High Order ◽  
X Ray

scholarly journals Femtosecond soft–X–Ray absorption spectroscopy of liquids with a water-window high-harmonic source

2020 ◽  
Author(s):  
Tadas Balčiūnas ◽  
Adam D. Smith ◽  
Yi–Ping Chang ◽  
Cédric Schmidt ◽  
Kristina Zinchenko ◽  
...  
Keyword(s):  
Absorption Spectroscopy ◽  
High Harmonic ◽  
X Ray ◽  
Water Window ◽  
Harmonic Source ◽  
X Ray Absorption

scholarly journals Ultraviolet surprise: Efficient soft x-ray high-harmonic generation in multiply ionized plasmas

Science ◽  
2015 ◽  
Vol 350 (6265) ◽  
pp. 1225-1231 ◽  
Author(s):  
D. Popmintchev ◽  
C. Hernandez-Garcia ◽  
F. Dollar ◽  
C. Mancuso ◽  
J. A. Perez-Hernandez ◽  
...  
Keyword(s):  
Harmonic Generation ◽  
High Harmonic ◽  
High Harmonic Generation ◽  
X Ray ◽  
Ionized Plasmas
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